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Published work

58 published item(s)

preprint2026arXiv

Conformal Path Reasoning: Trustworthy Knowledge Graph Question Answering via Path-Level Calibration

Knowledge Graph Question Answering (KGQA) has shown promise for grounded and interpretable reasoning, yet existing approaches often fail to provide reliable coverage guarantees over retrieved answers. While Conformal Prediction (CP) offers a principled framework for producing prediction sets with statistical guarantees, prior methods suffer from critical limitations in both calibration validity and score discriminability, resulting in violated coverage guarantees and excessively large prediction sets. To address these pitfalls, we propose Conformal Path Reasoning (CPR), a trustworthy KGQA framework with two key innovations. First, we perform query-level conformal calibration over path-level scores, preserving the exchangeability while generating path prediction sets. Second, we introduce the Residual Conformal Value Network (RCVNet), a lightweight module trained via PUCT-guided exploration to learn discriminative path-level nonconformity scores. Experiments on benchmarks show that CPR significantly improves the Empirical Coverage Rate by 34% while reducing average prediction set size by 40% compared to conformal baselines. These results validate the efficacy of CPR in satisfying coverage guarantees with substantially more compact answer sets.

preprint2024arXiv

RHOBIN Challenge: Reconstruction of Human Object Interaction

Modeling the interaction between humans and objects has been an emerging research direction in recent years. Capturing human-object interaction is however a very challenging task due to heavy occlusion and complex dynamics, which requires understanding not only 3D human pose, and object pose but also the interaction between them. Reconstruction of 3D humans and objects has been two separate research fields in computer vision for a long time. We hence proposed the first RHOBIN challenge: reconstruction of human-object interactions in conjunction with the RHOBIN workshop. It was aimed at bringing the research communities of human and object reconstruction as well as interaction modeling together to discuss techniques and exchange ideas. Our challenge consists of three tracks of 3D reconstruction from monocular RGB images with a focus on dealing with challenging interaction scenarios. Our challenge attracted more than 100 participants with more than 300 submissions, indicating the broad interest in the research communities. This paper describes the settings of our challenge and discusses the winning methods of each track in more detail. We observe that the human reconstruction task is becoming mature even under heavy occlusion settings while object pose estimation and joint reconstruction remain challenging tasks. With the growing interest in interaction modeling, we hope this report can provide useful insights and foster future research in this direction. Our workshop website can be found at \href{https://rhobin-challenge.github.io/}{https://rhobin-challenge.github.io/}.

preprint2023arXiv

Recent advances of transition radiation: fundamentals and applications

Transition radiation is a fundamental process of light emission and occurs whenever a charged particle moves across an inhomogeneous region. One feature of transition radiation is that it can create light emission at arbitrary frequency under any particle velocity. Therefore, transition radiation is of significant importance to both fundamental science and practical applications. In this paper, we provide a brief historical review of transition radiation and its recent development. Moreover, we pay special attention to four typical applications of transition radiation, namely the detection of high-energy particles, coherent radiation sources, beam diagnosis, and excitation of surface waves. Finally, we give an outlook for the research tendency of transition radiation, especially its flexible manipulation by exploiting artificially-engineered materials and nanostructures, such as gain materials, metamaterials, spatial-temporal materials, meta-boundaries, and layered structures with a periodic or non-periodic stacking.

preprint2022arXiv

Credible Persuasion

We propose a new notion of credibility for Bayesian persuasion problems. A disclosure policy is credible if the sender cannot profit from tampering with her messages while keeping the message distribution unchanged. We show that the credibility of a disclosure policy is equivalent to a cyclical monotonicity condition on its induced distribution over states and actions. We also characterize how credibility restricts the Sender's ability to persuade under different payoff structures. In particular, when the sender's payoff is state-independent, all disclosure policies are credible. We apply our results to the market for lemons, and show that no useful information can be credibly disclosed by the seller, even though a seller who can commit to her disclosure policy would perfectly reveal her private information to maximize profit.

preprint2022arXiv

Giant modulation of the electron mobility in semiconductor Bi$_2$O$_2$Se via incipient ferroelectric phase transition

High-mobility layered semiconductors have the potential to enable the next-generation electronics and computing. This paper demonstrates that the ultrahigh electron mobility observed in the layered semiconductor Bi$_2$O$_2$Se originates from an incipient ferroelectric transition that endows the material with a robust protection against mobility degradation by Coulomb scattering. Based on first-principles calculations of electron-phonon interaction and ionized impurity scattering, it is shown that the electron mobility of Bi$_2$O$_2$Se can reach 10$^4$ to 10$^6$ cm$^2$V$^{-1}$s$^{-1}$ over a wide range of realistic doping concentrations. Furthermore, a small elastic strain of 1.7% can drive the material toward a unique interlayer ferroelectric transition, resulting in a large increase in the dielectric permittivity and a giant enhancement of the low-temperature electron mobility by more than an order of magnitude. These results establish a new route to realize high-mobility layered semiconductors via phase and dielectric engineering.

preprint2022arXiv

Online Changepoint Detection on a Budget

Changepoints are abrupt variations in the underlying distribution of data. Detecting changes in a data stream is an important problem with many applications. In this paper, we are interested in changepoint detection algorithms which operate in an online setting in the sense that both its storage requirements and worst-case computational complexity per observation are independent of the number of previous observations. We propose an online changepoint detection algorithm for both univariate and multivariate data which compares favorably with offline changepoint detection algorithms while also operating in a strictly more constrained computational model. In addition, we present a simple online hyperparameter auto tuning technique for these algorithms.

preprint2022arXiv

The Zero-Coupon Rate Model for Derivatives Pricing

The aim of this paper is to present a dual-term structure model of interest rate derivatives in order to solve the two hardest problems in financial modeling: the exact volatility calibration of the entire swaption matrix, and the calculation of bucket vegas for structured products. The model takes a series of long-term zero-coupon rates as basic state variables that are driven directly by one or more Brownian motion. The model volatility is assigned in a matrix form with two terms. A numerical scheme for implementing the model has been developed in the paper. At the end, several examples have been given for the model calibration, the structured products pricing and the calculation of bucket vegas.

preprint2022arXiv

Titanium-based kagome superconductor CsTi_3Bi_5 and topological states

Since the discovery of a new family of vanadium-based kagome superconductor AV3Sb5 (A=K, Rb, and Cs) with topological band structures, extensive effort has been devoted to exploring the origin of superconducting states and the intertwined orders. Meanwhile, searching for new types of superconductors with novel physical properties and higher superconducting transition temperatures has always been a major thread in the history of superconductor research. Here we report a successful fabrication and the topological states of a Titanium-based kagome metal CsTi3Bi5 (CT3B5) crystal. The as-grown CT3B5 crystal is of high quality and possesses a perfect two-dimensional kagome net of Titanium. The superconductivity of the CT3B5 crystal shows that the critical temperature Tc is of ~4.8 K. First-principle calculations predict that the CT3B5 has robust topological surface states, implying that CT3B5 is a Z2 topological kagome superconductor. This finding provides a new type of superconductors and the base for exploring the origin of superconductivity and topological states in kagome superconductors.

