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Enhanced third harmonic generation from the epsilon-near-zero modes of ultrathin films

We experimentally demonstrate efficient third harmonic generation from an indium tin oxide (ITO) nanofilm (lambda/42 thick) on a glass substrate for a pump wavelength of 1.4 um. A conversion efficiency of 3.3x10^-6 is achieved by exploiting the field enhancement properties of the epsilon-near-zero (ENZ) mode with an enhancement factor of 200. This nanoscale frequency conversion method is applicable to other plasmonic materials and reststrahlen materials in proximity of the longitudinal optical phonon frequencies.

preprint2015arXivOpen access
Ting S. LukDomenico de CegliaSheng LiuGordon A. KeelerRohit P. PrasankumarMaria A. VincentiMichael ScaloraMichael B. SinclairSalvatore Campione
cond-mat.mes-hallphysics.optics
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Open access9 authors2 topics
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Ting S. LukDomenico de CegliaSheng LiuGordon A. KeelerRohit P. PrasankumarMaria A. VincentiMichael ScaloraMichael B. SinclairSalvatore Campione

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