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Anisotropic magnetization and resistivity of single crystalline RNi1-xBi2+-y (R = La-Nd, Sm, Gd-Dy)

We present a detailed study of RNi1-xBi2+-y (R = La-Nd, Sm, Gd-Dy) single crystals by measurements of stoichiometry and temperature dependent magnetic susceptibility, magnetization, and electrical resistivity. This series forms with partial Ni occupancy as well as a variable Bi occupancy. For R = Ce-Nd, Sm, Gd-Dy, the RNi1-xBi2+-y compounds show local-moment like behavior and order antiferromagnetically at low temperatures. Determination of anisotropies as well as antiferromagnetic ordering temperatures for RNi1-xBi2+-y (R = Ce-Nd, Sm, Gd-Dy) have been made. Although crystalline samples from this family exhibit minority, second phase superconductivity at low temperatures associated with Ni-Bi and Bi contamination, no evidence of bulk superconductivity has been observed.

preprint2012arXivOpen access
Xiao LinWarren E. StraszheimSergey L. Bud'koPaul C. Canfield
cond-mat.supr-concond-mat.str-el
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Xiao LinWarren E. StraszheimSergey L. Bud'koPaul C. Canfield

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