preprint2022arXiv

Trigger Hunting with a Topological Prior for Trojan Detection

Despite their success and popularity, deep neural networks (DNNs) are vulnerable when facing backdoor attacks. This impedes their wider adoption, especially in mission critical applications. This paper tackles the problem of Trojan detection, namely, identifying Trojaned models -- models trained with poisoned data. One popular approach is reverse engineering, i.e., recovering the triggers on a clean image by manipulating the model's prediction. One major challenge of reverse engineering approach is the enormous search space of triggers. To this end, we propose innovative priors such as diversity and topological simplicity to not only increase the chances of finding the appropriate triggers but also improve the quality of the found triggers. Moreover, by encouraging a diverse set of trigger candidates, our method can perform effectively in cases with unknown target labels. We demonstrate that these priors can significantly improve the quality of the recovered triggers, resulting in substantially improved Trojan detection accuracy as validated on both synthetic and publicly available TrojAI benchmarks.

preprint2021arXiv

A perspective of twisted photonic structures

Moire superlattices-twisted van der Waals (vdW) structures with small angles-are attracting increasing attention in condensed matter physics, due to important phenomena revealed therein, including unconventional superconductivity, correlated insulating states, and ferromagnetism. Moire superlattices are typically comprised of atomic layers of vdW materials where the exotic physics arises from the quantum electronic coupling between adjacent atomic layers. Recently, moire electronics has motivated their photonic counterparts. In addition to vdW materials, twisted photonic systems can also be comprised of metamaterials, metasurfaces, and photonic crystals, mediated by interlayer electromagnetic coupling instead. The interplay between short-ranged interlayer quantum and long-ranged electromagnetic coupling in twisted structures are expected to yield rich phenomena in nano-optics. This perspective reviews recent progress in twisted structures for nanophotonics and outlooks emerging topics, opportunities, fundamental challenges, and potential applications.

preprint2021arXiv

Chirality locking charge density waves in a chiral crystal

In Weyl semimetals, charge density wave (CDW) order can spontaneously break the chiral symmetry, gap out the Weyl nodes, and drive the material into the axion insulating phase. Investigations have however been limited since CDWs are rarely seen in Weyl semimetals. Here, using scanning tunneling microscopy/spectroscopy, we report the discovery of a novel unidirectional CDW order on the (001) surface of chiral crystal CoSi - a unique Weyl semimetal with unconventional chiral fermions. The CDW is incommensurate with both lattice momentum and crystalline symmetry directions, and exhibits an intra unit cell π phase shift in the layer stacking direction. The tunneling spectrum shows a particle-hole asymmetric V-shaped energy gap around the Fermi level that modulates spatially with the CDW wave vector. Combined with first-principle calculations, we identify that the CDW is locked to the crystal chirality and is related by a mirror reflection between the two enantiomers of the chiral crystal. Our findings reveal a novel correlated topological quantum state in chiral CoSi crystals and raise the potential for realizing an axion insulator and exploring the unprecedented physical behaviors of unconventional chiral fermions.

preprint2021arXiv

Demonstration of negative refraction induced by synthetic gauge fields

The phenomenon of negative refraction generally requires negative refractive indices or phase discontinuities, which can be realized using metamaterials or metasurfaces. Recent theories have proposed a novel mechanism for negative refraction based on synthetic gauge fields, which affect classical waves as if they were charged particles in electromagnetic fields, but this has not hitherto been demonstrated in experiment. Here, we report on the experimental demonstration of gauge-field-induced negative refraction in a twisted bilayer acoustic metamaterial. The bilayer twisting produces a synthetic gauge field for sound waves propagating within a projected two-dimensional geometry, with the magnitude of the gauge field parameterized by the choice of wavenumber along the third dimension. Waveguiding with backward propagating modes is also demonstrated in a trilayer configuration that implements strong gauge fields. These results provide an alternative route to achieving negative refraction in synthetic materials.

preprint2021arXiv

Toggling Near-field Directionality via Polarization Control of Surface Waves

Directional excitation of guidance modes is central to many applications ranging from light harvesting, optical information processing to quantum optical technology. Of paramount interest, especially, the active control of near-field directionality provides a new paradigm for the real-time on-chip manipulation of light. Here we find that for a given dipolar source, its near-field directionality can be toggled efficiently via tailoring the polarization of surface waves that are excited, for example, via tuning the chemical potential of graphene in a graphene-metasurface waveguide. This finding enables a feasible scheme for the active near-field directionality. Counterintuitively, we reveal that this scheme can transform a circular electric/magnetic dipole into a Huygens dipole in the near-field coupling. Moreover, for Janus dipoles, this scheme enables us to actively flip their near-field coupling and non-coupling faces.

preprint2020arXiv

Broadband Enhancement of On-chip Single Photon Extraction via Tilted Hyperbolic Metamaterials

A fundamental building block for on-chip quantum photonics is a single-photon source with high repetition rates, which can enable many applications such as high-speed quantum communication and quantum information processing. Ideally, such single photon sources would then require a large on-chip photon extraction decay rate, namely the rate of excited photons coupled into nanofibers or waveguides, over a broad spectral range. However, this goal has remained elusive till date. Here we propose a feasible scheme to enhance the on-chip photon extraction decay rate of quantum emitters, through the tilting of the optical axis of hyperbolic metamaterials with respect to the end-facet of nanofibers. Importantly, the revealed scheme is applicable to arbitrarily orientated quantum emitters over a broad spectral range, e.g., up to ~80 nm for visible light. The underlying physics relies on the emerging unique feature of hyperbolic metamaterials if their optical axis is judiciously tilted. That is, their supported high-k (i.e., wavevector) hyperbolic eigenmodes, which are intrinsically confined inside them if their optical axis is un-tilted, can now become momentum-matched with the guided modes of nanofibers, and more importantly, they can safely couple into nanofibers almost without reflection.

