μμSR and Neutron Diffraction Investigations on Reentrant Ferromagnetic Superconductor Eu(Fe{0.86}Ir{0.14})2As2

preprint2015arXivOpen access

Abstract

Results of muon spin relaxation (μμSR) and neutron powder diffraction measurements on a reentrant superconductor Eu(Fe0.86_{0.86}Ir0.14_{0.14})2_2As2_2 are presented. Eu(Fe0.86_{0.86}Ir0.14_{0.14})2_2As2_2 exhibits superconductivity at Tc on≈22.5T_{\rm c\,on} \approx 22.5~K competing with long range ordered Eu+2^{+2} moments below ≈18\approx 18 K. A reentrant behavior (manifested by nonzero resistivity in the temperature range 10--17.5 K) results from an exquisite competition between the superconductivity and magnetic order. The zero field μμSR data confirm the long range magnetic ordering below TEu=18.7(2)T_{\rm Eu} = 18.7(2) K. The transition temperature is found to increase with increasing magnetic field in longitudinal field μμSR which along with the neutron diffraction results, suggests the transition to be ferromagnetic. The neutron diffraction data reveal a clear presence of magnetic Bragg peaks below TEuT_{\rm Eu} which could be indexed with propagation vector k = (0, 0, 0), confirming a long range magnetic ordering in agreement with μμSR data. Our analysis of the magnetic structure reveals an ordered magnetic moment of 6.29(5) μB6.29(5)\,μ_{\rm B} (at 1.8 K) on the Eu atoms and they form a ferromagnetic structure with moments aligned along the cc-axis. No change in the magnetic structure is observed in the reentrant or superconducting phases and the magnetic structure remains same for 1.8 K ≤T≤TEu\leq T \leq T_{\rm Eu}. No clear evidence of structural transition or Fe moment ordering was found.

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