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physics.optics

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Papers in this area

24 featured work(s)

preprint2013arXiv

Broadband and efficient diffraction

Surface topography dictates the deterministic functionality of diffraction by a surface. In order to maximize the efficiency with which a diffractive optical component, such as a grating or a diffractive lens, directs light into a chosen order of diffraction, it is necessary that it be "blazed". The efficiency of most diffractive optical components reported so far varies with the wavelength, and blazing is achieved only at a specific nominal energy, the blaze wavelength. The existence of spurious light in undesirable orders represents a severe limitation that prevents using diffractive components in broadband systems. Here we experimentally demonstrate that broadband blazing over almost one octave can be achieved by combining advanced optical design strategies and artificial dielectric materials that offer dispersion chromatism much stronger than those of conventional bulk materials. The possibility of maintaining an efficient funneling of the energy into a specific order over a broad spectral range may empower advanced research to achieve greater control over the propagation of light, leading to more compact, efficient and versatile optical components.

preprint2015arXiv

High frequency electro-optic measurement of strained silicon racetrack resonators

The observation of the electro-optic effect in strained silicon waveguides has been considered as a direct manifestation of an induced $χ^{(2)}$ non-linearity in the material. In this work, we perform high frequency measurements on strained silicon racetrack resonators. Strain is controlled by a mechanical deformation of the waveguide. It is shown that any optical modulation vanishes independently of the applied strain when the applied voltage varies much faster than the carrier effective lifetime, and that the DC modulation is also largely independent of the applied strain. This demonstrates that plasma carrier dispersion is responsible for the observed electro-optic effect. After normalizing out free carrier effects, our results set an upper limit of $8\,pm/V$ to the induced high-speed $χ^{(2)}_{eff,zzz}$ tensor element at an applied stress of $-0.5\,GPa$. This upper limit is about one order of magnitude lower than the previously reported values for static electro-optic measurements.

preprint2016arXiv

Infrared dielectric properties of low-stress silicon oxide

Silicon oxide thin films play an important role in the realization of optical coatings and high-performance electrical circuits. Estimates of the dielectric function in the far- and mid-infrared regime are derived from the observed transmittance spectrum for a commonly employed low-stress silicon oxide formulation. The experimental, modeling, and numerical methods used to extract the dielectric function are presented.

preprint2016arXiv

Excitation of radiationless anapole mode of isotropic dielectric nanoparticles with tightly focused radially polarized beam

A high index dielectric nano-sphere can be excited and yet remain radiationless. A method to excite the non-radiating anapole mode of a high index isotropic dielectric nanosphere is presented. With tightly focused radially polarized beam illumination, the main-contributing electric dipole mode and magnetic modes can be zero with only a weak electric quadruple contributing to the total scattering. Further, with a standing wave illumination formed by two counter-propagating focused radially polarized beam under $4π$ configuration, the ideal radiationless ananpole can be excited.

preprint2016arXiv

Shaping the focal field of radially/azimuthally polarized phase vortex with Zernike polynomials

The focal field properties of radially/azimuthally polarized Zernike polynomials are studied. A method to design the pupil field in order to shape the focal field of radially or azimuthally polarized phase vortex is introduced. With this method, we are able to obtain a pupil field to achieve a longitudinally polarized hollow spot with a depth of focus up to $12λ$ and $0.14λ$ lateral resolution for a optical system with numerical aperture 0.99; A pupil field to generate 8 circularly polarized focal spots along the optical axis is also obtained with this method.

preprint2016arXiv

Monolayer MoS2/GaAs heterostructure self-driven photodetector with extremely high detectivity

Two dimensional material/semiconductor heterostructures offer alternative platforms for optoelectronic devices other than conventional Schottky and p-n junction devices. Herein, we use MoS2/GaAs heterojunction as a self-driven photodetector with wide response band width from ultraviolet to visible light, which exhibits high sensitivity to the incident light of 635 nm with responsivity as 446 mA/W and detectivity as 5.9*10^13 Jones (Jones = cm Hz1/2 W-1), respectively. Employing interface design by inserting h-BN and photo-induced doping by covering Si quantum dots on the device, the responsivity is increased to 419 mA/W for incident light of 635 nm. Distinctly, attributing to the low dark current of the MoS2/h-BN/GaAs sandwich structure based on the self-driven operation condition, the detectivity shows extremely high value of 1.9*10^14 Jones for incident light of 635 nm, which is higher than all the reported values of the MoS2 based photodetectors. Further investigations reveal that the MoS2/GaAs based photodetectors have response speed with the typical rise/fall time as 17/31 μs. The photodetectors are stable while sealed with polymethyl methacrylate after storage in air for one month. These results imply that monolayer MoS2/GaAs heterojunction may have great potential for practical applications as high performance self-driven photodetectors.