preprint2020arXiv

Charge Transport in a Polar Metal

The fate of electric dipoles inside a Fermi sea is an old issue, yet poorly-explored. Sr$_{1-x}$Ca$_x$TiO$_{3}$ hosts a robust but dilute ferroelectricity in a narrow ($0.002<x<0.02$) window of substitution. This insulator becomes metallic by removal of a tiny fraction of its oxygen atoms. Here, we present a detailed study of low-temperature charge transport in Sr$_{1-x}$Ca$_x$TiO$_{3-δ}$, documenting the evolution of resistivity with increasing carrier concentration ($n$). Below a threshold carrier concentration, $n^*(x)$, the polar structural phase transition has a clear signature in resistivity and Ca substitution significantly reduces the 2 K mobility at a given carrier density. For three different Ca concentrations, we find that the phase transition fades away when one mobile electron is introduced for about $7.9\pm0.6$ dipoles. This threshold corresponds to the expected peak in anti-ferroelectric coupling mediated by a diplolar counterpart of Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction. Our results imply that the transition is driven by dipole-dipole interaction, even in presence of a dilute Fermi sea. Charge transport for $n < n^*(x)$ shows a non-monotonic temperature dependence, most probably caused by scattering off the transverse optical phonon mode. A quantitative explanation of charge transport in this polar metal remains a challenge to theory. For $n\geq n^*(x)$, resistivity follows a T-square behavior together with slight upturns (in both Ca-free and Ca-substituted samples). The latter are reminiscent of Kondo effect and most probably due to oxygen vacancies.

preprint2020arXiv

Chiral plasmons with twisted atomic bilayers

Van der Waals heterostructures of atomically thin layers with rotational misalignments, such as twisted bilayer graphene, feature interesting structural moiré superlattices. Due to the quantum coupling between the twisted atomic layers, light-matter interaction is inherently chiral; as such, they provide a promising platform for chiral plasmons in the extreme nanoscale. However, while the interlayer quantum coupling can be significant, its influence on chiral plasmons still remains elusive. Here we present the general solutions from full Maxwell equations of chiral plasmons in twisted atomic bilayers, with the consideration of interlayer quantum coupling. We find twisted atomic bilayers have a direct correspondence to the chiral metasurface, which simultaneously possesses chiral and magnetic surface conductivities, besides the common electric surface conductivity. In other words, the interlayer quantum coupling in twisted van der Waals heterostructures may facilitate the construction of various (e.g., bi-anisotropic) atomically-thin metasurfaces. Moreover, the chiral surface conductivity, determined by the interlayer quantum coupling, determines the existence of chiral plasmons and leads to a unique phase relationship (i.e., +/-π/2 phase difference) between their TE and TM wave components. Importantly, such a unique phase relationship for chiral plasmons can be exploited to construct the missing longitudinal spin of plasmons, besides the common transverse spin of plasmons.

preprint2020arXiv

Controlling Cherenkov threshold with nonlocality

Cherenkov radiation is generally believed to be threshold-free in hyperbolic metamaterials owing to the extremely large photonic density of states in classical local framework. While recent advances in nonlocal and quantum effects extend our understanding of light-matter interactions in metallic nanostructures, the influence of nonlocality on threshold-free Cherenkov radiation still remains elusive. Here we theoretically demonstrate that the nonlocality provides an indispensable way to flexibly engineer Cherenkov thresholds in metallodielectric layered structures. Particularly, the nonlocality results in a lower-bound velocity cutoff, whose value is comparable to the electron Fermi velocity. Surprisingly, this lower-bound threshold can be significantly smaller than the classically predicted one if the metamaterial works around epsilon-near-zero frequencies. The capability to control Cherenkov thresholds opens numerous prospects for practical applications of Cherenkov radiation, in particular, for integrated free-electron radiation sources.

preprint2020arXiv

Negative refraction of ultra-squeezed in-plane hyperbolic designer polaritons

The in-plane negative refraction of high-momentum (i.e., high-k) photonic modes could enable many applications such as imaging and hyperlensing in a planar platform at deep-subwavelength scales. However, its practical implementation in experiments remains elusive so far. Here we propose a class of hyperbolic metasurfaces, which is characterized by an anisotropic magnetic sheet conductivity and can support the in-plane ultrahigh-k magnetic designer polaritons. Based on such metasurfaces, we report the first experimental observation of the all-angle negative refraction of designer polaritons at extremely deep-subwavelength scales. Moreover, we directly visualize the designer polaritons with hyperbolic dispersions. Importantly, for these hyperbolic polaritons, we find that their squeezing factor is ultra-large and, to be specific, it can be up to 129 in the experiments, a record-breaking value exceeding those in naturally hyperbolic materials. The present scheme for the achievement of negative refraction is also applicable to other natural materials and may enable intriguing applications in nanophotonics. Besides, the proposed metasurfaces are readily tailorable in space and frequency, which could serve as a versatile platform to explore the extremely high confinement and unusual propagation of hyperbolic polaritons.

preprint2020arXiv

Semi-supervised Collaborative Filtering by Text-enhanced Domain Adaptation

Data sparsity is an inherent challenge in the recommender systems, where most of the data is collected from the implicit feedbacks of users. This causes two difficulties in designing effective algorithms: first, the majority of users only have a few interactions with the system and there is no enough data for learning; second, there are no negative samples in the implicit feedbacks and it is a common practice to perform negative sampling to generate negative samples. However, this leads to a consequence that many potential positive samples are mislabeled as negative ones and data sparsity would exacerbate the mislabeling problem. To solve these difficulties, we regard the problem of recommendation on sparse implicit feedbacks as a semi-supervised learning task, and explore domain adaption to solve it. We transfer the knowledge learned from dense data to sparse data and we focus on the most challenging case -- there is no user or item overlap. In this extreme case, aligning embeddings of two datasets directly is rather sub-optimal since the two latent spaces encode very different information. As such, we adopt domain-invariant textual features as the anchor points to align the latent spaces. To align the embeddings, we extract the textual features for each user and item and feed them into a domain classifier with the embeddings of users and items. The embeddings are trained to puzzle the classifier and textual features are fixed as anchor points. By domain adaptation, the distribution pattern in the source domain is transferred to the target domain. As the target part can be supervised by domain adaptation, we abandon negative sampling in target dataset to avoid label noise. We adopt three pairs of real-world datasets to validate the effectiveness of our transfer strategy. Results show that our models outperform existing models significantly.

preprint2020arXiv

Surface Dyakonov-Cherenkov Radiation

Recent advances in engineered material technologies (e.g., photonic crystals, metamaterials, plasmonics, etc) provide valuable tools to control Cherenkov radiation. In all these approaches, however, the designed materials interact only with the particle velocity to affect Cherenkov radiation, while the influence of the particle trajectory is generally negligible. Here, we report on surface Dyakonov-Cherenkov radiation, i.e. the emission of directional Dyakonov surface waves from a swift charged particle moving atop a birefringent crystal. This new type of Cherenkov radiation is highly susceptible to both the particle velocity and trajectory, e.g. we observe a sharp radiation enhancement when the particle trajectory falls in the vicinity of a particular direction. Moreover, close to the Cherenkov threshold, such a radiation enhancement can be orders of magnitude higher than that obtained in traditional Cherenkov detectors. These distinct properties allow us to determine simultaneously the magnitude and direction of particle velocities on a compact platform. The surface Dyakonov-Cherenkov radiation studied in this work not only adds a new degree of freedom for particle identification, but also provides an all-dielectric route to construct compact Cherenkov detectors with enhanced sensitivity.

