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Papers in this area

24 featured work(s)

preprint2014arXiv

Characterizing Topological Order with Matrix Product Operators

One of the most striking features of quantum phases that exhibit topological order is the presence of long range entanglement that cannot be detected by any local order parameter. The formalism of projected entangled-pair states is a natural framework for the parameterization of the corresponding ground state wavefunctions, in which the full wavefunction is encoded in terms of local tensors. Topological order is reflected in the symmetries of these tensors, and we give a characterization of those symmetries in terms of matrix product operators acting on the virtual level. This leads to a set of algebraic rules characterizing states with topological quantum order. The corresponding matrix product operators fully encode all topological features of the theory, and provide a systematic way of constructing topological states. We generalize the conditions of $\mathsf{G}$ and twisted injectivity to the matrix product operator case, and provide a complete picture of the ground state manifold on the torus. As an example, we show how all string-net models of Levin and Wen fit within this formalism, and in doing so provide a particularly intuitive interpretation of the pentagon equation for F-symbols as the pulling of certain matrix product operators through the string-net tensor network. Our approach paves the way to finding novel topological phases beyond string-nets, and elucidates the description of topological phases in terms of entanglement Hamiltonians and edge theories.

preprint2014arXiv

Adiabatic and local approximations for the Kohn-Sham potential in time-dependent Hubbard chains

We obtain the exact Kohn-Sham potentials $V_{\mathrm{KS}}$ of time-dependent density-functional theory for 1D Hubbard chains, driven by a d.c.\ external field, using the time-dependent electron density and current density obtained from exact many-body time-evolution. The exact $V_{\mathrm{xc}}$ is compared to the adiabatically-exact $V_{\mathrm{xc}}^{\mathrm{ad}}$ and the "instantaneous ground state" $V_{\mathrm{xc}}^{\mathrm{igs}}$. The latter is shown to work effectively in some cases when the former fails. Approximations for the exchange-correlation potential $V_{\mathrm{xc}}$ and its gradient, based on the local density and on the local current density, are also considered and both physical quantities are observed to be far outside the reach of any possible local approximation. Insight into the respective roles of ground-state and excited-state correlation in the time-dependent system, as reflected in the potentials, is provided by the pair correlation function.

preprint2015arXiv

A multiferroic on the brink: uncovering the nuances of strain-induced transitions in BiFeO$_3$

Bismuth ferrite (BiFeO$_3$) is one of the very few known single-phase multiferroic materials. While the bulk compound is rhombohedral (R), the discovery of an epitaxial strain-induced structural transition into a so-called 'super tetragonal-phase' (T-phase) in this material incited a flurry of research activity focused on gaining an understanding of this phase transition and its possible functionalities. This metastable phase of BiFeO$_3$ is also multiferroic, with giant ferroelectric polarization and coexisting antiferromagnetic order, but above all it is the strain relaxation-induced phase mixtures and their outstanding piezoelectric and magnetoelectric responses which continue to intrigue and motivate the physicist and materials scientist communities. Here, we review the research into the T-phase and mixed-phase BiFeO$_3$ system. We begin with a brief summary of the history of the T-phase and an analysis of the structure of the various phases reported in the literature. We then address important questions regarding the symmetry and octahedral rotation patterns and the (as yet underexplored) important role of chemistry in the formation of the metastable T-phase. We follow by describing the phase transitions in this material, and how these may hold promise for large magnetoelectric responses. Finally we point out some experimental challenges inherent to the study of such a system, and potential pathways for how they may be overcome. It is our intention with this work to highlight important issues that, in our opinion, should be carefully considered by the community in order to use this fascinating materials system for a new paradigm of functionality.

preprint2013arXiv

Exact time-dependent density-functional potentials for strongly correlated tunneling electrons

By propagating the many-body Schrödinger equation, we determine the exact time-dependent Kohn-Sham potential for a system of strongly correlated electrons which undergo field-induced tunneling. Numerous features are entirely absent from the approximations commonly used in time-dependent density-functional theory. The self-interaction correction is strong and time dependent, owing to electron localization, and prominent dynamic spatial potential steps arise from minima in the charge density, as modified by the Coulomb interaction experienced by the partially tunneled electron.

preprint2016arXiv

Hydrodynamics of local excitations after an interaction quench in 1D cold atomic gases