preprint2018arXiv

Mitigation of dynamical instabilities in laser arrays via non-Hermitian coupling

Arrays of coupled semiconductor lasers are systems possessing complex dynamical behavior that are of major interest in photonics and laser science. Dynamical instabilities, arising from supermode competition and slow carrier dynamics, are known to prevent stable phase locking in a wide range of parameter space, requiring special methods to realize stable laser operation. Inspired by recent concepts of parity-time ($\mathcal{PT}$) and non-Hermitian photonics, in this work we consider non-Hermitian coupling engineering in laser arrays in a ring geometry and show, both analytically and numerically, that non-Hermitian coupling can help to mitigate the onset of dynamical laser instabilities. In particular, we consider in details two kinds of nearest-neighbor non-Hermitian couplings: symmetric but complex mode coupling (type-I non-Hermitian coupling) and asymmetric mode coupling (type-II non-Hermitian coupling). Suppression of dynamical instabilities can be realized in both coupling schemes, resulting in stable phase-locking laser emission with the lasers emitting in phase (for type-I coupling) or with $π/2$ phase gradient (for type-II coupling), resulting in a vortex far-field beam. In type-II non-Hermitian coupling, chirality induced by asymmetric mode coupling enables laser phase locking even in presence of moderate disorder in the resonance frequencies of the lasers.

preprint2017arXiv

Observation of forbidden phonons and dark excitons by resonance Raman scattering in few-layer WS$_2$

The optical properties of the two-dimensional (2D) crystals are dominated by tightly bound electron-hole pairs (excitons) and lattice vibration modes (phonons). The exciton-phonon interaction is fundamentally important to understand the optical properties of 2D materials and thus help develop emerging 2D crystal based optoelectronic devices. Here, we presented the excitonic resonant Raman scattering (RRS) spectra of few-layer WS$_2$ excited by 11 lasers lines covered all of A, B and C exciton transition energies at different sample temperatures from 4 to 300 K. As a result, we are not only able to probe the forbidden phonon modes unobserved in ordinary Raman scattering, but also can determine the bright and dark state fine structures of 1s A exciton. In particular, we also observed the quantum interference between low-energy discrete phonon and exciton continuum under resonant excitation. Our works pave a way to understand the exciton-phonon coupling and many-body effects in 2D materials.

preprint2018arXiv

Exceptional points and photonic catastrophe

Exceptional points (EPs) with a global collapse of pairs of eigenfunctions are shown to arise in two locally-coupled and spatially-extended optical structures with balanced gain and loss. Global collapse at the EP deeply changes light propagation, which becomes very sensitive to small changes of initial conditions or system parameters, similarly to what happens in models of classical or quantum catastrophes. The implications of global collapse for light behavior are illustrated by considering discrete beam diffraction and Bloch oscillation catastrophe in coupled waveguide lattices.

preprint2018arXiv

$\mathcal{PT}$ symmetry and anti-symmetry by anti-Hermitian wave coupling and nonlinear optical interactions

Light propagation in systems with anti-Hermitian coupling, described by a spinor-like wave equation, provides a general route for the observation of anti parity-time ($\mathcal{PT}$ ) symmetry in optics. Remarkably, under a different definition of parity operator, a $\mathcal{PT}$ symmetry can be found as well in such systems. Such symmetries are ubiquitous in nonlinear optical interactions and are exemplified by considering modulation instability in optical fibers and optical parametric amplification.

preprint2018arXiv

Dynamics of high-harmonic generation in terms of complex Floquet spectral analysis