preprint2020arXiv

T-square resistivity without Umklapp scattering in dilute metallic Bi$_2$O$_2$Se

The electrical resistivity of Fermi liquids (FLs) displays a quadratic temperature ($T$) dependence because of electron-electron (e-e) scattering. For such collisions to decay the charge current, there are two known mechanisms: inter-band scattering (identified by Baber) and Umklapp events. However, dilute metallic strontium titanate (STO) was found to display $T^2$ resistivity in absence of either of these two mechanisms. The presence of soft phonons and their possible role as scattering centers raised the suspicion that $T$-square resistivity in STO is not due to e-e scattering. Here, we present the case of Bi$_2$O$_2$Se, a layered semiconductor with hard phonons, which becomes a dilute metal with a small single-component Fermi surface upon doping. It displays $T$-square resistivity well below the degeneracy temperature where neither Umklapp nor interband scattering is conceivable. We observe a universal scaling between the prefactor of $T^2$ resistivity and the Fermi energy, which is an extension of the Kadowaki-Woods plot to dilute metals. Our results imply the absence of a satisfactory theoretical basis for the ubiquity of e-e driven $T$-square resistivity in Fermi liquids.

preprint2020arXiv

The Impact of Explanations on AI Competency Prediction in VQA

Explainability is one of the key elements for building trust in AI systems. Among numerous attempts to make AI explainable, quantifying the effect of explanations remains a challenge in conducting human-AI collaborative tasks. Aside from the ability to predict the overall behavior of AI, in many applications, users need to understand an AI agent's competency in different aspects of the task domain. In this paper, we evaluate the impact of explanations on the user's mental model of AI agent competency within the task of visual question answering (VQA). We quantify users' understanding of competency, based on the correlation between the actual system performance and user rankings. We introduce an explainable VQA system that uses spatial and object features and is powered by the BERT language model. Each group of users sees only one kind of explanation to rank the competencies of the VQA model. The proposed model is evaluated through between-subject experiments to probe explanations' impact on the user's perception of competency. The comparison between two VQA models shows BERT based explanations and the use of object features improve the user's prediction of the model's competencies.

preprint2019arXiv

Observation of an unpaired photonic Dirac point

At photonic Dirac points, electromagnetic waves are governed by the same equations as two-component massless relativistic fermions. However, photonic Dirac points are known to occur in pairs in "photonic graphene" and other similar photonic crystals, which necessitates special precautions to excite only states near one of the Dirac points. Systems hosting unpaired photonic Dirac points are significantly harder to realize, as they require broken time-reversal symmetry. Here, we report on the first observation of an unpaired Dirac point in a planar two-dimensional photonic crystal. The structure incorporates gyromagnetic materials, which break time-reversal symmetry; the unpaired Dirac point occurs when a parity-breaking parameter is fine-tuned to a topological transition between a photonic Chern insulator and a conventional photonic insulator phase. Evidence for the unpaired Dirac point is provided by transmission and field-mapping experiments, including a demonstration of strongly non-reciprocal reflection. This photonic crystal is suitable for investigating the unique features of two-dimensional Dirac states, such as one-way Klein tunneling.

preprint2016arXiv

Airy plasmons in graphene based waveguides

In this paper, we propose that both the quasi-transverse-magnetic (TM) and quasi-transverseelectric (TE) Airy plasmons can be supported in graphene-based waveguides. The solution of Airy plasmons is calculated analytically and the existence of Airy plasmons is studied under the paraxial approximation. Due to the tunability of the chemical potential of graphene, the self-accelerating behavior of quasi-TM Airy plasmons can be steered effectively, especially in multilayer graphene based waveguides. Besides the metals, graphene provides an additional platform to investigate the propagation of Airy plasmons and to design various plasmonic devices.

preprint2016arXiv

Colossal Seebeck coefficient of hopping electrons in (TMTSF)$_{2}$PF$_{6}$

We report on a study of Seebeck coefficient and resistivity in the quasi-one-dimensional conductor (TMTSF)$_{2}$PF$_{6}$ extended deep into the Spin-Density-Wave(SDW) state. The metal-insulator transition at $T_{SDW}$ = 12 K leads to a reduction in carrier concentration by seven orders of magnitude. Below 1 K, charge transport displays the behavior known as Variable Range Hopping (VRH). Until now, the Seebeck response of electrons in this regime has been barely explored and even less understood. We find that in this system, residual carriers, hopping from one trap to another, generate a Seebeck coefficient as large as 400 $k_{B}$/$e$. The results provide the first solid evidence for a long-standing prediction according to which hopping electrons in presence of Coulomb interaction can generate a sizeable Seebeck coefficient in the zero-temperature limit.

preprint2016arXiv

Design of Ultra-compact Graphene-based Superscatterers

The energy-momentum dispersion relation is a fundamental property of plasmonic systems. In this paper, we show that the method of dispersion engineering can be used for the design of ultra-compact graphene-based superscatterers. Based on the Bohr model, the dispersion relation of the equivalent planar waveguide is engineered to enhance the scattering cross section of a dielectric cylinder. Bohr conditions with different orders are fulfilled in multiple dispersion curves at the same resonant frequency. Thus the resonance peaks from the first and second order scattering terms are overlapped in the deepsubwavelength scale by delicately tuning the gap thickness between two graphene layers. Using this ultra-compact graphene-based superscatterer, the scattering cross section of the dielectric cylinder can be enhanced by five orders of magnitude.

preprint2016arXiv

Dynamical Mechanism of Two-Dimensional Plasmon Launching by Swift Electrons

Launching of surface plasmons by swift electrons has long been utilized in electron-energy-loss spectroscopy (EELS) to investigate plasmonic properties of ultrathin, or two-dimensional (2D), electron systems. However, its spatio-temporal process has never been revealed. This is because the impact of an electron will generate not only plasmons, but also photons, whose emission cannot be achieved at a single space-time point, as fundamentally determined from the uncertainty principle. Here, we propose that such a space-time limitation also applies to surface plasmon generation in EELS experiment. On the platform of graphene, we demonstrate within the framework of classical electrodynamics that the launching of 2D plasmons by an electron's impact is delayed after a hydrodynamic splashing-like process, which occurs during the plasmonic "formation time" when the electron traverses the "formation zone." Considering this newly revealed process, we show that previous estimates on the yields of graphene plasmons in EELS have been overestimated.

preprint2016arXiv

Ferromagnetic Quantum Critical Point Avoided by the Appearance of Another Magnetic Phase in LaCrGe$_3$ under Pressure

The temperature-pressure phase diagram of the ferromagnet LaCrGe$_3$ is determined for the first time from a combination of magnetization, muon-spin-rotation and electrical resistivity measurements. The ferromagnetic phase is suppressed near $2.1$~GPa, but quantum criticality is avoided by the appearance of a magnetic phase, likely modulated, AFM$_Q$. Our density functional theory total energy calculations suggest a near degeneracy of antiferromagnetic states with small magnetic wave vectors $Q$ allowing for the potential of an ordering wave vector evolving from $Q=0$ to finite $Q$, as expected from the most recent theories on ferromagnetic quantum criticality. Our findings show that LaCrGe$_3$ is a very simple example to study this scenario of avoided ferromagnetic quantum criticality and will inspire further study on this material and other itinerant ferromagnets.

