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Published work

110 published item(s)

preprint2026arXiv

M\textsuperscript{4}Fuse: Lightweight State-Space MoE with a Cross-Scale Gating Bridge for Brain Tumor Segmentation

Encoder-decoder imbalance and the reliance on large input volumes make many 3D brain tumor segmentation models both compute-heavy and brittle. We present M\textsuperscript{4}Fuse, a lightweight network that prioritizes discriminative brain tumor cues over exhaustive appearance reconstruction. Our method balances encoder and decoder capacity and replaces depth expansion with a synergistic design: it propagates long-range context with linear complexity via a grouped state space mixer, denoises and aligns skip features using a cross-scale dual-stage gating bridge, and absorbs cross-site acquisition shifts with a sample-level mixture-of-experts. On the BraTS2019 and BraTS2021 benchmarks, M\textsuperscript{4}Fuse outperforms other lightweight excellent methods in both parameter count and performance. Even at a challenging input resolution of \(64\times128\times128\) (half that of existing excellent models), M\textsuperscript{4}Fuse reduces parameters by 62.63\% and improves average performance by 0.09\%. Ablations of key components validate the method's exceptional parameter-to-accuracy efficiency and robustness across diverse data centers.

preprint2024arXiv

Point Cloud in the Air

Acquisition and processing of point clouds (PCs) is a crucial enabler for many emerging applications reliant on 3D spatial data, such as robot navigation, autonomous vehicles, and augmented reality. In most scenarios, PCs acquired by remote sensors must be transmitted to an edge server for fusion, segmentation, or inference. Wireless transmission of PCs not only puts on increased burden on the already congested wireless spectrum, but also confronts a unique set of challenges arising from the irregular and unstructured nature of PCs. In this paper, we meticulously delineate these challenges and offer a comprehensive examination of existing solutions while candidly acknowledging their inherent limitations. In response to these intricacies, we proffer four pragmatic solution frameworks, spanning advanced techniques, hybrid schemes, and distributed data aggregation approaches. In doing so, our goal is to chart a path toward efficient, reliable, and low-latency wireless PC transmission.

preprint2023arXiv

Feasibility Analysis of Grover-meets-Simon Algorithm

Quantum algorithm is a key tool for cryptanalysis. At present, people are committed to building powerful quantum algorithms and tapping the potential of quantum algorithms, so as to further analyze the security of cryptographic algorithms under quantum computing. Recombining classical quantum algorithms is one of the current ideas to construct quantum algorithms. However, they cannot be easily combined, the feasibility of quantum algorithms needs further analysis in quantum environment. This paper reanalyzes the existing combined algorithm Grover-meets-Simon algorithm in terms of the principle of deferred measurement. First of all, due to the collapse problem caused by the measurement, we negate the measurement process of Simon's algorithm during the process of the Grover-meets-Simon algorithm. Second, since the output of the unmeasured Simon algorithm is quantum linear systems of equations, we discuss the solution of quantum linear systems of equations and find it feasible to consider the deferred measurement of the parallel Simon algorithm alone. Finally, since the Grover-meets-Simon algorithm involves an iterative problem, we reconsider the feasibility of the algorithm when placing multiple measurements at the end. According to the maximum probability of success and query times, we get that the Grover-meets-Simon algorithm is not an effective attack algorithm when putting the measurement process of the Simon algorithm in the iterative process at the end of Grover-meets-Simon algorithm.

preprint2023arXiv

LostNet: A smart way for lost and find

Due to the enormous population growth of cities in recent years, objects are frequently lost and unclaimed on public transportation, in restaurants, or any other public areas. While services like Find My iPhone can easily identify lost electronic devices, more valuable objects cannot be tracked in an intelligent manner, making it impossible for administrators to reclaim a large number of lost and found items in a timely manner. We present a method that significantly reduces the complexity of searching by comparing previous images of lost and recovered things provided by the owner with photos taken when registered lost and found items are received. In this research, we will primarily design a photo matching network by combining the fine-tuning method of MobileNetv2 with CBAM Attention and using the Internet framework to develop an online lost and found image identification system. Our implementation gets a testing accuracy of 96.8% using only 665.12M GLFOPs and 3.5M training parameters. It can recognize practice images and can be run on a regular laptop.

preprint2023arXiv

Room-Temperature Highly-Tunable Coercivity and Highly-Efficient Nonvolatile Multi-States Magnetization Switching by Small Current in Single 2D Ferromagnet Fe$_3$GaTe$_2$

Room-temperature electrically-tuned coercivity and nonvolatile multi-states magnetization switching is crucial for next-generation low-power 2D spintronics. However, most methods have limited ability to adjust the coercivity of ferromagnetic systems, and room-temperature electrically-driven magnetization switching shows high critical current density and high power dissipation. Here, highly-tunable coercivity and highly-efficient nonvolatile multi-states magnetization switching are achieved at room temperature in single-material based devices by 2D van der Waals itinerant ferromagnet Fe$_3$GaTe$_2$. The coercivity can be readily tuned up to ~98.06% at 300 K by a tiny in-plane electric field that is 2-5 orders of magnitude smaller than that of other ferromagnetic systems. Moreover, the critical current density and power dissipation for room-temperature magnetization switching in 2D Fe$_3$GaTe$_2$ are down to ~1.7E5 A cm$^{-2}$ and ~4E12 W m$^{-3}$, respectively. Such switching power dissipation is 2-6 orders of magnitude lower than that of other 2D ferromagnetic systems. Meanwhile, multi-states magnetization switching are presented by continuously controlling the current, which can dramatically enhance the information storage capacity and develop new computing methodology. This work opens the avenue for room-temperature electrical control of ferromagnetism and potential applications for vdW-integrated 2D spintronics.

preprint2022arXiv

A Transfer Learning and Optimized CNN Based Intrusion Detection System for Internet of Vehicles

Modern vehicles, including autonomous vehicles and connected vehicles, are increasingly connected to the external world, which enables various functionalities and services. However, the improving connectivity also increases the attack surfaces of the Internet of Vehicles (IoV), causing its vulnerabilities to cyber-threats. Due to the lack of authentication and encryption procedures in vehicular networks, Intrusion Detection Systems (IDSs) are essential approaches to protect modern vehicle systems from network attacks. In this paper, a transfer learning and ensemble learning-based IDS is proposed for IoV systems using convolutional neural networks (CNNs) and hyper-parameter optimization techniques. In the experiments, the proposed IDS has demonstrated over 99.25% detection rates and F1-scores on two well-known public benchmark IoV security datasets: the Car-Hacking dataset and the CICIDS2017 dataset. This shows the effectiveness of the proposed IDS for cyber-attack detection in both intra-vehicle and external vehicular networks.

preprint2022arXiv

AUGER: Automatically Generating Review Comments with Pre-training Models

Code review is one of the best practices as a powerful safeguard for software quality. In practice, senior or highly skilled reviewers inspect source code and provide constructive comments, considering what authors may ignore, for example, some special cases. The collaborative validation between contributors results in code being highly qualified and less chance of bugs. However, since personal knowledge is limited and varies, the efficiency and effectiveness of code review practice are worthy of further improvement. In fact, it still takes a colossal and time-consuming effort to deliver useful review comments. This paper explores a synergy of multiple practical review comments to enhance code review and proposes AUGER (AUtomatically GEnerating Review comments): a review comments generator with pre-training models. We first collect empirical review data from 11 notable Java projects and construct a dataset of 10,882 code changes. By leveraging Text-to-Text Transfer Transformer (T5) models, the framework synthesizes valuable knowledge in the training stage and effectively outperforms baselines by 37.38% in ROUGE-L. 29% of our automatic review comments are considered useful according to prior studies. The inference generates just in 20 seconds and is also open to training further. Moreover, the performance also gets improved when thoroughly analyzed in case study.

preprint2022arXiv

Brain Cortical Functional Gradients Predict Cortical Folding Patterns via Attention Mesh Convolution

Since gyri and sulci, two basic anatomical building blocks of cortical folding patterns, were suggested to bear different functional roles, a precise mapping from brain function to gyro-sulcal patterns can provide profound insights into both biological and artificial neural networks. However, there lacks a generic theory and effective computational model so far, due to the highly nonlinear relation between them, huge inter-individual variabilities and a sophisticated description of brain function regions/networks distribution as mosaics, such that spatial patterning of them has not been considered. we adopted brain functional gradients derived from resting-state fMRI to embed the "gradual" change of functional connectivity patterns, and developed a novel attention mesh convolution model to predict cortical gyro-sulcal segmentation maps on individual brains. The convolution on mesh considers the spatial organization of functional gradients and folding patterns on a cortical sheet and the newly designed channel attention block enhances the interpretability of the contribution of different functional gradients to cortical folding prediction. Experiments show that the prediction performance via our model outperforms other state-of-the-art models. In addition, we found that the dominant functional gradients contribute less to folding prediction. On the activation maps of the last layer, some well-studied cortical landmarks are found on the borders of, rather than within, the highly activated regions. These results and findings suggest that a specifically designed artificial neural network can improve the precision of the mapping between brain functions and cortical folding patterns, and can provide valuable insight of brain anatomy-function relation for neuroscience.

preprint2022arXiv

Cointegration of SARS-CoV-2 Transmission with Weather Conditions and Mobility during the First Year of the COVID-19 Pandemic in the United States

Correlation between weather and the transmission of SARS-CoV-2 may suggest its seasonality. Cointegration analysis can avoid spurious correlation among time series data. We examined the cointegration of virus transmission with daily temperature, dewpoint, and confounding factors of mobility measurements during the first year of the pandemic in the United States. We examined the cointegration of the effective reproductive rate, Rt, of the virus with the dewpoint at two meters, the temperature at two meters, Apple driving mobility, and Google workplace mobility measurements. We found that dewpoint and Apple driving mobility are the best factors to cointegrate with Rt, although temperature and Google workplace mobility also cointegrate with Rt at substantial levels. We found that the optimal lag is two days for cointegration between Rt and weather variables, and three days for Rt and mobility. We observed clusters of states that share similar cointegration results of Rt, weather, and mobility, suggesting regional patterns. Our results support the correlation of weather with the spread of SARS-CoV-2 and its potential seasonality.

preprint2022arXiv

DeepRelease: Language-agnostic Release Notes Generation from Pull Requests of Open-source Software

The release note is an essential software artifact of open-source software that documents crucial information about changes, such as new features and bug fixes. With the help of release notes, both developers and users could have a general understanding of the latest version without browsing the source code. However, it is a daunting and time-consuming job for developers to produce release notes. Although prior studies have provided some automatic approaches, they generate release notes mainly by extracting information from code changes. This will result in language-specific and not being general enough to be applicable. Therefore, helping developers produce release notes effectively remains an unsolved challenge. To address the problem, we first conduct a manual study on the release notes of 900 GitHub projects, which reveals that more than 54% of projects produce their release notes with pull requests. Based on the empirical finding, we propose a deep learning based approach named DeepRelease (Deep learning based Release notes generator) to generate release notes according to pull requests. The process of release notes generation in DeepRelease includes the change entries generation and the change category (i.e., new features or bug fixes) generation, which are formulated as a text summarization task and a multi-class classification problem, respectively. Since DeepRelease fully employs text information from pull requests to summarize changes and identify the change category, it is language-agnostic and can be used for projects in any language. We build a dataset with over 46K release notes and evaluate DeepRelease on the dataset. The experimental results indicate that DeepRelease outperforms four baselines and can generate release notes similar to those manually written ones in a fraction of the time.

