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Fei Zhou

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Published work

53 published item(s)

preprint2026arXiv

UniTriGen: Unified Triplet Generation of Aligned Visible-Infrared-Label for Few-Shot RGB-T Semantic Segmentation

RGB-T semantic segmentation requires strictly aligned VIS-IR-Label triplets; however, such aligned triplet data are often scarce in real-world scenarios. Existing generative augmentation methods usually adopt cascaded generation paradigms, decomposing joint triplet generation into local conditional processes. As a result, consistency among VIS, IR, and Label in spatial structure, semantic content, and cross-modal details cannot be reliably maintained. To address this issue, we propose UniTriGen, a unified triplet generation framework that directly generates spatially aligned, semantically consistent, and modality complementary VIS-IR-Label triplets under the guidance of text prompts. UniTriGen first introduces a unified triplet generation mechanism, where VIS, IR, and Label are jointly encoded into a shared latent space and modeled with a diffusion process to enforce global cross-modal consistency. Lightweight modality-specific residual adapters are further integrated into this mechanism to accommodate modality-specific imaging characteristics and output formats. To mitigate generation bias caused by imbalanced scene and class distributions in limited paired triplets, UniTriGen also employs a scene-balanced and class-aware few-shot sampling strategy, which induces a more balanced sampling distribution and enhances the scene and class diversity of generated triplets. Experiments show that UniTriGen generates high-quality aligned triplets from limited real paired data, thereby achieving consistent performance improvements across various RGB-T semantic segmentation models.

preprint2022arXiv

An Interaction Bulk-Boundary Relation and its Applications Towards Symmetry Breaking and Beyond

In this article, we propose a simple but general scaling relation between interactions in a gapped bulk topological matter and gapless interacting surface states. We explicitly illustrate such a generic bulk-boundary relation (BBR) for a few specific interactions in a topological quantum matter, where we can perform dimensional reduction of a microscopic bulk theory to project out interacting surfaces. We have examined renormalization effects of the gapped bulk fermions on the interacting topological surface fermions. As simple applications, we utilize effective interacting quantum fields implied by BBR to explore feasibility of routes to various fascinating emergent phenomena on surfaces including emergent Majorana fermions induced by spontaneous symmetry breaking. We obtain sufficient conditions for these interacting surface phenomena to take place. We have also found that for given bulk electron-phonon interactions and when Ω_{D} \geq m, the phonon-mediated interactions on surface are strongest if the bulk Debye frequency Ω_{D} matches m, the mass gap of the topological matter

preprint2022arXiv

Detection of DC electric forces with zeptonewton sensitivity by single-ion phonon laser

Detecting extremely small forces helps exploring new physics quantitatively. Here we demonstrate that the phonon laser made of a single trapped $^{40}$Ca$^{+}$ ion behaves as an exquisite sensor for small force measurement. We report our successful detection of small electric forces regarding the DC trapping potential with sensitivity of 2.41$\pm$0.49 zN/$\sqrt{\rm Hz}$, with the ion only under Doppler cooling, based on the injection-locking of the oscillation phase of the phonon laser in addition to the classical squeezing applied to suppress the measurement uncertainty. We anticipate that such a single-ion sensor would reach a much better force detection sensitivity in the future once the trapping system is further improved and the fluorescence collection efficiency is further enhanced.

preprint2022arXiv

Portable ground stations for space-to-ground quantum key distribution

Quantum key distribution (QKD) uses the fundamental principles of quantum mechanics to share unconditionally secure keys between distant users. Previous works based on the quantum science satellite "Micius" have initially demonstrated the feasibility of a global QKD network. However, the practical applications of space-based QKD still face many technical problems, such as the huge size and weight of ground stations required to receive quantum signals. Here, we report space-to-ground QKD demonstrations based on portable receiving ground stations. The weight of the portable ground station is less than 100 kg, the space required is less than 1 m$^{3}$ and the installation time requires no more than 12 hours, all of the weight, required space and deployment time are about two orders of magnitude lower than those for the previous systems. Moreover, the equipment is easy to handle and can be placed on the roof of buildings in a metropolis. Secure keys have been successfully generated from the "Micius" satellite to these portable ground stations at six different places in China, and an average final secure key length is around 50 kb can be obtained during one passage. Our results pave the way for, and greatly accelerate the practical application of, space-based QKD.