preprint2016arXiv

Formation Mechanism of Guided Resonances and Bound States in the Continuum in Photonic Crystal Slabs

We develop a formalism, based on the mode expansion method, to describe the guided resonances and bound states in the continuum (BICs) in photonic crystal slabs with one-dimensional periodicity. This approach provides analytic insights to the formation mechanisms of these states: the guided resonances arise from the transverse Fabry-Pérot condition, and the divergence of the resonance lifetimes at the BICs is explained by a destructive interference of radiation from different propagating components inside the slab. We show BICs at the center and on the edge of the Brillouin zone protected by symmetry, as well as BICs at generic wave vectors not protected by symmetry.

preprint2016arXiv

Graphene induced mode bifurcation at low input power

We study analytically the plasmonic modes in the graphene-coated dielectric nanowire, based on the explicit form of nonlinear surface conductivity of graphene. The propagation constants of different plasmonic modes can be tuned by the input power at the order of a few tenths of mW. The lower and upper mode bifurcation branches are connected at the limitation value of the input power. Moreover, due to the nonlinearity of graphene, the dispersion curves of plasmonic modes at different input powers form an energy band, which is in sharp contrast with the single dispersion curve in the limit of zero input power.

preprint2016arXiv

Hybrid Airy Plasmons with Dynamically Steerable Trajectories

With the intriguing properties of diffraction-free, self-accelerating, and self-healing, Airy plasmons are promising to be used in the trapping, transporting, and sorting of micro-objects, imaging, and chip scale signal processing. However, the high dissipative loss and the lack of dynamical steerability restrict the implementation of Airy plasmons in these applications. Here we reveal the hybrid Airy plasmons for the first time by taking a hybrid graphene-based plasmonic waveguide in the terahertz (THz) domain as an example. Due to the coupling between an optical mode and a plasmonic mode, the hybrid Airy plasmons can have large propagation lengths and effective transverse deflections, where the transverse waveguide confinements are governed by the hybrid modes with moderate quality factors. Meanwhile, the propagation trajectories of hybrid Airy plasmons are dynamically steerable by changing the chemical potential of graphene. These hybrid Airy plasmons may promote the further discovery of non-diffracting beams with the emerging developments of optical tweezers and tractor beams.

preprint2016arXiv

Leveraging Visual Question Answering for Image-Caption Ranking

Visual Question Answering (VQA) is the task of taking as input an image and a free-form natural language question about the image, and producing an accurate answer. In this work we view VQA as a "feature extraction" module to extract image and caption representations. We employ these representations for the task of image-caption ranking. Each feature dimension captures (imagines) whether a fact (question-answer pair) could plausibly be true for the image and caption. This allows the model to interpret images and captions from a wide variety of perspectives. We propose score-level and representation-level fusion models to incorporate VQA knowledge in an existing state-of-the-art VQA-agnostic image-caption ranking model. We find that incorporating and reasoning about consistency between images and captions significantly improves performance. Concretely, our model improves state-of-the-art on caption retrieval by 7.1% and on image retrieval by 4.4% on the MSCOCO dataset.

preprint2016arXiv

Non-monotonic anisotropy in charge conduction induced by antiferrodistortive transition in metallic SrTiO$_{3}$

Cubic SrTiO$_{3}$ becomes tetragonal below 105 K. The antiferrodistortive (AFD) distortion leads to clockwise and counter-clockwise rotation of adjacent TiO$_{6}$ octahedra. This insulator becomes a metal upon the introduction of extremely low concentration of n-type dopants. However, signatures of the structural phase transition in charge conduction have remained elusive. Employing the Montgomery technique, we succeed in resolving the anisotropy of charge conductivity induced by the AFD transition, in the presence of different types of dopants. We find that the slight lattice distortion ($<6 \times 10^{-4}$) gives rise to a twenty percent anisotropy in charge conductivity, in agreement with the expectations of band calculations. Application of uniaxial strain amplifies the detectable anisotropy by disfavoring one of the three possible tetragonal domains. In contrast with all other known anisotropic Fermi liquids, the anisotropy has opposite signs for elastic and inelastic scattering. Increasing the concentration of dopants leads to a drastic shift in the temperature of the AFD transition either upward or downward. The latter result puts strong constraints on any hypothetical role played by the AFD soft mode in the formation of Cooper pairs and the emergence of superconductivity in SrTiO$_3$.

preprint2016arXiv

Probing topological protection using a designer surface plasmon structure

Topological photonic states, inspired by robust chiral edge states in topological insulators, have recently been demonstrated in a few photonic systems, including an array of coupled on-chip ring resonators at communication wavelengths. However, the intrinsic difference between electrons and photons determines that the topological protection in time-reversal-invariant photonic systems does not share the same robustness as its counterpart in electronic topological insulators. Here, in a designer surface plasmon platform consisting of tunable metallic sub-wavelength structures, we construct photonic topological edge states and probe their robustness against a variety of defect classes, including some common time-reversal-invariant photonic defects that can break the topological protection, but do not exist in electronic topological insulators. This is also the first experimental realization of anomalous Floquet topological edge states, whose topological phase cannot be predicted by the usual Chern number topological invariants.

preprint2016arXiv

Tailoring the energy distribution and loss of 2D plasmons

The ability to tailor the energy distribution of plasmons at the nanoscale has many applications in nanophotonics, such as designing plasmon lasers, spasers, and quantum emitters. To this end, we analytically study the energy distribution and the proper field quantization of 2D plasmons with specific examples for graphene plasmons. We find that the portion of the plasmon energy contained inside graphene (energy confinement factor) can exceed 50%, despite graphene being infinitely thin. In fact, this very high energy confinement can make it challenging to tailor the energy distribution of graphene plasmons just by modifying the surrounding dielectric environment or the geometry, such as changing the separation distance between two coupled graphene layers. However, by adopting concepts of parity-time symmetry breaking, we show that tuning the loss in one of the two coupled graphene layers can simultaneously tailor the energy confinement factor and propagation characteristics, causing the phenomenon of loss-induced plasmonic transparency.

preprint2016arXiv

Translation and Rotation of Transformation Media under Electromagnetic Pulse

It is well known that optical media create artificial geometry for light, and curved geometry acts as an effective optical medium. This correspondence originates from the form invariance of Maxwells equations, which recently has spawned a booming field called transformation optics. Here we investigate responses of three transformation media under electromagnetic pulses, and find that pulse radiation can induce unbalanced net force on transformation media, which will cause translation and rotation of transformation media although their final momentum can still be zero. Therefore, the transformation media do not necessarily stay the same after an electromagnetic wave passes through.