preprint2022arXiv

Event-based EV Charging Scheduling in A Microgrid of Buildings

With the popularization of the electric vehicles (EVs), EV charging demand is becoming an important load in the building. Considering the mobility of EVs from building to building and their uncertain charging demand, it is of great practical interest to control the EV charging process in a microgrid of buildings to optimize the total operation cost while ensuring the transmission safety between the microgrid and the main grid. We consider this important problem in this paper and make the following contributions. First, we formulate this problem as a Markov decision process to capture the uncertain supply and EV charging demand in the microgrid of buildings. Besides reducing the total operation cost of buildings, the model also considers the power exchange limitation to ensure transmission safety. Second, this model is reformulated under event-based optimization framework to alleviate the impact of large state and action space. By appropriately defining the event and event-based action, the EV charging process can be optimized by searching a randomized parametric event-based control policy in the microgrid controller and implementing a selecting-to-charging rule in each building controller. Third, a constrained gradient-based policy optimzation method with adjusting mechanism is proposed to iteratively find the optimal event-based control policy for EV charging demand in each building. Numerical experiments considering a microgrid of three buildings are conducted to analyze the structure and the performance of the event-based control policy for EV charging.

preprint2022arXiv

Improving Visual Grounding with Visual-Linguistic Verification and Iterative Reasoning

Visual grounding is a task to locate the target indicated by a natural language expression. Existing methods extend the generic object detection framework to this problem. They base the visual grounding on the features from pre-generated proposals or anchors, and fuse these features with the text embeddings to locate the target mentioned by the text. However, modeling the visual features from these predefined locations may fail to fully exploit the visual context and attribute information in the text query, which limits their performance. In this paper, we propose a transformer-based framework for accurate visual grounding by establishing text-conditioned discriminative features and performing multi-stage cross-modal reasoning. Specifically, we develop a visual-linguistic verification module to focus the visual features on regions relevant to the textual descriptions while suppressing the unrelated areas. A language-guided feature encoder is also devised to aggregate the visual contexts of the target object to improve the object's distinctiveness. To retrieve the target from the encoded visual features, we further propose a multi-stage cross-modal decoder to iteratively speculate on the correlations between the image and text for accurate target localization. Extensive experiments on five widely used datasets validate the efficacy of our proposed components and demonstrate state-of-the-art performance. Our code is public at https://github.com/yangli18/VLTVG.

preprint2022arXiv

LCCDE: A Decision-Based Ensemble Framework for Intrusion Detection in The Internet of Vehicles

Modern vehicles, including autonomous vehicles and connected vehicles, have adopted an increasing variety of functionalities through connections and communications with other vehicles, smart devices, and infrastructures. However, the growing connectivity of the Internet of Vehicles (IoV) also increases the vulnerabilities to network attacks. To protect IoV systems against cyber threats, Intrusion Detection Systems (IDSs) that can identify malicious cyber-attacks have been developed using Machine Learning (ML) approaches. To accurately detect various types of attacks in IoV networks, we propose a novel ensemble IDS framework named Leader Class and Confidence Decision Ensemble (LCCDE). It is constructed by determining the best-performing ML model among three advanced ML algorithms (XGBoost, LightGBM, and CatBoost) for every class or type of attack. The class leader models with their prediction confidence values are then utilized to make accurate decisions regarding the detection of various types of cyber-attacks. Experiments on two public IoV security datasets (Car-Hacking and CICIDS2017 datasets) demonstrate the effectiveness of the proposed LCCDE for intrusion detection on both intra-vehicle and external networks.

preprint2022arXiv

LIGS: Learnable Intrinsic-Reward Generation Selection for Multi-Agent Learning

Efficient exploration is important for reinforcement learners to achieve high rewards. In multi-agent systems, coordinated exploration and behaviour is critical for agents to jointly achieve optimal outcomes. In this paper, we introduce a new general framework for improving coordination and performance of multi-agent reinforcement learners (MARL). Our framework, named Learnable Intrinsic-Reward Generation Selection algorithm (LIGS) introduces an adaptive learner, Generator that observes the agents and learns to construct intrinsic rewards online that coordinate the agents' joint exploration and joint behaviour. Using a novel combination of MARL and switching controls, LIGS determines the best states to learn to add intrinsic rewards which leads to a highly efficient learning process. LIGS can subdivide complex tasks making them easier to solve and enables systems of MARL agents to quickly solve environments with sparse rewards. LIGS can seamlessly adopt existing MARL algorithms and, our theory shows that it ensures convergence to policies that deliver higher system performance. We demonstrate its superior performance in challenging tasks in Foraging and StarCraft II.

preprint2022arXiv

Manipulating Interlayer Excitons for Ultra-pure Near-infrared Quantum Light Generation

Interlayer excitons (IXs) formed at the interface of atomically-thin semiconductors possess various novel properties. In a parallel development, nanoscale strain engineering has emerged as an effective means for creating 2D quantum light sources. Exploring the intersection of these two exciting areas, where strain and defects are exploited for the manipulation of IX toward the emergence of new functionalities, is currently at a nascent stage. Here, using MoS2/WSe2 heterostructure as a model system, we demonstrate how strain, defects, and layering can be utilized to create defect-bound IXs capable of bright, robust, and tunable quantum light emission in the technologically important near-infrared spectral range. We were able to achieve ultra-high single-photon purity with g(2)(0) = 0.01. Our strategy of creating site-controlled QEs from the defect-bound IXs represents a paradigm shift in 2D quantum photonics research, from engineering intralayer exciton in monolayer structures towards IXs at the interface of 2D heterostructures.

preprint2022arXiv

Metal Lines Associated with the Lyman-alpha Forest from eBOSS Data

We investigate the metal species associated with the Ly$α$ forest in the eBOSS quasar spectra. Metal absorption lines are revealed in the stacked spectra from cross-correlating the selected Ly$α$ absorbers in the forest and the flux fluctuation field. Up to 13 metal species are identified associated with relatively strong Ly$α$ absorbers (those with flux fluctuation $-1.0<δ_{\rm Lyα}<-0.6$ and with neutral hydrogen column density of ~ $10^{15-16}$ $\rm cm^{-2}$) over absorber redshift range of $2<z_{\rm abs}<4$. The column densities of these species decrease toward higher redshift and for weaker Ly$α$ absorbers. From modelling the column densities of various species, we find that the column density pattern suggests contributions from multiple gas components both in the circumgalactic medium (CGM) and in the intergalactic medium (IGM). While the low-ionization species (e.g., C II, Si II, and Mg II) can be explained by high-density, cool gas ($T \sim 10^4$ K) from the CGM, the high-ionization species may reside in low-density or high-temperature gas in the IGM. The measurements provide inputs to model metal contamination in the Ly$α$ forest baryon acoustic oscillations measurement. Comparison with metal absorptions in high-resolution quasar spectra and with hydrodynamic galaxy formation simulations can further elucidate the physical conditions of these Ly$α$ absorbers.

preprint2022arXiv

Shifting Trends of COVID-19 Tweet Sentiment with Respect to Voting Preferences in the 2020 Election Year of the United States

COVID-19 related policies were extensively politicized during the 2020 election year of the United States, resulting in polarizing viewpoints. Twitter users were particularly engaged during the 2020 election year. Here we investigated whether COVID-19 related tweets were associated with the overall election results at the state level during the period leading up to the election day. We observed weak correlations between the average sentiment of COVID-19 related tweets and popular votes in two-week intervals, and the trends gradually become opposite. We then compared the average sentiments of COVID-19 related tweets between states called in favor of Republican (red states) or Democratic parties (blue states). We found that at the beginning of lockdowns sentiments in the blue states were much more positive than those in the red states. However, sentiments in the red states gradually become more positive during the summer of 2020 and persisted until the election day.

preprint2022arXiv

TRGP: Trust Region Gradient Projection for Continual Learning

Catastrophic forgetting is one of the major challenges in continual learning. To address this issue, some existing methods put restrictive constraints on the optimization space of the new task for minimizing the interference to old tasks. However, this may lead to unsatisfactory performance for the new task, especially when the new task is strongly correlated with old tasks. To tackle this challenge, we propose Trust Region Gradient Projection (TRGP) for continual learning to facilitate the forward knowledge transfer based on an efficient characterization of task correlation. Particularly, we introduce a notion of `trust region' to select the most related old tasks for the new task in a layer-wise and single-shot manner, using the norm of gradient projection onto the subspace spanned by task inputs. Then, a scaled weight projection is proposed to cleverly reuse the frozen weights of the selected old tasks in the trust region through a layer-wise scaling matrix. By jointly optimizing the scaling matrices and the model, where the model is updated along the directions orthogonal to the subspaces of old tasks, TRGP can effectively prompt knowledge transfer without forgetting. Extensive experiments show that our approach achieves significant improvement over related state-of-the-art methods.

preprint2021arXiv

Big Bird: Transformers for Longer Sequences

Transformers-based models, such as BERT, have been one of the most successful deep learning models for NLP. Unfortunately, one of their core limitations is the quadratic dependency (mainly in terms of memory) on the sequence length due to their full attention mechanism. To remedy this, we propose, BigBird, a sparse attention mechanism that reduces this quadratic dependency to linear. We show that BigBird is a universal approximator of sequence functions and is Turing complete, thereby preserving these properties of the quadratic, full attention model. Along the way, our theoretical analysis reveals some of the benefits of having $O(1)$ global tokens (such as CLS), that attend to the entire sequence as part of the sparse attention mechanism. The proposed sparse attention can handle sequences of length up to 8x of what was previously possible using similar hardware. As a consequence of the capability to handle longer context, BigBird drastically improves performance on various NLP tasks such as question answering and summarization. We also propose novel applications to genomics data.

preprint2021arXiv

Concept Drift Detection in Federated Networked Systems

As next-generation networks materialize, increasing levels of intelligence are required. Federated Learning has been identified as a key enabling technology of intelligent and distributed networks; however, it is prone to concept drift as with any machine learning application. Concept drift directly affects the model's performance and can result in severe consequences considering the critical and emergency services provided by modern networks. To mitigate the adverse effects of drift, this paper proposes a concept drift detection system leveraging the federated learning updates provided at each iteration of the federated training process. Using dimensionality reduction and clustering techniques, a framework that isolates the system's drifted nodes is presented through experiments using an Intelligent Transportation System as a use case. The presented work demonstrates that the proposed framework is able to detect drifted nodes in a variety of non-iid scenarios at different stages of drift and different levels of system exposure.

preprint2021arXiv

Fast Outage Analysis of Large-scale Production Clouds with Service Correlation Mining

Cloud-based services are surging into popularity in recent years. However, outages, i.e., severe incidents that always impact multiple services, can dramatically affect user experience and incur severe economic losses. Locating the root-cause service, i.e., the service that contains the root cause of the outage, is a crucial step to mitigate the impact of the outage. In current industrial practice, this is generally performed in a bootstrap manner and largely depends on human efforts: the service that directly causes the outage is identified first, and the suspected root cause is traced back manually from service to service during diagnosis until the actual root cause is found. Unfortunately, production cloud systems typically contain a large number of interdependent services. Such a manual root cause analysis is often time-consuming and labor-intensive. In this work, we propose COT, the first outage triage approach that considers the global view of service correlations. COT mines the correlations among services from outage diagnosis data. After learning from historical outages, COT can infer the root cause of emerging ones accurately. We implement COT and evaluate it on a real-world dataset containing one year of data collected from Microsoft Azure, one of the representative cloud computing platforms in the world. Our experimental results show that COT can reach a triage accuracy of 82.1%~83.5%, which outperforms the state-of-the-art triage approach by 28.0%~29.7%.