We discuss the hydrodynamic approach to the study of the time evolution -induced by a quench- of local excitations in one dimension. We focus on interaction quenches: the considered protocol consists in creating a stable localized excitation propagating through the system, and then operating a sudden change of the interaction between the particles. To highlight the effect of the quench, we take the initial excitation to be a soliton. The quench splits the excitation into two packets moving in opposite directions, whose characteristics can be expressed in a universal way. Our treatment allows to describe the internal dynamics of these two packets in terms of the different velocities of their components. We confirm our analytical predictions through numerical simulations performed with the Gross-Pitaevskii equation and with the Calogero model (as an example of long range interactions and solvable with a parabolic confinement). Through the Calogero model we also discuss the effect of an external trapping on the protocol. The hydrodynamic approach shows that there is a difference between the bulk velocities of the propagating packets and the velocities of their peaks: it is possible to discriminate the two quantities, as we show through the comparison between numerical simulations and analytical estimates. In the realizations of the discussed quench protocol in a cold atom experiment, these different velocities are accessible through different measurement procedures.

preprint2016arXiv

Origin of static and dynamic steps in exact Kohn-Sham potentials

Knowledge of exact properties of the exchange-correlation (xc) functional is important for improving the approximations made within density functional theory. Features such as steps in the exact xc potential are known to be necessary for yielding accurate densities, yet little is understood regarding their shape, magnitude and location. We use systems of a few electrons, where the exact electron density is known, to demonstrate general properties of steps. We find that steps occur at points in the electron density where there is a change in the `local effective ionization energy' of the electrons. We provide practical arguments, based on the electron density, for determining the position, shape and height of steps for ground-state systems, and extend the concepts to time-dependent systems. These arguments are intended to inform the development of approximate functionals, such as the mixed localization potential (MLP), which already demonstrate their capability to produce steps in the Kohn-Sham potential.

preprint2013arXiv

The macroscopic monopolization in diagonal magnetoelectrics

We develop the formalism of the macroscopic monopolization -- that is the monopole moment per unit volume -- in periodic solids, and discuss its relationship to the diagonal magnetoelectric effect. For the series of lithium transition metal phosphate compounds we use first-principles density functional theory to calculate the contributions to the macroscopic monopolization from the global distribution of magnetic moments within the unit cell, as well as from the distribution of magnetization around the atomic sites. We find one example within the series (LiMnPO$_4$) that shows a macroscopic monopolization corresponding to a ferromonopolar ordering consistent with its diagonal magnetoelectric response. The other members of the series (LiMPO$_4$, with M = Co, Fe and Ni) have zero net monopolization but have antiferromonopolar orderings that should lead to $q$-dependent diagonal magnetoelectric effects

preprint2018arXiv

Coupling between Spin and Charge Order Driven by Magnetic Field in Triangular Ising System LuFe2O4+δ

We present a study of the magnetic-field effect on spin correlations in the charge ordered triangular Ising system LuFe2O4+δ through single crystal neutron diffraction. In the absence of a magnetic field, the strong diffuse neutron scattering observed below the Neel temperature (TN = 240 K) indicates that LuFe2O4+δ shows short-range, two-dimensional (2D) correlations in the FeO5 triangular layers, characterized by the development of a magnetic scattering rod along the 1/3 1/3 L direction, persisting down to 5 K. We also found that on top of the 2D correlations, a long range ferromagnetic component associated with the propagation vector k1 = 0 sets in at around 240 K. On the other hand, an external magnetic field applied along the c-axis effectively favours a three-dimensional (3D) spin correlation between the FeO5 bilayers evidenced by the increase of the intensity of satellite reflections with propagation vector k2 = (1/3, 1/3, 3/2). This magnetic modulation is identical to the charge ordered superstructure, highlighting the field-promoted coupling between the spin and charge degrees of freedom. Formation of the 3D spin correlations suppresses both the rod-type diffuse scattering and the k1 component. Simple symmetry-based arguments provide a natural explanation of the observed phenomenon and put forward a possible charge redistribution in the applied magnetic field.

preprint2018arXiv

Tetrads in solids: from elasticity theory to topological quantum Hall systems and Weyl fermions

Theory of elasticity in topological insulators has many common features with relativistic quantum fields interacting with gravitational field in the tetrad form. Here we discuss several issues in the effective topological (pseudo)electromagnetic response in three-dimensional weak crystalline topological insulators with no time-reversal symmetry that feature elasticity tetrads, including a mixed "axial-gravitational" anomaly. This response has some resemblance to "quasitopological" terms proposed for massless Weyl quasiparticles with separate, emergent fermion tetrads. As an example, we discuss the chiral/axial anomaly in superfluid 3He-A. We demonstrate the principal difference between the elasticity tetrads and the Weyl fermion tetrads in the construction of the topological terms in the action. In particular, the topological action expressed in terms of the elasticity tetrads, cannot be expressed in terms of the Weyl fermion tetrads since in this case the gauge invariance is lost.