preprint2015arXiv

Atomically thin spherical shell-shaped superscatterers based on Bohr model

Graphene monolayers can be used for atomically thin three-dimensional shell-shaped superscatterer designs. Due to the excitation of the first-order resonance of transverse magnetic (TM) graphene plasmons, the scattering cross section of the bare subwavelength dielectric particle is enhanced significantly by five orders of magnitude. The superscattering phenomenon can be intuitively understood and interpreted with Bohr model. Besides, based on the analysis of Bohr model, it is shown that contrary to the TM case, superscattering is hard to occur by exciting the resonance of transverse electric (TE) graphene plasmons due to their poor field confinements.

preprint2015arXiv

Caustic graphene plasmons with Kelvin angle

A century-long argument made by Lord Kelvin that all swimming objects have an effective Mach number of 3, corresponding to the Kelvin angle of 19.5 degree for ship waves, has been recently challenged with the conclusion that the Kelvin angle should gradually transit to the Mach angle as the ship velocity increases. Here we show that a similar phenomenon can happen for graphene plasmons. By analyzing the caustic wave pattern of graphene plasmons stimulated by a swift charged particle moving uniformly above graphene, we show that at low velocities of the charged particle, the caustics of graphene plasmons form the Kelvin angle. At large velocities of the particle, the caustics disappear and the effective semi-angle of the wave pattern approaches the Mach angle. Our study introduces caustic wave theory to the field of graphene plasmonics, and reveals a novel physical picture of graphene plasmon excitation during electron energy-loss spectroscopy measurement.

preprint2015arXiv

Don't Just Listen, Use Your Imagination: Leveraging Visual Common Sense for Non-Visual Tasks

Artificial agents today can answer factual questions. But they fall short on questions that require common sense reasoning. Perhaps this is because most existing common sense databases rely on text to learn and represent knowledge. But much of common sense knowledge is unwritten - partly because it tends not to be interesting enough to talk about, and partly because some common sense is unnatural to articulate in text. While unwritten, it is not unseen. In this paper we leverage semantic common sense knowledge learned from images - i.e. visual common sense - in two textual tasks: fill-in-the-blank and visual paraphrasing. We propose to "imagine" the scene behind the text, and leverage visual cues from the "imagined" scenes in addition to textual cues while answering these questions. We imagine the scenes as a visual abstraction. Our approach outperforms a strong text-only baseline on these tasks. Our proposed tasks can serve as benchmarks to quantitatively evaluate progress in solving tasks that go "beyond recognition". Our code and datasets are publicly available.

preprint2015arXiv

Quantum oscillations, thermoelectric coefficients and the Fermi surface of semi-metallic WTe2

We present a study of angle-resolved quantum oscillations of electric and thermoelectric transport coefficients in semi-metallic WTe$_{2}$, which has the particularity of displaying a large B$^{2}$ magneto-resistance. The Fermi surface consists of two pairs of electron-like and hole-like pockets of equal volumes in a "Russian doll" structure. Carrier density, Fermi energy, mobility and the mean-free-path of the system are quantified. An additional frequency is observed above a threshold field and attributed to magnetic breakdown across two orbits. In contrast to all other dilute metals, the Nernst signal remains linear in magnetic field even in the high-field ($ω_cτ\gg 1$) regime. Surprisingly, none of the pockets extend across the c-axis of the first Brillouin zone, making the system a three-dimensional metal with moderate anisotropy in Fermi velocity yet a large anisotropy in mean-free-path.

preprint2015arXiv

Scalable T^2 resistivity in a small single-component Fermi surface

Scattering among electrons generates a distinct contribution to electrical resistivity that follows a quadratic temperature dependence. In strongly-correlated electron systems, the prefactor A of this T$^2$ resistivity scales with the magnitude of the electronic specific heat. Here, we show that one can change the magnitude of A by four orders of magnitude in metallic SrTiO3 by tuning the concentration of the carriers and consequently, the Fermi energy. The T$^2$ behavior persists in the single-band dilute limit despite the absence of two known mechanisms for T$^2$ behavior, distinct electron reservoirs and Umklapp processes. The results highlight the absence of a microscopic theory for momentum decay through electron-electron scattering in different Fermi liquids.

preprint2015arXiv

Topological Acoustics

The manipulation of acoustic wave propagation in fluids has numerous applications, including some in everyday life. Acoustic technologies frequently develop in tandem with optics, using shared concepts such as waveguiding and metamedia. It is thus noteworthy that an entirely novel class of electromagnetic waves, known as topological edge states, has recently been demonstrated. These are inspired by the electronic edge states occurring in topological insulators, and possess a striking and technologically promising property: the ability to travel in a single direction along a surface without backscattering, regardless of the existence of defects or disorder. Here, we develop an analogous theory of topological fluid acoustics, and propose a scheme for realizing topological edge states in an acoustic structure containing circulating fluids. The phenomenon of disorder-free one-way sound propagation, which does not occur in ordinary acoustic devices, may have novel applications for acoustic isolators, modulators, and transducers.

preprint2014arXiv

Combining the Best of Graphical Models and ConvNets for Semantic Segmentation

We present a two-module approach to semantic segmentation that incorporates Convolutional Networks (CNNs) and Graphical Models. Graphical models are used to generate a small (5-30) set of diverse segmentations proposals, such that this set has high recall. Since the number of required proposals is so low, we can extract fairly complex features to rank them. Our complex feature of choice is a novel CNN called SegNet, which directly outputs a (coarse) semantic segmentation. Importantly, SegNet is specifically trained to optimize the corpus-level PASCAL IOU loss function. To the best of our knowledge, this is the first CNN specifically designed for semantic segmentation. This two-module approach achieves $52.5\%$ on the PASCAL 2012 segmentation challenge.

preprint2014arXiv

Critical doping for the onset of a two-band superconducting ground state in SrTiO$_{3-δ}$

In doped SrTiO$_{3}$ superconductivity persists down to an exceptionally low concentration of mobile electrons. This restricts the relevant energy window and possible pairing scenarios. We present a study of quantum oscillations and superconducting transition temperature, $T_{c}$ as the carrier density is tuned from $10^{17}$ to $10^{20}$ $cm^{-3}$ and identify two critical doping levels corresponding to the filling thresholds of the upper bands. At the first critical doping, which separates the single-band and the two-band superconducting regimes in oxygen-deficient samples, the steady increase of T$_{c}$ with carrier concentration suddenly stops. Near this doping level, the energy dispersion in the lowest band displays a downward deviation from parabolic behavior. The results impose new constraints for microscopic pairing scenarios.