preprint2021arXiv

PWPAE: An Ensemble Framework for Concept Drift Adaptation in IoT Data Streams

As the number of Internet of Things (IoT) devices and systems have surged, IoT data analytics techniques have been developed to detect malicious cyber-attacks and secure IoT systems; however, concept drift issues often occur in IoT data analytics, as IoT data is often dynamic data streams that change over time, causing model degradation and attack detection failure. This is because traditional data analytics models are static models that cannot adapt to data distribution changes. In this paper, we propose a Performance Weighted Probability Averaging Ensemble (PWPAE) framework for drift adaptive IoT anomaly detection through IoT data stream analytics. Experiments on two public datasets show the effectiveness of our proposed PWPAE method compared against state-of-the-art methods.

preprint2021arXiv

Testing for Treatment Effect in Covariate-Adaptive Randomized Clinical Trials with Generalized Linear Models and Omitted Covariates

Concerns have been expressed over the validity of statistical inference under covariate-adaptive randomization despite the extensive use in clinical trials. In the literature, the inferential properties under covariate-adaptive randomization have been mainly studied for continuous responses; in particular, it is well known that the usual two sample t-test for treatment effect is typically conservative, in the sense that the actual test size is smaller than the nominal level. This phenomenon of invalid tests has also been found for generalized linear models without adjusting for the covariates and are sometimes more worrisome due to inflated Type I error. The purpose of this study is to examine the unadjusted test for treatment effect under generalized linear models and covariate-adaptive randomization. For a large class of covariate-adaptive randomization methods, we obtain the asymptotic distribution of the test statistic under the null hypothesis and derive the conditions under which the test is conservative, valid, or anti-conservative. Several commonly used generalized linear models, such as logistic regression and Poisson regression, are discussed in detail. An adjustment method is also proposed to achieve a valid size based on the asymptotic results. Numerical studies confirm the theoretical findings and demonstrate the effectiveness of the proposed adjustment method.

preprint2020arXiv

A Fast Radio Burst discovered in FAST drift scan survey

We report the discovery of a highly dispersed fast radio burst, FRB~181123, from an analysis of $\sim$1500~hr of drift-scan survey data taken using the Five-hundred-meter Aperture Spherical radio Telescope (FAST). The pulse has three distinct emission components, which vary with frequency across our 1.0--1.5~GHz observing band. We measure the peak flux density to be $>0.065$~Jy and the corresponding fluence $>0.2$~Jy~ms. Based on the observed dispersion measure of 1812~cm$^{-3}$~pc, we infer a redshift of $\sim 1.9$. From this, we estimate the peak luminosity and isotropic energy to be $\lesssim 2\times10^{43}$~erg~s$^{-1}$ and $\lesssim 2\times10^{40}$~erg, respectively. With only one FRB from the survey detected so far, our constraints on the event rate are limited. We derive a 95\% confidence lower limit for the event rate of 900 FRBs per day for FRBs with fluences $>0.025$~Jy~ms. We performed follow-up observations of the source with FAST for four hours and have not found a repeated burst. We discuss the implications of this discovery for our understanding of the physical mechanisms of FRBs.

preprint2020arXiv

A Progressive Sub-Network Searching Framework for Dynamic Inference

Many techniques have been developed, such as model compression, to make Deep Neural Networks (DNNs) inference more efficiently. Nevertheless, DNNs still lack excellent run-time dynamic inference capability to enable users trade-off accuracy and computation complexity (i.e., latency on target hardware) after model deployment, based on dynamic requirements and environments. Such research direction recently draws great attention, where one realization is to train the target DNN through a multiple-term objective function, which consists of cross-entropy terms from multiple sub-nets. Our investigation in this work show that the performance of dynamic inference highly relies on the quality of sub-net sampling. With objective to construct a dynamic DNN and search multiple high quality sub-nets with minimal searching cost, we propose a progressive sub-net searching framework, which is embedded with several effective techniques, including trainable noise ranking, channel group and fine-tuning threshold setting, sub-nets re-selection. The proposed framework empowers the target DNN with better dynamic inference capability, which outperforms prior works on both CIFAR-10 and ImageNet dataset via comprehensive experiments on different network structures. Taken ResNet18 as an example, our proposed method achieves much better dynamic inference accuracy compared with prior popular Universally-Slimmable-Network by 4.4%-maximally and 2.3%-averagely in ImageNet dataset with the same model size.

preprint2020arXiv

Artificial Multiferroics and Enhanced Magnetoelectric Effect in van der Waals Heterostructures

Multiferroic materials with coupled ferroelectric and ferromagnetic properties are important for multifunctional devices due to their potential ability of controlling magnetism via electric field, and vice versa. The recent discoveries of two-dimensional ferromagnetic and ferroelectric materials have ignited tremendous research interest and aroused hope to search for two-dimensional multiferroics. However, intrinsic two-dimensional multiferroic materials and, particularly, those with strong magnetoelectric couplings are still rare to date. In this paper, using first-principles simulations, we propose artificial two-dimensional multiferroics via a van der Waals heterostructure formed by ferromagnetic bilayer chromium triiodide (CrI3) and ferroelectric monolayer Sc2CO2. In addition to the coexistence of ferromagnetism and ferroelectricity, our calculations show that, by switching the electric polarization of Sc2CO2, we can tune the interlayer magnetic couplings of bilayer CrI3 between ferromagnetic and antiferromagnetic states. We further reveal that such a strong magnetoelectric effect is from a dramatic change of the band alignment induced by the strong build-in electric polarization in Sc2CO2 and the subsequent change of the interlayer magnetic coupling of bilayer CrI3. These artificial multiferroics and enhanced magnetoelectric effect give rise to realizing multifunctional nanoelectronics by van der Waals heterostructures.

preprint2020arXiv

Exciton Transport under Periodic Potential in MoSe2/WSe2 Heterostructures

The predicted formation of moire superlattices leading to confined excitonic states in heterostructures formed by stacking two lattice mismatched transition metal dichalcogenide (TMD) monolayers was recently experimentally confirmed. Such periodic potential in TMD heterostructure functions as a diffusion barrier that affects the energy transport and dynamics of interlayer excitons (electron and hole spatially concentrated in different monolayers). Understanding the transport of excitons under such condition is essential to establish the material system as a next generation device platform. In this work, we experimentally quantify the diffusion barrier experienced by the interlayer excitons in a hexagonal boron nitride (hBN) encapsulated, molybdenum diselenide tungsten/diselenide (MoSe2/WSe2) heterostructure by studying the exciton transport at various temperatures.

preprint2020arXiv

First-Principles Studies of Second-Order Nonlinear Optical Properties of Organic-Inorganic Hybrid Halide Perovskites

Organic-inorganic hybrid halide perovskites have ignited tremendous interests for photovoltaic applications. However, their nonlinear optical response has not been studied although many of these structures lack the centrosymmetry and exhibit ferroelectricity. In this work, we employ our developed large-scale parallel, first-principles simulation tool (ArchNLO) to explore second-order nonlinear optical properties of a typical family of organic-inorganic hybrid halide perovskites, CH3NH3MX3 (M= Ge, Sn, Pb; X=Cl, Br, I). We find that these hybrid perovskites exhibit second harmonic generation and linear electro-optic effect. The nonlinear optical effects are strongly influenced by the types and positions of cations/anions and corresponding band gaps. Particularly, the distorted cubic phase, which is essentially triclinic, of CH3NH3SnI3 shows significant second harmonic generation and electro-optic effect, which are comparable with those widely used materials, such as GaAs. These second-order optical properties of organic-inorganic hybrid halide perovskites and their low-temperature, solution-based fabrication pave the way for achieving and implementing nonlinear optical devices with low cost.

preprint2020arXiv

Giant linearly-polarized photogalvanic effect and second harmonic generation in two-dimensional axion insulators

The second-order nonlinear optical (NLO) processes, such as the photogalvanic effect and second-order harmonic generation (SHG), play crucial roles in probing and controlling light-matter interactions for energy and device applications. To date, most studies of second-order NLO processes focus on materials with broken spatial inversion symmetry, such as proper ferroelectrics and noncentrosymmetric Weyl semimetals. Nevertheless, inversion symmetry of Shubnikov groups can be broken via spin-ordering in centrosymmetric crystals. Unfortunately, these materials are less common, and their NLO responses are usually weak. Combining quantum perturbation theory and first-principles simulations, we predict a giant injection-current photogalvanic effect and SHG in a family of emerging axion insulators, the even septuple layers of MnBi2Te4 (MBT) materials that exhibit the zero-plateau quantum anomalous Hall (QAH) effect. Their amplitudes of injection current and SHG are about two orders of magnitude larger than those of widely used ferroelectrics, such as BiFeO3 and LiNbO3. Moreover, unlike the usual injection current observed under circularly-polarized light, the injection photocurrent of MBTs only emerges under linearly polarized light, making it convenient for device applications. These unique characters are from a combination effect of parity-time symmetry, three-fold rotation symmetry, and significant spin-orbit coupling. These enhanced NLO effects are valuable for characterizing subtle topological orders in QAH systems and also shed light on novel infrared photo-detector and photovoltaic applications based on magnetic topological materials.

preprint2020arXiv

Intrinsic Spin Photogalvanic Effect in Nonmagnetic Insulator

We show that with the help of spin-orbit coupling, nonlinear light-matter interactions can efficiently couple with spin and valley degrees of freedom. This revealed spin photogalvanic effect can generate the long-time pursued intrinsic pure spin current (PSC) in non-centrosymmetric nonmagnetic insulators. Different from the spin and valley Hall effect, such a photo-driven spin current is universal and can be generated without external bias field. Using first-principles simulation, we study monolayer transition metal dichalcogenides (TMDs) to demonstrate this effect and confirm an enhanced PSC under linearly polarized photoexcitation. The amplitude of the PSC is one order larger than that of the charge current observed in monolayer TMDs. This exotic nonlinear light-spin interaction indicates that light can be utilized as a rapid fashion to manipulate the spin-polarized current, which is crucial for future low-dissipation nanodevices.

preprint2020arXiv

KSM: Fast Multiple Task Adaption via Kernel-wise Soft Mask Learning

Deep Neural Networks (DNN) could forget the knowledge about earlier tasks when learning new tasks, and this is known as \textit{catastrophic forgetting}. While recent continual learning methods are capable of alleviating the catastrophic problem on toy-sized datasets, some issues still remain to be tackled when applying them in real-world problems. Recently, the fast mask-based learning method (e.g. piggyback \cite{mallya2018piggyback}) is proposed to address these issues by learning only a binary element-wise mask in a fast manner, while keeping the backbone model fixed. However, the binary mask has limited modeling capacity for new tasks. A more recent work \cite{hung2019compacting} proposes a compress-grow-based method (CPG) to achieve better accuracy for new tasks by partially training backbone model, but with order-higher training cost, which makes it infeasible to be deployed into popular state-of-the-art edge-/mobile-learning. The primary goal of this work is to simultaneously achieve fast and high-accuracy multi task adaption in continual learning setting. Thus motivated, we propose a new training method called \textit{kernel-wise Soft Mask} (KSM), which learns a kernel-wise hybrid binary and real-value soft mask for each task, while using the same backbone model. Such a soft mask can be viewed as a superposition of a binary mask and a properly scaled real-value tensor, which offers a richer representation capability without low-level kernel support to meet the objective of low hardware overhead. We validate KSM on multiple benchmark datasets against recent state-of-the-art methods (e.g. Piggyback, Packnet, CPG, etc.), which shows good improvement in both accuracy and training cost.

preprint2020arXiv

Nonreciprocal Second-Harmonic Generation in Few-Layer Chromium Triiodide

It is of fundamental importance but challenging to simultaneously identify atomic and magnetic configurations of two-dimensional van der Waals materials. In this work, we show that the nonreciprocal second-harmonic generation (SHG) can be a powerful tool to answer this challenge. Despite the preserved lattice inversion symmetry, the interlayer antiferromagnetic order and spin-orbit coupling generate enhanced SHG in PT-symmetric bilayer chromium triiodide (CrI3). Importantly, the in-plane polarization-resolved SHG is sensitive to subtly different interlayer structures that cannot be told by linear optical spectra. Beyond bilayer, we further predict that the intensity and angle-resolved SHG can be employed to identify both interlayer atomic and magnetic configurations of trilayer CrI3. Our first-principles results agree with available measurements and show the potential of SHG as a non-contacting approach to explore correlations between interlayer structures and magnetic orders of emerging ultra-thin magnetic materials.

