Spin liquid close to a quantum critical point in Na4_4Ir3_3O8_8

preprint2013arXivOpen access

Abstract

Na4_4Ir3_3O8_8 is a candidate material for a 3-dimensional quantum spin-liquid on the hyperkagome lattice. We present thermodynamic measurements of heat capacity CC and thermal conductivity κκ on high quality polycrystalline samples of Na4_4Ir3_3O8_8 down to T=500T = 500 mK and 7575 mK, respectively. Absence of long-range magnetic order down to T=75T = 75 mK strongly supports claims of a spin-liquid ground state. The constant magnetic susceptibility χχ below T≈25T \approx 25 K and the presence of a small but finite linear-TT term in C(T)C(T) suggest the presence of gapless spin excitations. Additionally, the magnetic Gru¨\ddot{\rm{u}}neisen ratio shows a divergence as T→0T \rightarrow 0 K and a scaling behavior which clearly demonstrates that Na4_4Ir3_3O8_8 is situated close to a zero-field QCP.

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