Abstract

Elastic neutron scattering, ac susceptibility, and specific heat experiments on the pyrochlores Er2_{2}Ge2_{2}O7_{7} and Yb2_{2}Ge2_{2}O7_{7} show that both systems are antiferromagnetically ordered in the Γ5Γ_5 manifold. The ground state is a ψ3ψ_{3} phase for the Er sample and a ψ2ψ_{2} or ψ3ψ_{3} phase for the Yb sample, which suggests "Order by Disorder"(ObD) physics. Furthermore, we unify the various magnetic ground states of all known R2_{2}B2_{2}O7_{7} (R = Er, Yb, B = Sn, Ti, Ge) compounds through the enlarged XY type exchange interaction J±J_{\pm} under chemical pressure. The mechanism for this evolution is discussed in terms of the phase diagram proposed in the theoretical study [Wong et al., Phys. Rev. B 88, 144402, (2013)].

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