preprint2020arXiv

Photo-degradation Protection in 2D In-Plane Heterostructures Revealed by Hyperspectral Nanoimaging: the Role of Nano-Interface 2D Alloys

Single-layer heterostructures exhibit striking quasiparticle properties and many-body interaction effects that hold promise for a range of applications. However, their properties can be altered by intrinsic and extrinsic defects, thus diminishing their applicability. Therefore, it is of paramount importance to identify defects and understand 2D materials' degradation over time using advanced multimodal imaging techniques as well as stabilize degradation via built-in interface protection. Here we implemented a liquid-phase precursor approach to synthesize 2D in-plane MoS2-WS2 heterostructures exhibiting nanoscale alloyed interfaces and map exotic interface effects during photo-degradation using a novel combination of hyperspectral tip-enhanced photoluminescence, Raman and near-field nanoscopy. Surprisingly, 2D alloyed regions exhibit remarkable thermal and photo-degradation stability providing protection against oxidation. Coupled with surface and interface strain, 2D alloy regions create localized potential wells that concentrate excitonic species via a charge carrier funneling effect. These results provide a clear understanding of the importance of 2D alloys as systems able to withstand degradation effects over time, and could be now used to stabilize optoelectronic devices based on 2D materials.

preprint2020arXiv

Quasiparticle Energies and Excitonic Effects of Chromium Trichloride: from Two Dimensions to Bulk

Layered van der Waals (vdW) magnetic materials have attracted significant research interest to date. In this work, we employ the first-principles many-body perturbation theory to calculate excited-state properties of a prototype vdW magnet, chromium trichloride (CrCl3), covering monolayer, bilayer, and bulk structures. Unlike usual non-magnetic vdW semiconductors, in which many-electron interactions and excited states are sensitive to dimensionality, many-electron interactions are always enhanced and dominate quasiparticle energies and optical responses of both two-dimensional and bulk CrCl3. The electron-hole (e-h) binding energy can reach 3 eV in monolayer and remains as high as 2 eV in bulk. Because of the cancellation effect between self-energy corrections and e-h binding energies, the lowest-energy exciton (optical gap) is almost not affected by the change of dimensionality. Besides, for the excitons with similar e-h binding energies, their dipole oscillator strength can differ by a few orders of magnitude.Our analysis shows that such a big difference is from a unique interference effect between complex exciton wavefunctions and interband transitions. Finally, we find that the interlayer stacking sequence and magnetic coupling barely change quasiparticle band gaps and optical absorption spectra of CrCl3. Our calculated low-energy exciton peak positions agree with available measurements. These findings give insight into the understanding of many-electron interactions and the interplay between magnetic orders and optical excitations in vdW magnetic materials.

preprint2020arXiv

Raman Response and Transport Properties of One-Dimensional van der Waals Tellurium Nanowires

Tellurium can form nanowires of helical atomic chains. Given their unique one-dimensional van der Waals structure, these nanowires are expected to show remarkably different physical and electronic properties than bulk tellurium. Here we show that few-chain and single-chain van der Waals tellurium nanowires can be isolated using carbon nanotube and boron nitride nanotube encapsulation. With the approach, the number of atomic chains can be controlled by the inner diameter of the nanotube. The Raman response of the structures suggests that the interaction between a single-atomic tellurium chain and a carbon nanotube is weak, and that the inter-chain interaction becomes stronger as the number of chains increases. Compared with bare tellurium nanowires on SiO2, nanowires encapsulated in boron nitride nanotubes exhibit a dramatically enhanced current-carrying capacity, with a current density of 1.5*10^8 A cm-2, which exceeds that of most semiconducting nanowires. We also use our tellurium nanowires encapsulated in boron nitride nanotubes to create field-effect transistors that have a diameter of only 2 nm.

preprint2020arXiv

Study on $η_{c2}(η_{b2})$ electromagnetic decay into double photons

Within the framework of nonrelativistic QCD (NRQCD) factorization formalism, we compute the helicity amplitude as well as the decay width of $η_{Q2}$ ($Q=c,b$) electromagnetic decay into two photons up to next-to-next-to-leading order (NNLO) in $α_s$ expansion. For the first time, we verify the validity of NRQCD factorization for the D-wave quarkonium decay at NNLO. We find that the $\mathcal{O}(α_s)$ and $\mathcal{O}(α_s^2)$ corrections to the helicity amplitude are negative and moderate, nevertheless both corrections combine to suppress the leading-order prediction for the decay width significantly. By approximating the total decay width of $η_{Q2}$ as the sum of those for the hadronic decay and the electric $E1$ transition, we obtain the branching ratios ${\rm Br}(η_{c2}\to 2γ)\approx 5\times10^{-6}$ and ${\rm Br}(η_{b2}\to 2γ)\approx 4\times10^{-7}$. To explore the potential measurement on $η_{Q2}$, we further evaluate the production cross section of $η_{Q2}$ at LHCb at the lowest order in $α_s$ expansion. With the kinematic constraint on the longitudinal rapidity $4.5>y>2$ and transverse momentum $P_T>(2-4)m_Q$ for $η_{Q2}$, we find the cross section can reach $2-50$ nb for $η_{c2}$, and $1-22$ pb for $η_{b2}$. Considering the integrated luminosity $\mathcal{L}=10\, {\rm fb}^{-1}$ at $\sqrt{s}=7$ TeV and $\sqrt{s}=13$ TeV, we estimate that there are several hundreds events of $pp\to η_{c2}\to 2γ$. Since the background is relatively clean, it is promising to reconstruct $η_{c2}$ through its electromagnetic decay. On the contrary, due to small branching ratio and production cross section, it is quite challenging to detect $η_{b2}\to 2γ$ at LHCb.

preprint2019arXiv

Curie Temperature of Emerging Two-Dimensional Magnetic Structures

Recent realizations of intrinsic, long-range magnetic orders in two-dimensional (2D) van der Waals materials have ignited tremendous research interests. In this work, we employ the XXZ Heisenberg model and Monte Carlo simulations to study a fundamental property of these emerging 2D magnetic materials, the Curie temperature (Tc). By including both onsite and neighbor couplings extracted from first-principles simulations, we have calculated Tc of monolayer chromium trihalides and Cr2Ge2Te6, which are of broad interests currently, and the simulation results agree with available measurements. We also clarify the roles played by anisotropic and isotropic interactions in deciding Tc of magnetic orders. Particularly, we find a universal, linear dependence between Tc and magnetic interactions within the parameter space of realistic materials. With this linear dependence, we can predict Tc of general 2D lattice structures, omitting the Monte Carlo simulations. Compared with the widely used Ising model, mean-field theory, and spin-wave theory, this work provides a convenient and quantitative estimation of Tc, giving hope to speeding up the search for novel 2D materials with higher Curie temperatures.

preprint2019arXiv

Deep Learning-Enhanced Variational Monte Carlo Method for Quantum Many-Body Physics

Artificial neural networks have been successfully incorporated into variational Monte Carlo method (VMC) to study quantum many-body systems. However, there have been few systematic studies of exploring quantum many-body physics using deep neural networks (DNNs), despite of the tremendous success enjoyed by DNNs in many other areas in recent years. One main challenge of implementing DNN in VMC is the inefficiency of optimizing such networks with large number of parameters. We introduce an importance sampling gradient optimization (ISGO) algorithm, which significantly improves the computational speed of training DNN in VMC. We design an efficient convolutional DNN architecture to compute the ground state of a one-dimensional (1D) SU($N$) spin chain. Our numerical results of the ground-state energies with up to 16 layers of DNN show excellent agreement with the Bethe-Ansatz exact solution. Furthermore, we also calculate the loop correlation function using the wave function obtained. Our work demonstrates the feasibility and advantages of applying DNNs to numerical quantum many-body calculations.

preprint2016arXiv

A locally preferred structure characterises all dynamical regimes of a supercooled liquid

Recent experimental results suggest that metallic liquids universally exhibit a high-temperature dynamical crossover, which is correlated with the glass transition temperature ($T_{g}$). We demonstrate, using molecular dynamics results for Cu64Zr36, that this temperature, $T_{A} \approx 2 \times T_{g}$, is linked with cooperative atomic rearrangements that produce domains of connected icosahedra. Supercooling to a new characteristic temperature, $T_{D}$, is shown to produce higher order cooperative rearrangements amongst connected icosahedra, leading to large-scale domain fluctuations and the onset of glassy dynamics. These extensive domains then abruptly stabilize above $T_{g}$ and eventually percolate before the glass is formed. All characteristic temperatures ($T_{A}$, $T_{D}$ and $T_{g}$) are thus connected by successive manifestations of the structural cooperativity that begins at $T_{A}$.

preprint2016arXiv

Bose-Fermi Mapping and Multi-Branch Spin Chain Model for Strongly Interacting Quantum Gases in One-Dimension: Dynamics and Collective Excitations

We show that the wave function of a one dimensional spinor gas with contact $s$-wave interaction, either bosonic or fermionic, can be mapped to the direct product of the wave function of a spinless Fermi gas with short-range $p$-wave interaction and that of a spin system governed by spin parity projection operators. Applying this mapping to strongly interacting spinor gases, we obtain a generalized spin chain model that captures both the static and dynamics properties of the system. Using this spin chain model, we investigate the breathing mode frequency and the quench dynamics of strongly interacting harmonically trapped spinor gases.

preprint2016arXiv

Magnetized quark matter with a magnetic-field dependent coupling

It was recently derived that the QCD running coupling is a function of the magnetic field strength under the strong magnetic field approximation. Inspired by this progress and based on the self-consistent solutions of gap equations, the properties of two-flavor and three-flavor quark matter are studied in the framework of the Nambu-Jona-Lasinio model with a magnetic-field dependent running coupling. We find that the dynamical quark masses as functions of the magnetic field strength are not monotonous in the fully chirally broken phase. Furthermore, the stability of magnetized quark matter with the running coupling is enhanced by lowering the free energy per baryon, which is expected to be more stable than that of the conventional constant coupling case. It is concluded that the magnetized strange quark matter described by running coupling can be absolutely stable.

preprint2016arXiv

Robust Ferroelectricity in Monolayer Group-IV Monochalcogenides

Ferroelectricity usually fades away when materials are thinned down below a critical value. Employing the first-principles density functional theory and modern theory of polarization, we show that the unique ionic-potential anharmonicity can induce spontaneous in-plane electrical polarizations and ferroelectricity in monolayer group-IV monochalcogenides MX (M=Ge, Sn; X=S, Se). Using Monte Carlo simulations with an effective Hamiltonian extracted from the parameterized energy space, we show these materials exhibit a two-dimensional ferroelectric phase transition that is described by fourth-order Landau theory. We also show the ferroelectricity in these materials is robust and the corresponding Curie temperature is higher than room temperature, making these materials promising for realizing ultra-thin ferroelectric devices of broad interest.

preprint2016arXiv

Strain-controlled fundamental gap and structure of bulk black phosphorus

We study theoretically the structural and electronic response of layered bulk black phosphorus to in-layer strain. Ab initio density functional theory (DFT) calculations reveal that the strain energy and interlayer spacing display a strong anisotropy with respect to the uniaxial strain direction. To correctly describe the dependence of the fundamental band gap on strain, we used the computationally more involved GW quasiparticle approach that is free of parameters and superior to DFT studies, which are known to underestimate gap energies. We find that the band gap depends sensitively on the in-layer strain and even vanishes at compressive strain values exceeding about 2%, thus suggesting a possible application of black P in strain-controlled infrared devices.