preprint2014arXiv

Model-Driven Data Collection for Biological Systems

For biological experiments aiming at calibrating models with unknown parameters, a good experimental design is crucial, especially for those subject to various constraints, such as financial limitations, time consumption and physical practicability. In this paper, we discuss a sequential experimental design based on information theory for parameter estimation and apply it to two biological systems. Two specific issues are addressed in the proposed applications, namely the determination of the optimal sampling time and the optimal choice of observable. The optimal design, either sampling time or observable, is achieved by an information-theoretic sensitivity analysis. It is shown that this is equivalent with maximizing the mutual information and contrasted with non-adaptive designs, this information theoretic strategy provides the fastest reduction of uncertainty.

preprint2014arXiv

Multiple nodeless superconducting gaps in optimally-doped SrTi$_{1-x}$Nb$_{x}$O$_{3}$

We present the first study of thermal conductivity in superconducting SrTi$_{1-x}$Nb$_{x}$O$_{3}$, sufficiently doped to be near its maximum critical temperature. The bulk critical temperature, determined by the jump in specific heat, occurs at a significantly lower temperature than the resistive T$_{c}$. Thermal conductivity, dominated by the electron contribution, deviates from its normal-state magnitude at bulk T$_{c}$, following a Bardeen-Rickayzen-Tewordt (BRT) behavior, expected for thermal transport by Bogoliubov excitations. Absence of a T-linear term at very low temperatures rules out the presence of nodal quasi-particles. On the other hand, the field dependence of thermal conductivity points to the existence of at least two distinct superconducting gaps. We conclude that optimally-doped strontium titanate is a multigap nodeless superconductor.

preprint2013arXiv

Fermi surface of the most dilute superconductor

The origin of superconductivity in bulk SrTiO$_{3}$ is a mystery, since the non-monotonous variation of the critical transition with carrier concentration defies the expectations of the crudest version of the BCS theory. Here, employing the Nernst effect, an extremely sensitive probe of tiny bulk Fermi surfaces, we show that down to concentrations as low as $5.5 \times 10^{17}cm^{-3}$, the system has both a sharp Fermi surface and a superconducting ground state. The most dilute superconductor currently known has therefore a metallic normal state with a Fermi energy as little as 1.1 meV on top of a band gap as large as 3 eV. Occurrence of a superconducting instability in an extremely small, single-component and barely anisotropic Fermi surface implies strong constraints for the identification of the pairing mechanism.

preprint2013arXiv

Suppression of ferromagnetism in the La(V$_x$Cr$_{1-x}$)Sb$_3$ system

To explore the possibility of quantum phase transitions and even quantum criticality in LaCrSb$_3$ based compounds, we performed measurements under pressure as well as a vanadium substitution study. The Curie temperature of LaCrSb$_3$ was found to be invariant under pressure. Although pressure was not able to suppress the ferromagnetism, chemical substitution was used as another parameter to tune the magnetism. We grew La(V$_x$Cr$_{1-x}$)Sb$_3$ (\textit{x} = 0 -- 1.0) single crystals, and studied the series by measurements of temperature and field dependent magnetic susceptibility, magnetization, resistivity, and specific heat. Ferromagnetism has been observed for $x \leq 0.22$, and the system manifests a strong anisotropy in its ordered state. The Curie temperature decreases monotonically as the V concentration increases. For $0.42 \leq x \leq 0.73$, the system enters a new magnetic state at low temperatures, and no magnetic ordering above 1.8 K can be observed for $x \geq 0.88$. The effective moment $μ_{\rm eff}$/Cr varies only slightly as the V concentration increases, from 3.9 $μ_{\rm B}$ for $x$ = 0 to 2.9 $μ_{\rm B}$ for $x$ = 0.88. Features related to quantum criticality have not been observed in the La(V$_x$Cr$_{1-x}$)Sb$_3$ system.

preprint2013arXiv

Suppression of ferromagnetism in the LaVxCr1-xGe3 system

We report synthesis of hexagonal LaVxCr1-xGe3 (x = 0-0.21, 1.00) single crystals, and present a systematic study of this series by measurements of temperature and field dependent magnetic susceptibility, magnetization, resistivity, and specific heat. Ferromagnetism has been observed for x = 0-0.21, and the system manifests a strong axial anisotropy in its ordered state. The decrease of the saturated moment and the effective moment per Cr with the increase of V-concentration suggests this is an itinerant ferromagnetic system. The Curie temperature declines monotonically as the V-concentration increases. Single crystalline samples could only be grown for x-values up to 0.21 for which the transition temperature was suppressed down to 36 K. Although we could not fully suppress TC via V-substitution, for x = 0.16, we performed magnetization measurements under pressure. The ferromagnetic state is suppressed under pressure at an initial rate of dTC/dp = -11.7 K/GPa and vanishes by 3.3 GPa.

preprint2013arXiv

Thermodynamic and transport properties of single crystalline RCo$_{2}$Ge$_{2}$ (R = Y, La-Nd, Sm-Tm)

Single crystals of RCo$_{2}$Ge$_{2}$ (R = Y, La-Nd, Sm-Tm) were grown using a self-flux method and were characterized by room-temperature powder x-ray diffraction; anisotropic, temperature and field dependent magnetization; temperature and field dependent, in-plane resistivity; and specific heat measurements. In this series, the majority of the moment-bearing members order antiferromagnetically; YCo$_{2}$Ge$_{2}$ and LaCo$_{2}$Ge$_{2}$ are non-moment-bearing. Ce is trivalent in CeCo$_{2}$Ge$_{2}$ at high temperatures, and exhibits an enhanced electronic specific heat coefficient due to Kondo effect at low temperatures. In addition, CeCo$_{2}$Ge$_{2}$ shows two low-temperature anomalies in temperature-dependent magnetization and specific heat measurements. Three members (R = Tb-Ho) have multiple phase transitions above 1.8 K. Eu appears to be divalent with total angular momentum L = 0. Both EuCo$_{2}$Ge$_{2}$ and GdCo$_{2}$Ge$_{2}$ manifest essentially isotropic paramagnetic properties consistent with J = S = 7/2. Clear magnetic anisotropy for rare-earth members with finite L was observed, with ErCo$_{2}$Ge$_{2}$ and TmCo$_{2}$Ge$_{2}$ manifesting planar anisotropy and the rest members manifesting axial anisotropy. The experimentally estimated crystal electric field (CEF) parameters B$_{2}^{0}$ were calculated from the anisotropic paramagnetic $θ_{ab}$ and $θ_{c}$ values and follow a trend that agrees well with theoretical predictions. The ordering temperatures, T$_{N}$, as well as the polycrystalline averaged paramagnetic Curie-Weiss temperature, $Θ_{avg}$, for the heavy rare-earth members deviate from the de Gennes scaling, as the magnitude of both are the highest for Tb, which is sometimes seen for extremely axial systems. Except for SmCo$_{2}$Ge$_{2}$, metamagnetic transitions were observed at 1.8 K for all members that ordered antiferromagnetically.