preprint2018arXiv

Fermion condensation and super pivotal categories

We study fermionic topological phases using the technique of fermion condensation. We give a prescription for performing fermion condensation in bosonic topological phases which contain a fermion. Our approach to fermion condensation can roughly be understood as coupling the parent bosonic topological phase to a phase of physical fermions, and condensing pairs of physical and emergent fermions. There are two distinct types of objects in fermionic theories, which we call "m-type" and "q-type" particles. The endomorphism algebras of q-type particles are complex Clifford algebras, and they have no analogues in bosonic theories. We construct a fermionic generalization of the tube category, which allows us to compute the quasiparticle excitations in fermionic topological phases. We then prove a series of results relating data in condensed theories to data in their parent theories; for example, if $\mathcal{C}$ is a modular tensor category containing a fermion, then the tube category of the condensed theory satisfies $\textbf{Tube}(\mathcal{C}/ψ) \cong \mathcal{C} \times (\mathcal{C}/ψ)$. We also study how modular transformations, fusion rules, and coherence relations are modified in the fermionic setting, prove a fermionic version of the Verlinde dimension formula, construct a commuting projector lattice Hamiltonian for fermionic theories, and write down a fermionic version of the Turaev-Viro-Barrett-Westbury state sum. A large portion of this work is devoted to three detailed examples of performing fermion condensation to produce fermionic topological phases: we condense fermions in the Ising theory, the $SO(3)_6$ theory, and the $\frac{1}{2}\text{E}_6$ theory, and compute the quasiparticle excitation spectrum in each of these examples.

preprint2017arXiv

Metal-insulator transition in the hybridized two-orbital Hubbard model revisited

In this work we study the two-orbital Hubbard model on a square lattice in the presence of hybridization between nearest-neighbor orbitals and a crystal-field splitting. We use a highly reliable numerical technique based on the density matrix renormalization group to solve the dynamical mean field theory self-consistent impurity problem. We find that the orbital mixing always leads to a finite local density states at the Fermi energy in both orbitals when at least one band is metallic. When one band is doped, and the chemical potential lies between the Hubbard bands in the other band, the coherent quasiparticle peak in this orbital has an exponential behavior with the Hubbard interaction $U$.

preprint2016arXiv

Universality of pseudogap and emergent order in lightly doped Mott insulators

It is widely believed that high-temperature superconductivity in the cuprates emerges from doped Mott insulators. The physics of the parent state seems deceivingly simple: The hopping of the electrons from site to site is prohibited because their on-site Coulomb repulsion U is larger than the kinetic energy gain t. When doping these materials by inserting a small percentage of extra carriers, the electrons become mobile but the strong correlations from the Mott state are thought to survive; inhomogeneous electronic order, a mysterious pseudogap and, eventually, superconductivity appear. How the insertion of dopant atoms drives this evolution is not known, nor whether these phenomena are mere distractions specific to hole-doped cuprates or represent the genuine physics of doped Mott insulators. Here, we visualize the evolution of the electronic states of (Sr1-xLax)2IrO4, which is an effective spin-1/2 Mott insulator like the cuprates, but is chemically radically different. Using spectroscopic-imaging STM, we find that for doping concentration of x=5%, an inhomogeneous, phase separated state emerges, with the nucleation of pseudogap puddles around clusters of dopant atoms. Within these puddles, we observe the same glassy electronic order that is so iconic for the underdoped cuprates. Further, we illuminate the genesis of this state using the unique possibility to localize dopant atoms on topographs in these samples. At low doping, we find evidence for much deeper trapping of carriers compared to the cuprates. This leads to fully gapped spectra with the chemical potential at mid-gap, which abruptly collapse at a threshold of around 4%. Our results clarify the melting of the Mott state, and establish phase separation and electronic order as generic features of doped Mott insulators.

preprint2018arXiv

Evolution of ferromagnetism in two-dimensional electron gas of LaTiO3/SrTiO3

Understanding, creating, and manipulating spin polarization of two-dimensional electron gases at complex oxide interfaces presents an experimental challenge. For example, despite almost a decade long research effort, the microscopic origin of ferromagnetism in LaAlO3/SrTiO3 heterojunction is still an open question. Here, by using a prototypical two-dimensional electron gas (2DEG) which emerges at the interface between band insulator SrTiO3 and antiferromagnetic Mott insulator LaTiO3 , the experiment reveals the evidence for magnetic phase separation in hole-doped Ti d1 t2g system resulting in spin-polarized 2DEG. The details of electronic and magnetic properties of the 2DEG were investigated by temperature-dependent d.c. transport, angle-dependent X-ray photoemission spectroscopy, and temperature-dependent magnetoresistance. The observation of clear hysteresis in magnetotransport at low magnetic fields implies spin-polarization from magnetic islands in the hole rich LaTiO3 near the interface. These findings emphasize the role of magnetic instabilities in doped Mott insulators thus providing another path for designing all-oxide structures relevant to spintronics applications.