preprint2015arXiv

A complete Classification of Quantum Public-key Encryption Protocols

We present a classification of quantum public-key encryption protocols. There are six elements in quantum public-key encryption: plaintext, ciphertext, public-key, private-key, encryption algorithm and decryption algorithm. According to the property of each element which is either quantum or classical, the quantum public-key encryption protocols can be divided into 64 kinds. Among 64 kinds of protocols, 8 kinds have already been constructed, 52 kinds can be proved to be impossible to construct and the remaining 4 kinds have not been presented effectively yet. This indicates that the research on quantum public-key encryption protocol should be focus on the existed kinds and the unproposed kinds.

preprint2015arXiv

A quantum algorithm for approximating the influences of Boolean functions and its applications

We investigate the influences of variables on a Boolean function $f$ based on the quantum Bernstein-Vazirani algorithm. A previous paper (Floess et al. in Math. Struct. in Comp. Science 23: 386, 2013) has proved that if a $n$-variable Boolean function $f(x_1,\ldots,x_n)$ does not depend on an input variable $x_i$, using the Bernstein-Vazirani circuit to $f$ will always obtain an output $y$ that has a $0$ in the $i$th position. We generalize this result and show that after one time running the algorithm, the probability of getting a 1 in each position $i$ is equal to the dependence degree of $f$ on the variable $x_i$, i.e. the influence of $x_i$ on $f$. On this foundation, we give an approximation algorithm to evaluate the influence of any variable on a Boolean function. Next, as an application, we use it to study the Boolean functions with juntas, and construct probabilistic quantum algorithms to learn certain Boolean functions. Compared with the deterministic algorithms given by Floess et al., our probabilistic algorithms are faster.

preprint2015arXiv

A quantum algorithm to approximate the linear structures of Boolean functions

We present a quantum algorithm for approximating the linear structures of a Boolean function $f$. Different from previous algorithms (such as Simon's and Shor's algorithms) which rely on restrictions on the Boolean function, our algorithm applies to every Boolean function with no promise. Here, our methods are based on the result of the Bernstein-Vazirani algorithm which is to identify linear Boolean functions and the idea of Simon's period-finding algorithm. More precisely, how the extent of approximation changes over the time is obtained, and meanwhile we also get some quasi linear structures if there exists. Next, we obtain that the running time of the quantum algorithm to thoroughly determine this question is related to the relative differential uniformity $δ_f$ of $f$. Roughly speaking, the smaller the $δ_f$ is, the less time will be needed.

preprint2015arXiv

Bit-oriented quantum public-key encryption

We propose a bit-oriented quantum public-key scheme which uses Boolean function as private-key and randomly changed pairs of quantum state and classical string as public-keys. Contrast to the typical classical public-key scheme, one private-key in our scheme corresponds to an exponential number of public-keys. The goal of our scheme is to achieve information-theoretic security, and the security analysis is also given.

preprint2015arXiv

Full quantum theory of control-not gate in ion-trap quantum computation

We investigate the exact effect on ion trap quantum computation after field quantization. First an exact expression of failure probability from field quantization after many CNOT operations in Cirac-Zoller scheme is given. It is proportional to operation number and the amplitude of $|1\rangle_x |0\rangle_y$ or $|1\rangle_x |1\rangle_y$ in initial state, and inverse proportional to mean number of photons and amplitude of $|0\rangle_x |0\rangle_y$ or $|0\rangle_x |1\rangle_y$ in initial state. Then we calculate the failure probability when the limitation to mean number of photons in sideband transition is considered. When the initial state is $|1\rangle_x |0\rangle_y$ or $|1\rangle_x |1\rangle_y$, after about $10^2$ times of CNOT operations, failure probability is no less than $10^{-2}$, while $10^{-2}$ is the known maximum threshold in fault-tolerant quantum computation. Then when the initial state is $|1\rangle_x |0\rangle_y$ or $|1\rangle_x |1\rangle_y$, the number of CNOT gates on the same pair of physical qubits should be no more than $10^2$ in one error-correction period, or else the computation cannot be implemented reliably. This conclusion can help to determine the number of CNOT operations between coding and decoding in one error-correction period in fault-tolerant quantum computation.

preprint2015arXiv

Giant Piezoelectricity in Monolayer Group IV Monochalcogenides: SnSe, SnS, GeSe and GeS

We predict enormous piezoelectric effects in intrinsic monolayer group IV monochalcogenides (MX, M=Sn or Ge, X=Se or S), including SnSe, SnS, GeSe and GeS. Using first-principle simulations based on the modern theory of polarization, we find that their characteristic piezoelectric coefficients are about two orders of magnitude larger than those of other 2D materials, such as MoS2 and GaSe, and bulk quartz and AlN which are widely used in industry. This enhancement is a result of the unique "puckered" C2v symmetry and weaker chemical bonds of monolayer group IV monochalcogenides. Given the achieved experimental advances in fabrication of monolayers, their flexible character and ability to withstand enormous strain, these 2D structures with giant piezoelectric effects may be promising for a broad range of applications, such as nano-sized sensors, piezotronics, and energy harvesting in portable electronic devices.

preprint2015arXiv

Indistinguishability and semantic security for quantum encryption scheme

We investigate the definition of security for encryption scheme in quantum context. We systematically define the indistinguishability and semantic security for quantum public-key and private-key encryption schemes, and for computational security, physical security and information-theoretic security. Based on our definition, we present a necessary and sufficient condition that leads to information-theoretic indistinguishability for quantum encryption scheme. The equivalence between the indistinguishability and semantic security of quantum encryption scheme is also proved.

preprint2015arXiv

Interfacial Properties of Monolayer and Bilayer MoS2 Contacts with Metals: Beyond the Energy Band Calculations

Although many prototype devices based on two-dimensional (2D) MoS2 have been fabricated and wafer scale growth of 2D MoS2 has been realized, the fundamental nature of 2D MoS2-metal contacts has not been well understood yet. We provide a comprehensive ab initio study of the interfacial properties of a series of monolayer (ML) and bilayer (BL) MoS2-metal contacts (metal = Sc, Ti, Ag, Pt, Ni, and Au). A comparison between the calculated and observed Schottky barrier heights (SBHs) suggests that many-electron effects are strongly suppressed in channel 2D MoS2 due to a charge transfer. The extensively adopted energy band calculation scheme fails to reproduce the observed SBHs in 2D MoS2-Sc interface. By contrast, an ab initio quantum transport device simulation better reproduces the observed SBH in the two types of contacts and highlights the importance of a higher level theoretical approach beyond the energy band calculation in the interface study. BL MoS2-metal contacts have a reduced SBH than ML MoS2-metal contacts due to the interlayer coupling and thus have a higher electron injection efficiency.

preprint2015arXiv

Interlayer Interactions in Anisotropic Atomically-thin Rhenium Diselenide

Recently, two-dimensional (2D) materials with strong in-plane anisotropic properties such as black phosphorus have demonstrated great potential for developing new devices that can take advantage of its reduced lattice symmetry with potential applications in electronics, optoelectronics and thermoelectrics. However, the selection of 2D material with strong in-plane anisotropy has so far been very limited and only sporadic studies have been devoted to transition metal dichalcogenides (TMDC) materials with reduced lattice symmetry, which is yet to convey the full picture of their optical and phonon properties, and the anisotropy in their interlayer interactions. Here, we study the anisotropic interlayer interactions in an important TMDC 2D material with reduced in-plane symmetry - atomically thin rhenium diselenide (ReSe2) - by investigating its ultralow frequency interlayer phonon vibration modes, the layer dependent optical bandgap, and the anisotropic photoluminescence (PL) spectra for the first time. The ultralow frequency interlayer Raman spectra combined with the first study of polarization-resolved high frequency Raman spectra in mono- and bi-layer ReSe2 allows deterministic identification of its layer number and crystal orientation. PL measurements show anisotropic optical emission intensity with bandgap increasing from 1.26 eV in the bulk to 1.32 eV in monolayer, consistent with the theoretical results based on first-principle calculations. The study of the layer-number dependence of the Raman modes and the PL spectra reveals the relatively weak van der Waals interaction and 2D quantum confinement in atomically-thin ReSe2.

preprint2015arXiv

Quantum differential cryptanalysis to the block ciphers

Differential cryptanalysis is one of the most popular methods in attacking block ciphers. However, there still some limitations in traditional differential cryptanalysis. On the other hand, researches of quantum algorithms have made great progress nowadays. This paper proposes two methods to apply quantum algorithms in differential cryptanalysis, and analysis their efficiencies and success probabilities. One method is using quantum algorithm in the high probability differential finding period for every S-Box. The second method is taking the encryption as a whole, using quantum algorithm in this process.

preprint2015arXiv

Quantum fully homomorphic encryption scheme based on quantum fault-tolerant construction

Fully homomorphic encryption is a kind of encryption scheme, which enables arbitrary computation on encrypted data without accessing the data. We present the quantum version of fully homomorphic encryption scheme, which is constructed based on quantum fault-tolerant construction. Two schemes are constructed. The first is a symmetric scheme, and the secret key is the quantum CSS code. In the scheme, when Server performs quantum computation on the encrypted plaintext, some ancillary quantum states should be provided by Client. The second is an asymmetric scheme, which contains the periodical interaction between Client and Server.

preprint2015arXiv

Quantum McEliece public-key encryption scheme

This paper investigates a quantum version of McEliece public-key encryption (PKE) scheme, and analyzes its security. As is well known, the security of classical McEliece PKE is not stronger than the onewayness of related classical one-way function. We prove the security of quantum McEliece PKE ranks between them. Moreover, we propose the double-encryption technique to improve its security, and the security of the improved scheme is proved to be between the original scheme and the quantum one-time pad.

preprint2015arXiv

Quasiparticle Band Gaps, Excitonic Effects, and Anisotropic Optical Properties of Monolayer Distorted 1-T Diamond-chain Structures

We report many-body perturbation theory calculations of excited-state properties of distorted 1-T diamond-chain monolayer rhenium disulfide (ReS2) and diselenide (ReSe2). Electronic self-energy substantially enhances their quasiparticle band gaps and, surprisingly, converts monolayer ReSe2 to a direct-gap semiconductor, which was, however, regarded to be an indirect one by density-functional-theory calculations. Their optical absorption spectra are dictated by strongly bound excitons. Unlike hexagonal structures, the lowest-energy bright exciton of distorted 1-T ReS2 exhibits a perfect figure-8 shape polarization dependence but those of ReSe2 only exhibit a partial polarization dependence, which results from two nearly-degenerated bright excitons whose polarization preferences are not aligned. Our first-principles calculations are in agreement with experiments and pave the way for optoelectronic applications.

preprint2015arXiv

Strain-tunable topological quantum phase transition in buckled honeycomb lattices

Low-buckled silicene is a prototypical quantum spin Hall insulator with the topological quantum phase transition controlled by an out-of-plane electric field. We show that this field-induced electronic transition can be further tuned by an in-plane hydrostatic biaxial strain $\varepsilon$, owing to the curvature-dependent spin-orbit coupling (SOC): There is a $Z_2$ = 1 topological insulator phase for biaxial strain $|\varepsilon|$ smaller than 0.07, and the band gap can be tuned from 0.7 meV for $\varepsilon = +0.07$ up to a fourfold 3.0 meV for $\varepsilon = -0.07$. First-principles calculations also show that the critical field strength $E_c$ can be tuned by more than 113\%, with the absolute values nearly 10 times stronger than the theoretical predictions based on a tight-binding model. The buckling structure of the honeycomb lattice thus enhances the tunability of both the quantum phase transition and the SOC-induced band gap, which are crucial for the design of topological field-effect transistors based on two-dimensional materials.