High-harmonic generation (HHG) of a two-level-system driven by an intense monochromatic phase-locked laser is studied in terms of complex spectral analysis with the Floquet method. In contrast to the phenomenological approaches, this analysis deals with the whole process as a coherent quantum process based on microscopic dynamics. The spectral decomposition corresponding to the contributions of the Floquet resonance and dressed continuous states of the total system have been obtained. The calculated HHG spectrum exhibits the characteristic features of the HHG from solids. We found that the quantum interference of the Floquet resonance states is responsible for the transition from the adiabatic to the stationary regime in the HHG process and that the phase of the driving laser controls the dynamics of the HHG photon emission.

preprint2018arXiv

Directional scattering from particles under evanescent wave illumination: the role of reactive power

Study of photonic spin-orbital interactions, which involves control of the propagation and spatial distributions of light with the polarization of electromagnetic fields, is not only important at the fundamental level but also has significant implications for functional photonic applications that require active tuning of directional light propagation. Many of the experimental demonstrations have been attributed to the spin-momentum locking characteristic of evanescent waves. In this letter, we show another property of evanescent waves: the polarization dependent direction of the imaginary part of the Poynting vector, i.e. reactive power. Based on this property, we propose a simple and robust way to tune the directional far-field scattering from nanoparticles near a surface under evanescent wave illumination by controlling linear polarization and direction of the incident light.

preprint2017arXiv

Near-Infrared Emitting Single Squaraine Dye Aggregate with large Stokes shift

The study of supramolecular interactions and aggregation behaviour of functional materials is of great importance to tune and extend their spectral sensitivity and, hence, improve the optoelectronic response of related devices. In this study, we resolve spatially and spectrally the absorption and emission features of a squaraine aggregate by means of confocal microscopy and absorption/photoluminescence spectroscopy. We observe that the aggregate affords both a broad absorption spectrum (centred at 670 nm), likely originated by a dyes configuration with allowed J- and H- arrangements, and a strong and relatively narrow emission in the near-infrared (NIR) part of the spectrum (centred at 780 nm), with a remarkable Stokes shift of 110 nm that is among the largest exhibited by squaraine dyes. These peculiarities would be beneficial for extending the spectral sensitivity of bot photovoltaic and light-emitting diodes, and extremely appealing for possible applications of these aggregates as NIR fluorescent probes in biomedical applications.

preprint2019arXiv

Classical versus quantum views of intense laser pulse propagation in gases

We study the behavior of reduced models for the propagation of intense laser pulses in atomic gases. The models we consider incorporate ionization, blueshifting, and other nonlinear propagation effects in an ab initio manner, by explicitly taking into account the microscopic electron dynamics. Numerical simulations of the propagation of ultrashort linearly-polarized and elliptically-polarized laser pulses over experimentally-relevant propagation distances are presented. We compare the behavior of models where the electrons are treated classically with those where they are treated quantum-mechanically. A classical equivalent to the ground state is found, which maximizes the agreement between the quantum and classical predictions of the single-atom ionization probability as a function of laser intensity. We show that this translates into quantitative agreement between the quantum and classical models for the laser field evolution during propagation through gases of ground-state atoms. This agreement is exploited to provide a classical perspective on low- and high-order harmonic generation in linearly-polarized fields. In addition, we demonstrate the stability of the polarization of a nearly-linearly-polarized pulse using a two-dimensional model.

preprint2019arXiv

Non-diffracting broadband incoherent space-time fields

Space-time (ST) wave packets are coherent pulsed beams that propagate diffraction-free and dispersion-free by virtue of tight correlations introduced between their spatial and temporal spectral degrees of freedom. Less is known of the behavior of incoherent ST fields that maintain the spatio-temporal spectral structure of their coherent wave-packet counterparts while losing all purely spatial or temporal coherence. We show here that structuring the spatio-temporal spectrum of an incoherent field produces broadband incoherent ST fields that are diffraction-free. The intensity profile of these fields consists of a narrow spatial feature atop a constant background. Spatio-temporal spectral engineering allows controlling the width of this spatial feature, tuning it from a bright to a dark diffraction-free feature, and varying its amplitude relative to the background. These results pave the way to new opportunities in the experimental investigation of optical coherence of fields jointly structured in space and time by exploiting the techniques usually associated with ultrafast optics.