preprint2018arXiv

Ultrafast jamming of electrons into an amorphous entangled state

New emergent states of matter in quantum systems may be created under non-equilibrium conditions if - through many body interactions - its constituents order on a timescale which is shorter than the time required for the system to reach thermal equilibrium. Conventionally non-equilibrium ordering is discussed in terms of symmetry breaking, nonthermal order-disorder, and more recently quenched topological transitions. Here we report a fundamentally new and unusual metastable form of amorphous correlation-localized fermionic matter, which is formed in a new type of quantum transition at low temperature either by short pulse photoexcitation or by electrical charge injection in the transition metal dichalcogenide 1T-TaS2. Scanning tunnelling microscopy (STM) reveals a pseudo-amorphous packing of localized electrons within the crystal lattice that is significantly denser than its hexagonally ordered low-temperature ground state, or any other ordered states of the system. Remarkably, the arrangement is not random, but displays a hyperuniform spatial density distribution commonly encountered in classical jammed systems, showing no signs of aggregation or phase separation. Unexpectedly for a localized electron system, tunnelling spectroscopy and multi- STM-tip surface resistance measurements reveal that the overall state is gapless and conducting, which implies that localized and itinerant carriers are resonantly entangled. The amorphous localized electron subsystem can be understood theoretically to arise from strong correlations between polarons sparsely dispersed on a 2D hexagonal atomic lattice, while itinerant carriers act as a resonantly coupled reservoir distinct in momentum space.

preprint2018arXiv

Quantum Annealed Criticality

Experimentally there exist many materials with first-order phase transitions at finite temperature that display quantum criticality. Classically a strain-energy density coupling is known to drive first-order transitions in compressible systems, and here we generalize this Larkin-Pikin mechanism to the quantum case. We show that if the T=0 system lies above its upper critical dimension, the line of first-order transitions can end in a quantum annealed critical point where zero-point fluctuations restore the underlying criticality of the order parameter.

preprint2017arXiv

The Memory Function Formalism: A Review

An introduction to the Zwanzig-Mori-Götze-Wölfle memory function formalism (or generalized Drude formalism) is presented. This formalism is used extensively in analyzing the experimentally obtained optical conductivity of strongly correlated systems like cuprates and Iron based superconductors etc. For a broader perspective both the generalised Langevin equation approach and the projection operator approach for the memory function formalism are given. The Götze-Wölfle perturbative expansion of memory function is presented and its application to the computation of the dynamical conductivity of metals is also reviewd. This review of the formalism contains all the mathematical details for pedagogical purposes.

preprint2017arXiv

How is the derivative discontinuity related to steps in the exact Kohn-Sham potential?

The reliability of density-functional calculations hinges on accurately approximating the unknown exchange-correlation (xc) potential. Common (semi-)local xc approximations lack the jump experienced by the exact xc potential as the number of electrons infinitesimally surpasses an integer, and the spatial steps that form in the potential as a result of the change in the decay rate of the density. These features are important for an accurate prediction of the fundamental gap and the distribution of charge in complex systems. Although well-known concepts, the exact relationship between them remained unclear. In this Letter, we establish the common fundamental origin of these two features of the exact xc potential via an analytical derivation. We support our result with an exact numerical solution of the many-electron Schroedinger equation for a single atom and a diatomic molecule in one dimension. Furthermore, we propose a way to extract the fundamental gap from the step structures in the potential.

preprint2017arXiv

Correlation effects in superconducting quantum dot systems

We study the effect of electron correlations on a system consisting of a single-level quantum dot with local Coulomb interaction attached to two superconducting leads. We use the single-impurity Anderson model with BCS superconducting baths to study the interplay between the proximity induced electron pairing and the local Coulomb interaction. We show how to solve the model using the continuous-time hybridization-expansion quantum Monte Carlo method. The results obtained for experimentally relevant parameters are compared with results of self-consistent second order perturbation theory as well as with the numerical renormalization group method.

preprint2017arXiv

Unusual magnetic structure of high-pressure synthesized perovskites ACrO3(A=Sc, In, Tl)