preprint2015arXiv

Strongly bound excitons dominate electronic relaxation in resonantly excited twisted bilayer graphene

When two sheets of graphene stack in a twisted bilayer graphene (tBLG) configuration, the resulting constrained overlap between interplanar 2p orbitals produce angle-tunable electronic absorption resonances. Using a novel combination of multiphoton transient absorption (TA) microscopy and TEM, we resolve the resonant electronic structure, and ensuing electronic relaxation inside single tBLG domains. Strikingly, we find that the transient electronic population in resonantly excited tBLG domains is enhanced many fold, forming a major electronic relaxation bottleneck. 2-photon TA microscopy shows this bottleneck effect originates from a strongly bound, dark exciton state lying 0.37 eV below the 1-photon absorption resonance. This stable coexistence of strongly bound excitons alongside free-electron continuum states has not been previously observed in a metallic, 2D material.

preprint2015arXiv

Strongly Interacting Quantum Gases in One-Dimensional Traps

Under the second-order degenerate perturbation theory, we show that the physics of $N$ particles with arbitrary spin confined in a one dimensional trap in the strongly interacting regime can be described by super-exchange interaction. An effective spin-chain Hamiltonian (non-translational-invariant Sutherland model) can be constructed from this procedure. For spin-1/2 particles, this model reduces to the non-translational-invariant Heisenberg model, where a transition between Heisenberg anti-ferromagnetic (AFM) and ferromagnetic (FM) states is expected to occur when the interaction strength is tuned from the strongly repulsive to the strongly attractive limit. We show that the FM and the AFM states can be distinguished in two different methods: the first is based on their distinct response to a spin-dependent magnetic gradient, and the second is based on their distinct momentum distribution. We confirm the validity of the spin-chain model by comparison with results obtained from several unbiased techniques

preprint2015arXiv

The Classification of Quantum Symmetric-Key Encryption Protocols

The classification of quantum symmetric-key encryption protocol is presented. According to five elements of a quantum symmetric-key encryption protocol: plaintext, ciphertext, key, encryption algorithm and decryption algorithm, there are 32 different kinds of them. Among them, 5 kinds of protocols have already been constructed and studied, and 21 kinds of them are proved to be impossible to construct, the last 6 kinds of them are not yet presented effectively. That means the research on quantum symmetric-key encryption protocol only needs to consider with 5 kinds of them nowadays.

preprint2015arXiv

Topological Protected Dirac Cones in Compressed Bulk Black Phosphorus

Using the k.p theory and first-principles simulations, we report that applying a moderate pressure (> 0.6 GPa) on black phosphorus can diminish its band gap and produce one-dimensional and even two-dimensional (2D) Dirac cones, distinguishing this material for use in novel non-compound topological insulators. Similar to topological insulators, these 2D Dirac cones result from two competing mechanisms: the unique linear band dispersion tends to open a gap via a "pseudo spin-orbit" coupling, while the band symmetry requirements preserve the material's gapless spectrum. Moreover, these unique Dirac cones are bulk states that do not require time-reversal symmetry, thus they are robust even in the presence of surface or magnetic perturbations. Ultimately, we show that our predictions can be detected by the material's unusual Landau levels.

preprint2014arXiv

Carrier Plasmon Induced Nonlinear Band Gap Renormalization in Two-Dimensional Semiconductors

In reduced-dimensional semiconductors, doping-induced carrier plasmons can strongly couple with quasiparticle excitations, leading to a significant band gap renormalization. We develop a new plasmon-pole theory that efficiently and accurately capture this coupling. Using monolayer molybdenum disulfide (MoS2) as a prototype two-dimensional (2D) semiconductor, we reveal an enhanced band gap renormalization around 400 meV and an unusual nonlinear evolution of its band gap with doping. This 2D prediction significantly differs from the linear behaviors that are common to one-dimensional structures. Our developed approach allows for a quantitative understanding of many-body interactions in general doped 2D semiconductors and paves the way for novel band gap engineering techniques.

preprint2014arXiv

Enhanced Thermoelectric Efficiency via Orthogonal Electrical and Thermal Conductances in Phosphorene

Thermoelectric devices that utilize the Seebeck effect convert heat flow into electrical energy and are highly desirable for the development of portable, solid state, passively-powered electronic systems. The conversion efficiencies of such devices are quantified by the dimensionless thermoelectric figure of merit (ZT), which is proportional to the ratio of a device's electrical conductance to its thermal conductance. High ZT (>2) has been achieved in materials via all-scale hierarchical architecturing. This efficiency holds at high temperatures (700K~900K) but quickly diminishes at lower temperatures. In this paper, a recently-fabricated two-dimensional (2D) semiconductor called phosphorene (monolayer black phosphorus) is assessed for its thermoelectric capabilities. First-principles and model calculations reveal that phosphorene possesses spatially-anisotropic electrical and thermal conductances. The prominent electrical and thermal conducting directions are orthogonal to one another, enhancing the ratio of these conductances. As a result, ZT can reach 2.5 (the criterion for commercial deployment) along the armchair direction of phosphorene at T=500K and is greater than 1 even at room temperature given moderate doping (~2 x 10^16 m-2). Ultimately, phosphorene stands out as an environmentally sound thermoelectric material with unprecedented qualities: intrinsically, it is a mechanically flexible material that converts heat energy with high efficiency at low temperatures (~ 300K) - one whose performance does not require any sophisticated engineering techniques.

preprint2014arXiv

Highly Anisotropic and Robust Excitons in Monolayer Black Phosphorus

Semi-metallic graphene and semiconducting monolayer transition metal dichalcogenides (TMDCs) are the two-dimensional (2D) materials most intensively studied in recent years. Recently, black phosphorus emerged as a promising new 2D material due to its widely tunable and direct bandgap, high carrier mobility and remarkable in-plane anisotropic electrical, optical and phonon properties. However, current progress is primarily limited to its thin-film form, and its unique properties at the truly 2D quantum confinement have yet to be demonstrated. Here, we reveal highly anisotropic and tightly bound excitons in monolayer black phosphorus using polarization-resolved photoluminescence measurements at room temperature. We show that regardless of the excitation laser polarization, the emitted light from the monolayer is linearly polarized along the light effective mass direction and centers around 1.3 eV, a clear signature of emission from highly anisotropic bright excitons. In addition, photoluminescence excitation spectroscopy suggests a quasiparticle bandgap of 2.2 eV, from which we estimate an exciton binding energy of around 0.9 eV, consistent with theoretical results based on first-principles. The experimental observation of highly anisotropic, bright excitons with exceedingly large binding energy not only opens avenues for the future explorations of many-electron effects in this unusual 2D material, but also suggests a promising future in optoelectronic devices such as on-chip infrared light sources.

preprint2014arXiv

Lattice Vibrational Modes and Raman Scattering Spectra of Strained Phosphorene

Strain is prominent in fabricated samples of two-dimensional semiconductors and it also serves as an exploitable tool for engineering their properties. However, quantifying strain and characterizing its spatially inhomogeneous distribution across a material are challenging tasks. Here, we report the lattice vibrational modes and corresponding Raman spectra of strained monolayer black phosphorus (phosphorene) by first-principles simulations. We show that frequencies of vibrational modes of phosphorene and their Raman scattering peaks exhibit substantial and distinct shifts according to the types and size of strain. Therefore, combined with high spatial-resolution Raman scattering measurements, our calculated results can quantify strain distributions in phosphorene. This information is essential for understanding structures of future large-scale fabrication and strain engineering of phosphorene.

preprint2014arXiv

New Mechanism for Strongly Bound Excitons in Gapless Two-Dimensional Structures

Common wisdom asserts that bound excitons cannot form in high-dimensional (d>1) metallic structures because of their overwhelming screening and unavoidable resonance with nearby continuous bands. Strikingly, here we illustrate that this prevalent assumption is not quite true. A key ingredient that has been overlooked is that of viable decoherence that thwarts the formation of resonances. As an example of this general mechanism, we focus on an experimentally relevant material and predict bound excitons in twisted bilayer graphene, which is a two-dimensional gapless structure exhibiting metallic screening. The binding energies calculated by first-principles simulations are surprisingly large. The low-energy effective model reveals that these bound states are produced by a unique destructive coherence between two alike subband resonant excitons. In particular, this destructive coherent effect is not sensitive to the screening and dimensionality, and hence may persist as a general mechanism for creating bound excitons in various metallic structures, opening the door for excitonic applications based on metallic structures.

preprint2014arXiv

Proton cloud and the possibility of direct perceiving of a Hydrogen nucleon

We introduce a concept of proton cloud and calculate the radius of the proton cloud of the Hydrogen atom. Then, we estimate the radius of the proton cloud of a Hydrogen atom on highly excited Rydberg states. Based on the size of proton cloud, the stability of the atom and technical level, we guess that the direct perceiving of the Hydrogen nucleon cloud, or proton cloud, is possible in near future.

preprint2014arXiv

Quantum Oscillations in Black Phosphorus Two-dimensional Electron Gas

Two-dimensional electron gases (2DEG) have been an important source of experimental discovery and conceptual development in condensed matter physics for decades. When combined with the unique electronic properties of two-dimensional (2D) crystals, rich new physical phenomena can be probed at the quantum level. Here, we create a new 2DEG in black phosphorus, a recent member of the two-dimensional atomic crystal family, using a gate electric field. We achieve high carrier mobility in black phosphorus 2DEG by placing it on a hexagonal boron nitride substrate (h-BN). This allows us, for the first time, to observe quantum oscillations in this material. The temperature and magnetic field dependence of the oscillations yields crucial information about the system, such as cyclotron mass and lifetime of its charge carriers. Our results, coupled with the fact that black phosphorus possesses anisotropic energy bands with a tunable, direct bandgap, distinguishes black phosphorus 2DEG as a novel system with unique electronic and optoelectronic properties.

preprint2014arXiv

Strain-Engineering Anisotropic Electrical Conductance of Phosphorene and Few-Layer Black Phosphorus

Newly fabricated monolayer phosphorene and its few-layer structures are expected to be promising for electronic and optical applications because of their finite direct band gaps and sizable but anisotropic electronic mobility. By first-principles simulations, we show that this unique anisotropic conductance can be controlled by using simple strain conditions. With the appropriate biaxial or uniaxial strain, we can rotate the preferred conducting direction by 90 degrees. This will be of useful for exploring quantum Hall effects, and exotic electronic and mechanical applications based on phosphorene.

preprint2014arXiv

Temperature Renormalization of Optical Spectra of Monolayer MoS2

Newly measured optical absorption and photoluminescence spectra reveal substantial frequency shifts of both exciton and trion peaks as monolayer MoS2 is cooled from 363 K to 4 K. First-principles simulations using the GW-Bethe-Salpeter Equation approach satisfactorily reproduce these frequency shifts by incorporating many-electron interactions and the thermal expansion of the in-plane lattice constant. Studying these temperature effects in monolayer MoS2 is crucial for rectifying the results of room-temperature experiments with the previous predictions of zero-temperature-limit simulations. Moreover, we estimate that the thermal expansion coefficient of monolayer MoS2 is around 25% less than that of bulk counterpart by tracking the frequency shifts of the exciton or trion peaks in optical spectra. This may serve as a convenient way to estimate thermal expansion coefficients of general two-dimensional chalcogenides.