preprint2019arXiv

Four-wave mixing based orbital angular momentum translation

We theoretically study the generation of orbital angular momentum(OAM) based on four-wave mixing (FWM) process in a diamond-type inhomogeneously broadened $^{85}$Rb atomic system. We use density matrix formalism at weak probe limit to explain the origin of vortex translation between different optical fields and generated signal. We show how the singularities which are omnipresent in phase of the input optical vortex beams can be profoundly mapped to atomic coherence in the transverse plane that hold the origin of OAM translation. This translation process works well even for moderately intense control field which enhances medium nonlinearity. Further we have manoeuvred an additional rotation of the phase wavefront in both clockwise and anti-clockwise direction controlled by the single photon detuning. The generation and manipulation of OAM of light beam in nonlinear medium may have important applications in optical tweezers and quantum information processing systems.

preprint2019arXiv

Optical Control of Chiral Charge Pumping in a Topological Weyl Semimetal

Solids with topologically robust electronic states exhibit unusual electronic and optical transport properties that do not exist in other materials. A particularly interesting example is chiral charge pumping, the so-called chiral anomaly, in recently discovered topological Weyl semimetals, where simultaneous application of parallel DC electric and magnetic fields creates an imbalance in the number of carriers of opposite topological charge (chirality). Here, using time-resolved terahertz measurements on the Weyl semimetal TaAs in a magnetic field, we optically interrogate the chiral anomaly by dynamically pumping the chiral charges and monitoring their subsequent relaxation. Theory based on Boltzmann transport shows that the observed effects originate from an optical nonlinearity in the chiral charge pumping process. Our measurements reveal that the chiral population relaxation time is much greater than 1 ns. The observation of terahertz-controlled chiral carriers with long coherence times and topological protection suggests the application of Weyl semimetals for quantum optoelectronic technology.

preprint2018arXiv

Four wave mixing based generation and control of light pulse

We present an efficient scheme for the generation and control of a degenerate four-wave mixing (FWM) signal in a N-type inhomogeneously broadened 85Rb atomic system. We observe the propagation dynamics of the generated FWM signal along with the probe pulse under the condition of Electromagnetically Induced Transparency. The FWM signal clones the temporal shape of the probe pulse and travels through the medium without changing its shape and intensity. We have also shown that a time dependent control field permits the storage and retrieval of these optical signals without losing their identity. This work allows us to generate, control, store and retrieve FWM signal of any arbirary shape.

preprint2019arXiv

What is the maximum differential group delay achievable by a space-time wave packet in free space?

The group velocity of 'space-time' wave packets $-$ propagation-invariant pulsed beams endowed with tight spatio-temporal spectral correlations $-$ can take on arbitrary values in free space. Here we investigate theoretically and experimentally the maximum achievable group delay that realistic finite-energy space-time wave packets can achieve with respect to a reference pulse traveling at the speed of light. We find that this delay is determined solely by the spectral uncertainty in the association between the spatial frequencies and wavelengths underlying the wave packet spatio-temporal spectrum $-$ and not by the beam size, bandwidth, or pulse width. We show experimentally that the propagation of space-time wave packets is delimited by a spectral-uncertainty-induced `pilot envelope' that travels at a group velocity equal to the speed of light in vacuum. Temporal walk-off between the space-time wave packet and the pilot envelope limits the maximum achievable differential group delay to the width of the pilot envelope. Within this pilot envelope, the space-time wave packet can locally travel at an arbitrary group velocity and yet not violate relativistic causality because the leading or trailing edge of superluminal and subluminal space-time wave packets, respectively, are suppressed once they reach the envelope edge. Using pulses of width $\sim$4ps and a spectral uncertainty of $\sim$ 20 pm, we measure maximum differential group delays of approximately $\pm$ 150 ps, which exceed previously reported measurements by at least three orders of magnitude.

preprint2019arXiv

Classification of propagation-invariant space-time wave packets in free space: Theory and experiments