preprint2012arXiv

Anisotropic magnetization and resistivity of single crystalline RNi1-xBi2+-y (R = La-Nd, Sm, Gd-Dy)

We present a detailed study of RNi1-xBi2+-y (R = La-Nd, Sm, Gd-Dy) single crystals by measurements of stoichiometry and temperature dependent magnetic susceptibility, magnetization, and electrical resistivity. This series forms with partial Ni occupancy as well as a variable Bi occupancy. For R = Ce-Nd, Sm, Gd-Dy, the RNi1-xBi2+-y compounds show local-moment like behavior and order antiferromagnetically at low temperatures. Determination of anisotropies as well as antiferromagnetic ordering temperatures for RNi1-xBi2+-y (R = Ce-Nd, Sm, Gd-Dy) have been made. Although crystalline samples from this family exhibit minority, second phase superconductivity at low temperatures associated with Ni-Bi and Bi contamination, no evidence of bulk superconductivity has been observed.

preprint2012arXiv

Anisotropic magnetization, resistivity and heat capacity of single crystalline R3Ni2-xSn7 (R = La, Ce, Pr and Nd)

We present a detailed study of R3Ni2-xSn7 (R = La, Ce, Pr and Nd) single crystals by measurements of crystal structure, stoichiometry, temperature dependent magnetic susceptibility, magnetization, electrical resistivity, magnetoresistance, and specific heat. This series forms with partial Ni occupancy with x varying from ~ 0.1 for R = La to ~0.7 for R = Nd. The electrical resistivity of this series follows metallic behavior at high temperatures. Determination of clear anisotropies as well as antiferromagnetic ordering temperatures for R3Ni2-xSn7 (R = Ce, Pr and Nd) have been made. For Pr3Ni1.56Sn7 and Nd3Ni1.34Sn7, multiple magnetic transitions take place upon cooling. Metamagnetic transitions in this family (R = Ce, Pr and Nd) were detected for applied magnetic fields below 70 kOe. An H-T phase diagram of Ce3Ni1.69Sn7 was assembled to shed light on its low field properties and to rule out possible quantum critical effects.

preprint2012arXiv

Optical and electronic properties of two dimensional graphitic silicon carbide

Optical and electronic properties of two dimensional few layers graphitic silicon carbide (GSiC), in particular monolayer and bilayer, are investigated by density functional theory and found different from that of graphene and silicene. Monolayer GSiC has direct bandgap while few layers exhibit indirect bandgap. The bandgap of monolayer GSiC can be tuned by an in-plane strain. Properties of bilayer GSiC are extremely sensitive to the interlayer distance. These predictions promise that monolayer GSiC could be a remarkable candidate for novel type of light-emitting diodes utilizing its unique optical properties distinct from graphene, silicene and few layers GSiC.

preprint2012arXiv

Physical properties of single crystalline BaSn5

We present a comprehensive study of the binary intermetallic superconductor, BaSn5. High-quality single crystalline BaSn5 was grown out of Sn flux. Detailed thermodynamic and transport measurements were performed to study BaSn5's normal and superconducting state properties. This material appears to be a strongly coupled, multiband superconductor. Hc2(T)is almost isotropic. De Haas-van Alphen oscillations were observed and two effective masses were estimated from the FFT spectra. Hydrostatic pressure causes a decrease in the superconducting transition temperature at the rate of ~ -0.053 K/kbar.

preprint2011arXiv

CeNiAsO: an antiferromagnetic dense Kondo lattice

A cerium containing pnictide, CeNiAsO, crystallized in the ZrCuSiAs type structure, has been investigated by measuring transport and magnetic properties, as well as specific heat. We found that CeNiAsO is an antiferromagnetic dense Kondo lattice metallic compound with Kondo scale $T_K \sim$ 15 K and shows an enhanced Sommerfeld coefficient of $γ_0 \sim$ 203 mJ/mol$\cdot$K$^{2}$. While no superconductivity can been observed down to 30 mK, Ce ions exhibit two successive antiferromagnetic (AFM) transitions. We propose that the magnetic moment of Ce ion could align in the G type AFM order below the first transition at $T_{N1}$=9.3 K, and it might be modified into the C type AFM order below a lower transition at $T_{N2}$=7.3 K. Our results indicate that the 3$d-4f$ interlayer Kondo interactions play an important role in Ni-based Ce-containing pnictide.

preprint2011arXiv

Physical properties of SrSn4 single crystals

We present detailed thermodynamic and transport measurements on single crystals of the recently discovered binary intermetallic superconductor, SrSn4. We find this material to be a slightly anisotropic three-dimensional, strongly-coupled, possibly multi-band, superconductor. Hydrostatic pressure causes a decrease in the superconducting transition temperature at the rate of -0.068 K/kbar. Band structure calculations are consistent with experimental data on Sommerfeld coefficient and upper superconducting critical field anisotropy and suggest complex, multi-sheet Fermi surface formed by four bands.

preprint2010arXiv

Comparative study on the thermoelectric effect of parent oxypnictides La$T$AsO ($T$ = Fe, Ni)

The thermopower and Nernst effect were investigated for undoped parent compounds LaFeAsO and LaNiAsO. Both thermopower and Nernst signal in iron-based LaFeAsO are significantly larger than those in nickel-based LaNiAsO. Furthermore, abrupt changes in both thermopower and Nernst effect are observed below the structural phase transition temperature and spin-density wave (SDW) type antiferromagnetic (AFM) order temperature in Fe-based LaFeAsO. On the other hand, Nernst effect is very small in the Ni-based LaNiAsO and it is weakly temperature-dependent, reminiscent of the case in normal metals. We suggest that the effect of SDW order on the spin scattering rate should play an important role in the anomalous temperature dependence of Hall effect and Nernst effect in LaFeAsO. The contrast behavior between the LaFeAsO and LaNiAsO systems implies that the LaFeAsO system is fundamentally different from the LaNiAsO system and this may provide clues to the mechanism of high $T_c$ superconductivity in the Fe-based systems.

preprint2009arXiv

Evidence of Magnetically Driven Structural Phase Transition in Parent Compounds RFeAsO (R = La, Sm, Gd, Tb): study of low-temperature X-ray diffraction

We report measurements of structural phase transition of four parent compounds $R$FeAsO ($R$ = La, Sm, Gd, and Tb) by means of low-temperature X-ray diffraction (XRD). Magnetic transition temperatures associated with Fe ions ($T_{N1}$) are also determined from the temperature dependence of resistivity. As $R$ is changed from La, through Sm and Gd, to Tb, both the c-axis and a-axis lattice constants decrease significantly. Meanwhile both the structural phase transition temperature ($T_S$) and $T_{N1}$ decrease monotonously. It is also found that the temperature gap between $T_S$ and $T_{N1}$ becomes smaller when the distance between FeAs layer becomes shorter. This result is consistent with magnetically driven structural phase transition and suggests that the dimensionality have an important effect on the AFM ordering.