preprint2014arXiv

Tunable Band Gap and Anisotropic Optical Response in Few-layer Black Phosphorus

We report the quasiparticle band gap, excitons, and highly anisotropic optical responses of few-layer black phosphorous (phosphorene). It is shown that these new materials exhibit unique many-electron effects; the electronic structures are dispersive essentially along one dimension, leading to particularly enhanced self-energy corrections and excitonic effects. Additionally, within a wide energy range, including infrared light and part of visible light, few-layer black phosphorous absorbs light polarized along the structure's armchair direction and is transparent to light polarized along the zigzag direction, making them viable linear polarizers for applications. Finally, the number of phosphorene layers included in the stack controls the material's band gap, optical absorption spectrum, and anisotropic polarization energy-window across a wide range.

preprint2014arXiv

Unusual Scaling Laws of the Band Gap and Optical Absorption of Phosphorene Nanoribbons

We report the electronic structure and optical absorption spectra of monolayer black phosphorus (phosphorene) nanoribbons (PNRs) via first-principles simulations. The band gap of PNRs is strongly enhanced by quantum confinement. However, differently orientated PNRs exhibit distinct scaling laws for the band gap vs the ribbon width (w). The band gaps of armchair PNRs scale as 1/(w^2), while zigzag PNRs exhibit a 1/w behavior. These distinct scaling laws reflect a significant implication of the band dispersion of phosphorene: electrons and holes behave as classical particles along the zigzag direction, but resemble relativistic particles along the armchair direction. This unexpected merging of classical and relativistic properties in a single material may produce novel electrical and magnetotransport properties of few-layer black phosphorus and its ribbon structures. Finally, the respective PNRs host electrons and holes with markedly different effective masses and optical responses, which are suitable for a wide range of applications.

preprint2014arXiv

Van Hove Singularities and Excitonic Effects in the Optical Conductivity of Twisted Bilayer Graphene

We report a systematic study of the optical conductivity of twisted bilayer graphene (tBLG) across a large energy range (1.2 eV to 5.6 eV) for various twist angles, combined with first-principles calculations. At previously unexplored high energies, our data show signatures of multiple van Hove singularities (vHSs) in the tBLG bands, as well as the nonlinearity of the single layer graphene bands and their electron-hole asymmetry. Our data also suggest that excitonic effects play a vital role in the optical spectra of tBLG. Including electron-hole interactions in first-principles calculations is essential to reproduce the shape of the conductivity spectra, and we find evidence of coherent interactions between the states associated with the multiple vHSs in tBLG.

preprint2013arXiv

Connectivity of the Icosahedral Network and a Dramatically Growing Static Length Scale in Cu-Zr Binary Metallic Glasses

We report on and characterize, via molecular dynamics (MD) studies, the evolution of the structure of Cu50Zr50 and Cu64Zr36 metallic glasses (MGs) as temperature is varied. Interestingly, a percolating icosahedral network appears in the Cu64Zr36 system as it is supercooled. This leads us to introduce a static length scale, which grows dramatically as this three dimensional system approaches the glass transition. Amidst interpenetrating connections, non-interpenetrating connections between icosahedra are shown to become prevalent upon supercooling and to greatly enhance the connectivity of the MG's icosahedral network. Additionally, we characterize the chemical compositions of the icosahedral networks and their components. These findings demonstrate the importance of non-interpenetrating connections for facilitating extensive structural networks in Cu-Zr MGs, which in turn drive dynamical slowing in these materials.

preprint2013arXiv

Dissipation attack on Bennett-Brassard 1984 protocol in practical quantum key distribution system

We propose a new kind of individual attack, based on randomly selected dissipation, on Bennett-Brassard 1984 protocol of practical quantum key distribution (QKD) system with lossy and noisy quantum channel. Since an adversary with super quantum channel can disguise loss and errors induced by his attack as that of the system, he can obtain innegligible amount of information for a practical QKD system, without being detected by legal participants.

preprint2013arXiv

Distributed quantum election scheme

In an electronic voting protocol, a distributed scheme can be used for forbidding the malicious acts of the voting administrator and the counter during the election, but it cannot prevent them from collaborating to trace the ballots and destroy their privacy after the election. We present a distributed anonymous quantum key distribution scheme and further construct a distributed quantum election scheme with a voting administrator made up of more than one part. This quantum election scheme can resist the malicious acts of the voting administrator and the counter after the election and can work in a system with lossy and noisy quantum channels.

preprint2013arXiv

Exciton Energy Spectra in Two-Dimensional Graphene Derivatives

The energy spectra and wavefunctions of bound excitons in important two-dimensional (2D) graphene derivatives, i.e., graphyne and graphane, are found to be strongly modified by quantum confinement, making them qualitatively different from the usual Rydberg series. However, their parity and optical selection rules are preserved. Thus a one-parameter modified hydrogenic model is applied to quantitatively explain the ab initio exciton spectra, and allows one to extrapolate the electron-hole binding energy from optical spectroscopies of 2D semiconductors without costly simulations. Meanwhile, our calculated optical absorption spectrum and enhanced spin singlet-triplet splitting project graphyne, an allotrope of graphene, as a candidate for intriguing energy and biomedical applications.

preprint2013arXiv

Full quantum treatment of Rabi oscillation driven by a pulse train and its application in ion-trap quantum computation

Rabi oscillation of a two-level system driven by a pulse train is a basic process involved in quantum computation. We present a full quantum treatment of this process and show that the population inversion of this process collapses exponentially, has no revival phenomenon, and has a dual-pulse structure in every period. As an application, we investigate the properties of this process in ion-trap quantum computation. We find that in the Cirac--Zoller computation scheme, when the wavelength of the driving field is of the order $10^{-6}$ m, the lower bound of failure probability is of the order $10^{-2}$ after about $10^2$ controlled-NOT gates. This value is approximately equal to the generally-accepted threshold in fault-tolerant quantum computation.

preprint2013arXiv

On the post-quantum security of encrypted key exchange protocols

We investigate the post-quantum security of the encrypted key exchange(EKE) protocols based on some basic physical parameters of ion-trap quantum computer, and show that the EKE protocol with a 40-bit password will be secure against a quantum adversary with several ion-trap quantum computers. We present a password encrypted no-key protocol to resist middle-man attack, and prove that it is also with the post-quantum security. The analysis presented here is probably of general meaning for the security evaluation of various hybrid cryptosystems.

preprint2013arXiv

Quantum no-key protocol for secure communication of classical message

We propose a class of quantum no-key protocols for private communication of classical message based on quantum computing of random Boolean permutations, and demonstrate that they are information-theoretic secure. These protocols are designed to resist middleman attack for two parties preshared authentication key, and achieve perfect mutual data origin authentication which ensures the permanent reusing of authentication key. Finally, we simplify the protocol to a 4-round one, and show that any protocol with 3 or less rounds cannot achieve perfect security without consuming preshared key.

preprint2013arXiv

Quantum probabilistic encryption scheme based on conjugate coding

We present a quantum probabilistic encryption algorithm for a private-key encryption scheme based on conjugate coding of the qubit string. A probabilistic encryption algorithm is generally adopted in public-key encryption protocols. Here we consider the way it increases the unicity distance of both classical and quantum private-key encryption schemes. The security of quantum probabilistic private-key encryption schemes against two kinds of attacks is analyzed. By using the no-signalling postulate, we show that the scheme can resist attack to the key. The scheme's security against plaintext attack is also investigated by considering the information-theoretic indistinguishability of the encryption scheme. Finally, we make a conjecture regarding Breidbart's attack.

preprint2013arXiv

Quantum Public-Key Encryption Schemes Based on Conjugate Coding

We present several quantum public-key encryption (QPKE) protocols designed with conjugate coding single-photon string, thus may be realized in laboratory with nowadays techniques. Two of these schemes are orienting one-bit message, and are extended to two kinds of QPKE schemes orienting multi-bits. The novel structure of these protocols ensures they are information-theoretically secure with, probably, a bound greater than any given polynomial of $n$. Finally, we describe a way to conceal the classical part of the public key with quantum state, this idea is expected to enhance a scheme to be information-theoretically secure.

preprint2013arXiv

Quasiparticle band-edge energy and band offsets of monolayer of molybdenum and tungsten chalcogenide

We report the quasiparticle energy of monolayer of molybdenum and tungsten dichalcogenides, MX2 (M=Mo, W; X=S, Se, Te). Beyond calculating bandgaps, we have achieved converged absolute band energies relative to the vacuum level. Compared with the results from other approaches, the GW calculation reveals substantially larger bandgaps and different absolute band energies because of enhanced many-electron effects. Interestingly, our fully-converged quasiparticle energies ratify the band-gap-center approximation, making it a convenient way to estimate quasiparticle energy. The absolute quasiparticle energies and band offsets obtained in this work are important for designing heterojunction devices and chemical catalysts based on monolayer dichalcogenides.

preprint2013arXiv

Topological kink states at a tilt boundary in gated multi-layer graphene

The search for new realization of topologically protected edge states is an active area of research. We show that a tilt boundary in gated multi-layer graphene supports topologically protected gapless kink states, associated with quantum valley Hall insulator (QVH). We investigate such kink states from two perspectives: the microscopic perspective of a tight-binding model and an ab-initio calculation on bilayer, and the perspective of symmetry protected topological (SPT) states for general multi-layer. We show that a AB-BA bilayer tilt boundary supports gapless kink states that are undeterred by strain concentrated at the boundary. Further, we establish the kink states as concrete examples of edge states of {\it time-reversal symmetric} ${\mathbb Z}$-type SPT, protected by no valley mixing, electron number conservation, and time reversal $T$ symmetries. This allows us to discuss possible phase transitions upon symmetry changes from the SPT perspective. Recent experimental observations of a network of such tilt boundaries suggest that transport through these novel topological kink states might explain the long standing puzzle of sub-gap conductance. Further, recent observation of gap closing and re-opening in gated bi-layer might be the first example of a transition between two distinct SPT's: QVH and LAF.

preprint2012arXiv

Cryptography based on operator theory (I): quantum no-key protocols

We study cryptography based on operator theory, and propose quantum no-key (QNK) protocols from the perspective of operator theory, then present a framework of QNK protocols. The framework is expressed in two forms: trace-preserving quantum operators and natural presentations. Then we defined the information-theoretical security of QNK protocols and the security of identification keys. Two kinds of QNK protocols are also proposed. The first scheme is constructed based on unitary transformation, and the other is constructed based on two multiplicative commutative sets.

preprint2012arXiv

Effect of interaction strength on the evolution of cooperation

Cooperative behaviors are ubiquitous in nature,which is a puzzle to evolutionary biology,because the defector always gains more benefit than the cooperator,thus,the cooperator should decrease and vanish over time.This typical "prisoners' dilemma" phenomenon has been widely researched in recent years.The interaction strength between cooperators and defectors is introduced in this paper(in human society,it can be understood as the tolerance of cooperators).We find that only when the maximum interaction strength is between two critical values,the cooperator and defector can coexist,otherwise, 1) if it is greater than the upper value,the cooperator will vanish, 2) if it is less than the lower value,a bistable state will appear.

preprint2012arXiv

Enhanced Many-Electron Effects on Excited States of Gated Bilayer Graphene

By employing the first-principles GW-Bethe-Salpeter Equation (BSE) simulation, we obtain, for the first time, the accurate quasiparticle (QP) band gap, optical absorption spectra and their dependence on the gate field of gated bilayer graphene (GBLG). Many-electron effects are shown to be extremely important to understand these excited-state properties; enhanced electron-electron interactions dramatically enlarge the QP band gap; infrared optical absorption spectra are dictated by bright bound excitons. Our results well explain recent experiments and satisfyingly solve the puzzle about the inconsistency between experimentally measured transport and optical band gaps. Moreover, our calculation reveals fine excitonic structures and predicts exotic excitonic effects that have not been observed yet, which can be of interest for optoelectronics applications based on GBLG.