Magnetic structures of metastable perovskites ScCrO3, InCrO3 and TlCrO3, stabilized under high-pressure and high-temperature conditions, have been studied by neutron powder diffraction. Similar to the other orthochromites LnCrO3 (Ln=lanthanide or Y), these materials crystallize into the orthorhombic structure with Pnma10 symmetry. The spin configuration of the metastable perovskites has been found to be C-type, contrasting with the G-type structure usually observed in LnCrO3. First-principles calculations demonstrate that the Ctype structure found in ScCrO3 and InCrO3 is attributed to a ferromagnetic (FM) nearest-neighbor interaction, while in TlCrO3, this type of magnetic ordering is stabilized by a strong next-nearest-neighbor antiferromagnetic (AFM) exchange. The spins in the C-type magnetic structure line up along the orthorhombic b-axis, yielding the Pnma magnetic symmetry. The dominant mechanism controlling this spin direction has been concluded to be the single ion anisotropy imposed by a uniaxial distortion of CrO6 octahedra.

preprint2016arXiv

Many-body localization and delocalization from the perspective of Integrals of Motion

We study many-body localization (MBL) and delocalization from the perspective of integrals of motion (IOMs). MBL can be understood phenomenologically through the existence of macroscopically many localized IOMs. However, IOMs exist for all many-body systems, and non-localized IOMs determine properties on the ergodic side of the MBL transition too. Here we explore their properties using our method of displacement transformations. We show how different quantities can be calculated using the IOMs as an expansion in the number of operators. For all values of disorder the typical IOMs are localized, suggesting the importance of rare fluctuations in understanding the delocalization transition.

preprint2017arXiv

Supersymmetric SYK models

We discuss a supersymmetric generalization of the Sachdev-Ye-Kitaev model. These are quantum mechanical models involving $N$ Majorana fermions. The supercharge is given by a polynomial expression in terms of the Majorana fermions with random coefficients. The Hamiltonian is the square of the supercharge. The ${\cal N}=1$ model with a single supercharge has unbroken supersymmetry at large $N$, but non-perturbatively spontaneously broken supersymmetry in the exact theory. We analyze the model by looking at the large $N$ equation, and also by performing numerical computations for small values of $N$. We also compute the large $N$ spectrum of "singlet" operators, where we find a structure qualitatively similar to the ordinary SYK model. We also discuss an ${\cal N}=2$ version. In this case, the model preserves supersymmetry in the exact theory and we can compute a suitably weighted Witten index to count the number of ground states, which agrees with the large $N$ computation of the entropy. In both cases, we discuss the supersymmetric generalizations of the Schwarzian action which give the dominant effects at low energies.

preprint2016arXiv

Universality and critical behavior of the dynamical Mott transition in a system with long-range interactions

We study numerically the voltage-induced breakdown of a Mott insulating phase in a system of charged classical particles with long-range interactions. At half-filling on a square lattice this system exhibits Mott localization in the form of a checkerboard pattern. We find universal scaling behavior of the current at the dynamic Mott insulator-metal transition and calculate scaling exponents corresponding to the transition. Our results are in agreement, up to a difference in universality class, with recent experimental evidence of dynamic Mott transition in a system of interacting superconducting vortices.

preprint2019arXiv

Optical conductivity of triple point fermions

As a low-energy effective theory on non-symmorphic lattices, we consider a generic triple point fermion Hamiltonian which is parameterized by an angular parameter $λ$. We find strong $λ$ dependence in both Drude and interband optical absorption of these systems. The deviation of the $T^2$ coefficient of the Drude weight from Dirac/Weyl fermions can be used as a quick way to optically distinguish the triple point degeneracies from the Dirac/Weyl degeneracies. At the particular $λ=π/6$ point, we find that the "helicity" reversal optical transition matrix element is identically zero. But deviating from this point, the helicity reversal emerges as an absorption channel.

preprint2018arXiv

Charge trapping and super-Poissonian noise centers in a cuprate high-temperature superconductor

The electronic properties of cuprate high temperature superconductors in their normal state are very two-dimensional: while transport in the ab plane is perfectly metallic, it is insulating along the c-axis, with ratios between the two exceeding 10^4. This anisotropy has been identified as one of the mysteries of the cuprates early on, and while widely different proposals exist for its microscopic origin, little is known empirically on the microscopic scale. Here, we elucidate the properties of the insulating layers with a newly developed scanning noise spectroscopy technique that can spatially map not only the current but also the current fluctuations in time. We discover atomic-scale noise centers that exhibit MHz current fluctuations 40 times the expectation from Poissonian noise, more than what has been observed in mesoscopic systems. Such behaviour can only happen in highly polarizable insulators and represents strong evidence for trapping of charge in the charge reservoir layers. Our measurements suggest a picture of metallic layers separated by polarizable insulators within a three-dimensional superconducting state.

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