Introducing correlations between the spatial and temporal degrees of freedom of a pulsed optical beam (or wave packet) can profoundly alter its propagation in free space. Indeed, appropriate spatio-temporal spectral correlations can render the wave packet propagation-invariant: the spatial and temporal profiles remain unchanged along the propagation axis. The spatio-temporal spectral locus of any such wave packet lies at the intersection of the light-cone with tilted spectral hyperplanes. We investigate (2+1)D 'space-time' propagation-invariant light sheets, and identify 10 classes categorized according to the magnitude and sign of their group velocity and the nature of their spatial spectrum - whether the low spatial frequencies are physically allowed or forbidden according to their compatibility with causal excitation and propagation. We experimentally synthesize and characterize all 10 classes using an experimental strategy capable of synthesizing space-time wave packets that incorporate arbitrary spatio-temporal spectral correlations.

preprint2019arXiv

Hybrid 1D Plasmonic/Photonic Crystals are Responsive to Escherichia Coli

Photonic crystal-based biosensors hold great promise as valid and low-cost devices for real-time monitoring of a variety of biotargets. Given the high processability and easiness of read-out even for unskilled operators, these systems can be highly appealing for the detection of bacterial contaminants in food and water. Here, we propose a novel hybrid plasmonic/photonic device that is responsive to Escherichia coli, which is one of the most hazardous pathogenic bacterium. Our system consists of a thin layer of silver, a metal that exhibits both a plasmonic behavior and a well-known biocidal activity, on top of a solution processed 1D photonic crystal. We attribute the bio-responsivity to the modification of the dielectric properties of the silver film upon bacterial contamination, an effect that likely stems from the formation of polarization charges at the Ag/bacterium interface within a sort of bio-doping mechanism. Interestingly, this triggers a blue-shift in the photonic response. This work demonstrates that our hybrid plasmonic/photonic device can be a low-cost and portable platform for the detection of common contaminants in food and water.

preprint2019arXiv

Generation of very high-order high purity Gaussian modes via spatial light modulation

We experimentally demonstrate the conversion of a fundamental $\text{TEM}_{00}$ laser mode at 1064\,nm to higher order Hermite-Gaussian modes (HG) of arbitrary order via a commercially available liquid crystal Spatial Light Modulator (SLM). We particularly studied the $\text{HG}_{5,5}/\text{HG}_{10,10}/\text{HG}_{15,15}$ modes. A two-mirror plano-spherical cavity filters the higher-order modes spatially. We analyze the cleaned modes via a three-mirror diagnosis cavity and measure a mode purity of 96/93/78\% and a conversion efficiency of 6.6\%/3.7\%/1.7\% respectively. The generated high-purity Hermite-Gaussian modes can be employed for the mitigation of mirror thermal noise in optical cavities for both optical clocks and gravitational wave (GW) detectors. HG modes are then converted into high order LG modes which can be of particular interest in cold atom physics.

preprint2018arXiv

Photonic Flatband Laser

Flatband photonic lattices, i.e. arrays of waveguides or resonators displaying a flat Bloch band, offer new routes for light trapping and distortion-free imaging. Here it is shown that flatland lattices can show stable and cooperative laser emission when optical gain is supplied to the system, despite the large degree of degeneracy of flatland supermodes. By considering a quasi one-dimensional rhombic lattice of coupled semiconductor microrings, selective pumping of the outer sublattices can induce cooperative lasing in a supermode of the flat band

preprint2019arXiv

Efficient wide-field FLIM

Nanosecond temporal resolution enables new methods for wide-field imaging like time-of-flight, gated detection, and fluorescence lifetime. The optical efficiency of existing approaches, however, presents challenges for low-light applications common to fluorescence microscopy and single-molecule imaging. We demonstrate the use of Pockels cells for wide-field image gating with nanosecond temporal resolution and high photon collection efficiency. Two temporal frames are obtained by combining a Pockels cell with a pair of polarizing beam-splitters. We show multi-label fluorescence lifetime imaging microscopy (FLIM), single-molecule lifetime spectroscopy, and fast single-frame FLIM at the camera frame rate with $10^3 - 10^5$ times higher throughput than single photon counting. Finally, we demonstrate a space-to-time image multiplexer using a re-imaging optical cavity with a tilted mirror to extend the Pockels cell technique to multiple temporal frames. These methods enable nanosecond imaging with standard optical systems and sensors, opening a new temporal dimension for low-light microscopy.

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