preprint2012arXiv

Lattice Vibrational Modes in Si/Ge Core-shell Nanowires

We present a first-principles study on lattice vibrational modes of Si/Ge core-shell nanowires (NWs). In addition to quantum confinement, the internal strain induced by the lattice mismatch between core and shell contributes to significant frequency shifts of characteristic optical modes. More importantly, our simulation shows that these frequency shifts can be detected by Raman scattering experiments, providing convenient and nondestructive ways to obtain structural information of core-shell materials. Meanwhile, another type of collective modes, radial breathing modes (RBMs), are identified in Si-core/Ge-shell NWs and their frequency dependence is explained by an elastic media model.

preprint2012arXiv

On Quantum Turing Machine Halting Deterministically

We define a subclass of quantum Turing machine (QTM) named SR-QTM, which halts deterministically and has deterministic tape head position. A quantum state transition diagram (QSTD) is proposed to describe SR-QTM. With the help of QSTD, we construct a SR-QTM which is universal for all near-trivial transformations. This means there exists a QTM which is universal for the above subclass. Finally we prove that SR-QTM is computational equivalent with ordinary QTM in the bounded error setting. It can be seen that, because SR-QTM has the same time steps for different branches of computation, the halting scheme problem will not exist when considering SR-QTM as a model of quantum computing.

preprint2012arXiv

One-way information reconciliation schemes of quantum key distribution

Information reconciliation(IR) is a basic step of quantum key distribution (QKD). Classical message interaction is necessary in a practical IR scheme, and the communication complexity has become a bottleneck of QKD's development. Here we propose a concatenated method of IR scheme which requires only one time one-way communication to achieve any given error rate level. A QKD scheme with the concatenated IR can work without the special interaction of error rate estimation.

preprint2012arXiv

Quantum election scheme based on anonymous quantum key distribution

An unconditionally secure authority-certified anonymous quantum key distribution scheme using conjugate coding is presented, base on which we construct a quantum election scheme without the help of entanglement state. We show that this election scheme ensures the completeness, soundness, privacy, eligibility, unreusability, fairness and verifiability of a large-scale election in which the administrator and counter are semi-honest. This election scheme can work even if there exist loss and errors in quantum channels. In addition, any irregularity in this scheme is sensible.

preprint2012arXiv

Quantum public-key algorithms to encrypt and authenticate quantum messages with information-theoretic security

Public-key cryptosystems for quantum messages are considered from two aspects: public-key encryption and public-key authentication. Firstly, we propose a general construction of quantum public-key encryption scheme, and then construct an information-theoretic secure instance. Then, we propose a quantum public-key authentication scheme, which can protect the integrity of quantum messages. This scheme can both encrypt and authenticate quantum messages. It is information-theoretic secure with regard to encryption, and the success probability of tampering decreases exponentially with the security parameter with regard to authentication. Compared with classical public-key cryptosystems, one private-key in our schemes corresponds to an exponential number of public-keys, and every quantum public-key used by the sender is an unknown quantum state to the sender.

preprint2012arXiv

Quantum Public-Key Encryption with Information Theoretic Security

We propose a definition for the information theoretic security of a quantum public-key encryption scheme, and present bit-oriented and two-bit-oriented encryption schemes satisfying our security definition via the introduction of a new public-key algorithm structure. We extend the scheme to a multi-bitoriented one, and conjecture that it is also information theoretically secure, depending directly on the structure of our new algorithm.

preprint2012arXiv

Qubit-string-based bit commitment protocols with physical security

Several kinds of qubit-string-based(QS-based) bit commitment protocols are presented, and a definition of information-theoretic concealing is given. All the protocols presented here are proved to be secure under this definition. We suggest an attack algorithm to obtain the local unitary transformation introduced in no-go theorem, which is used to attack the binding condition, then study the security of our QS-based bit commitment protocols under this attack via introducing a new concept "physical security of protocol". At last we present a practical QS-based bit commitment scheme against channel loss and error.

preprint2012arXiv

Tacit knowledge mining algorithm based on linguistic truth-valued concept lattice

This paper is the continuation of our research work about linguistic truth-valued concept lattice. In order to provide a mathematical tool for mining tacit knowledge, we establish a concrete model of 6-ary linguistic truth-valued concept lattice and introduce a mining algorithm through the structure consistency. Specifically, we utilize the attributes to depict knowledge, propose the 6-ary linguistic truth-valued attribute extended context and congener context to characterize tacit knowledge, and research the necessary and sufficient conditions of forming tacit knowledge. We respectively give the algorithms of generating the linguistic truth-valued congener context and constructing the linguistic truth-valued concept lattice.

preprint2011arXiv

Excitonic Effects on Optical Absorption Spectra of Doped Graphene

We have performed first-principles calculations to study optical absorption spectra of doped graphene with many-electron effects included. Both self-energy corrections and electron-hole interactions are reduced due to the enhanced screening in doped graphene. However, self-energy corrections and excitonic effects nearly cancel each other, making the prominent optical absorption peak fixed around 4.5 eV under different doping conditions. On the other hand, an unexpected increase of the optical absorbance is observed within the infrared and visible-light frequency regime (1 ~ 3 eV). Our analysis shows that a combining effect from the band filling and electron-hole interactions results in such an enhanced excitonic effect on the optical absorption. These unique variations of the optical absorption of doped graphene are of importance to understand relevant experiments and design optoelectronic applications.

preprint2011arXiv

First-principles investigation of hydrogen adatoms on uniaxially strained graphene

We have performed first-principles studies on adsorption patterns of hydrogen adatoms on uniaxially strained graphene. Our simulation reveals that the adsorption energy of adatoms are sensitive to the strain. Hydrogen adatoms on zigzag strained graphene tend to form a chain-like adsorption patterns perpendicular to the strain direction, but those under armchair strain cannot form any long-range chain pattern. We explain our results in terms of a tight-binding model and the electronic structure of strained graphene. These anisotropic adsorption behaviors under uniaxial strain suggest methods for obtaining regular adsorption patterns and tailoring the electronic structure of graphene.

preprint2011arXiv

Lattice Vibrational Modes and their Frequency Shifts in Semiconductor Nanowires

We have performed first-principles calculations to study the lattice vibrational modes and their Raman activities in silicon nanowires (SiNWs). Two types of characteristic vibrational modes are examined: high-frequency optical modes and low-frequency confined modes. Their frequencies have opposite size dependence with a red shift for the optical modes and a blue shift for the confined modes as the diameter of SiNWs decreases. In addition, our calculations show that these vibrational modes can be detected by Raman scattering measurements, providing an efficient way to estimate the size of SiNWs.

preprint2011arXiv

Many-Electron Effects on Optical Absorption Spectra of Strained Graphene

We employ the first-principles GW+Bethe Salpeter equation approach to study the electronic structure and optical absorption spectra of uniaxial strained graphene with many-electron effects included. Applied strain not only induces an anisotropic Fermi velocity but also tilts the axis of the Dirac cone. As a result, the optical response of strained graphene is dramatically changed; the optical absorption is anisotropic, strongly depending on the polarization direction of the incident light and the strain orientation; the characteristic single optical absorption peak from π-π* transitions of pristine graphene is split into two peaks and both display enhanced excitonic effects. Within the infrared regime, the optical absorbance of uniaxial strained graphene is no longer a constant because of the broken symmetry and associated anisotropic excitonic effects. Within the visible-light regime, we observe a prominent optical absorption peak due to a significant red shift by electron-hole interactions, enabling us to change the visible color and transparency of stretched graphene. Finally, we also reveal enhanced excitonic effects within the ultraviolet regime (8 to 15 eV), where a few nearly bound excitons are identified.

preprint2011arXiv

Quantum no-key protocols for secret transmission of quantum and classical message

A theoretical framework of quantum no-key (QNK) protocol has been presented. As its applications, we develop three kinds of QNK protocols: the practical QNK protocols, the QNK protocol based on quantum perfect encryption, and the QNK protocols based on Boolean function computing. The security of these protocols is based on the laws of quantum mechanics, other than computational hypothesis.

preprint2011arXiv

Quantum public-key cryptosystems based on induced trapdoor one-way transformations

A concept named induced trapdoor one-way quantum transformation (OWQT) has been introduced, and a theoretical framework of public-key encryption (PKE) of quantum message is presented based on it. Then several kinds of quantum public-key encryption (QPKE) protocols, such as quantum version PKE of RSA, ElGamal, Goldwasser-Micali, elliptic curve, McEliece, Niederreiter and Okamoto-Tanaka-Uchiyama, are given within this framework. Though all of these protocols are only computationally secure, the last three are probably secure in post-quantum era. Besides, theoretical frameworks for public-key authentication and signature of quantum message are also given based on the induced trapdoor OWQT. As examples, a public-key authentication protocol of quantum message based on SN-S authentication scheme and two quantum digital signature protocols based on RSA and McEliece algorithms respectively are presented.

preprint2011arXiv

Universal Quantum Circuit of Near-Trivial Transformations

Any unitary transformation can be decomposed into a product of a group of near-trivial transformations. We investigate in details the construction of universal quantum circuit of near trivial transformations. We first construct two universal quantum circuits which can implement any single-qubit rotation $R_y(θ)$ and $R_z(θ)$ within any given precision, and then we construct universal quantum circuit implementing any single-qubit transformation within any given precision. Finally, a universal quantum circuit implementing any $n$-qubit near-trivial transformation is constructed using the universal quantum circuits of $R_y(θ)$ and $R_z(θ)$. In the universal quantum circuit presented, each quantum transformation is encoded to a bit string which is used as ancillary inputs. The output of the circuit consists of the related bit string and the result of near-trivial transformation. Our result may be useful for the design of universal quantum computer in the future.

preprint2010arXiv

A note on threshold theorem of fault-tolerant quantum computation

Error-correction process has to be carried out periodically to prevent accumulation of errors in fault-tolerant quantum computation. It is believed that the best choice to get maximum threshold value is carrying out an error-correction process after each quantum gate operation. Result of this note shows that the optimal error-correction period depends on the value of k which is the level number of concatenated quantum error-correction code.

preprint2010arXiv

Computationally Efficient Estimation of Factor Multivariate Stochastic Volatility Models

An MCMC simulation method based on a two stage delayed rejection Metropolis-Hastings algorithm is proposed to estimate a factor multivariate stochastic volatility model. The first stage uses kstep iteration towards the mode, with k small, and the second stage uses an adaptive random walk proposal density. The marginal likelihood approach of Chib (1995) is used to choose the number of factors, with the posterior density ordinates approximated by Gaussian copula. Simulation and real data applications suggest that the proposed simulation method is computationally much more efficient than the approach of Chib. Nardari and Shephard (2006}. This increase in computational efficiency is particularly important in calculating marginal likelihoods because it is necessary to carry out the simulation a number of times to estimate the posterior ordinates for a given marginal likelihood. In addition to the MCMC method, the paper also proposes a fast approximate EM method to estimate the factor multivariate stochastic volatility model. The estimates from the approximate EM method are of interest in their own right, but are especially useful as initial inputs to MCMC methods, making them more efficient computationally. The methodology is illustrated using simulated and real examples.

preprint2010arXiv

Optical Absorption Spectra of Electrically Gated Bilayer Graphene

The electronic structure and optical response of electrically gated bilayer graphene are studied by first-principles approaches. We have obtained the induced band gap that is in good agreement with experiment when the applied electric field is less than 1.5 V/nm. The infrared optical absorbance is calculated within the single-particle excitation picture and its fine structures are presented. In addition, the calculated infrared optical absorbance is found to be strongly depending on stacking styles of bilayer graphene and the polarization direction of the incident light, which provides efficient ways to identify the electric-field intensity and stacking styles in experiment. Finally, many-electron effects are discussed.