preprint2022arXiv

Restoration of User Videos Shared on Social Media

User videos shared on social media platforms usually suffer from degradations caused by unknown proprietary processing procedures, which means that their visual quality is poorer than that of the originals. This paper presents a new general video restoration framework for the restoration of user videos shared on social media platforms. In contrast to most deep learning-based video restoration methods that perform end-to-end mapping, where feature extraction is mostly treated as a black box, in the sense that what role a feature plays is often unknown, our new method, termed Video restOration through adapTive dEgradation Sensing (VOTES), introduces the concept of a degradation feature map (DFM) to explicitly guide the video restoration process. Specifically, for each video frame, we first adaptively estimate its DFM to extract features representing the difficulty of restoring its different regions. We then feed the DFM to a convolutional neural network (CNN) to compute hierarchical degradation features to modulate an end-to-end video restoration backbone network, such that more attention is paid explicitly to potentially more difficult to restore areas, which in turn leads to enhanced restoration performance. We will explain the design rationale of the VOTES framework and present extensive experimental results to show that the new VOTES method outperforms various state-of-the-art techniques both quantitatively and qualitatively. In addition, we contribute a large scale real-world database of user videos shared on different social media platforms. Codes and datasets are available at https://github.com/luohongming/VOTES.git

preprint2021arXiv

Authentication of Metropolitan Quantum Key Distribution Network with Post-quantum Cryptography

Quantum key distribution (QKD) provides information theoretically secures key exchange requiring authentication of the classic data processing channel via pre-sharing of symmetric private keys. In previous studies, the lattice-based post-quantum digital signature algorithm Aigis-Sig, combined with public-key infrastructure (PKI) was used to achieve high-efficiency quantum security authentication of QKD, and its advantages in simplifying the MAN network structure and new user entry were demonstrated. This experiment further integrates the PQC algorithm into the commercial QKD system, the Jinan field metropolitan QKD network comprised of 14 user nodes and 5 optical switching nodes. The feasibility, effectiveness and stability of the post-quantum cryptography (PQC) algorithm and advantages of replacing trusted relays with optical switching brought by PQC authentication large-scale metropolitan area QKD network were verified. QKD with PQC authentication has potential in quantum-secure communications, specifically in metropolitan QKD networks.

preprint2021arXiv

Dynamics of strongly interacting Fermi gases with time-dependent interactions: Consequence of conformal symmetry

In this Letter, we investigate the effects of a time-dependent, short-ranged interaction on the long-time expansion dynamics of Fermi gases. We show that the effects of the interaction on the dynamics is dictated by how it changes under a conformal transformation, and derive an explicit criterion for the relevancy of time-dependent interactions in both the strongly and non-interacting nearly scale invariant quantum gases. In addition, we show that it is possible to engineer interactions that give rise to non-exponential thermalization dynamics in trapped Fermi gases. To supplement the symmetry analysis, we also perform hydrodynamic simulations to show that the moment of inertia of the trapped gas indeed follows a universal time-dependence determined jointly by the conformal symmetry and time-dependent scattering length $a(t)$. Our results should also be relevant to the dynamics of other systems that are nearly scale invariant and that are governed by a non-relativistic conformal symmetry.

preprint2021arXiv

Topological Quantum Critical Points in Strong Coupling limits: Global Symmetries and Strongly Interacting Majorana Fermions

In this article, we discuss strong coupling limits of topological quantum critical points (TQCPs) where quantum phase transitions between two topological distinct superconducting states take place. We illustrate that while superconducting phases on both sides of TQCPs spontaneously break same symmetries, universality classes of critical states can be identified only when global symmetries in topological states are further specified. In dimensions $d=2,3$, we find that continuous $(d+1)$th order transitions at weakly interacting TQCPs that were pointed out previously in the presence of emergent Lorentz symmetry can be terminated by strongly interacting fixed points of majorana fields. For $2d$ time reversal symmetry breaking TQCPs, termination points are supersymmetric with ${\mathcal N}=4N_f={1}$ (where $N_f$ is the number of four-component Dirac fermions and ${\mathcal N}$ is the number of two-component real fermions) beyond which transitions are discontinuous first order ones. For $2d$ time reversal symmetric TQCPs without other global symmetries, termination points of $(d+1)$th order continuous transition lines are generically conformal invariant without supersymmetry. Beyond these strong coupling fixed points, there are first-order discontinuous transitions as far as the protecting symmetry is not spontaneously broken but no direct transitions if the protecting symmetry is spontaneously broken in the presence of strong interactions. In $3d$, strong coupling termination points can be further effectively represented by new emergent gapless real bosons weakly coupled with free gapless majorana fermions. However, in $1d$, time reversal symmetric $(d+1)$th continuous transition lines of TQCPs are terminated by simple free majorana fermion fixed points.

preprint2021arXiv

VHS to HDTV Video Translation using Multi-task Adversarial Learning

There are large amount of valuable video archives in Video Home System (VHS) format. However, due to the analog nature, their quality is often poor. Compared to High-definition television (HDTV), VHS video not only has a dull color appearance but also has a lower resolution and often appears blurry. In this paper, we focus on the problem of translating VHS video to HDTV video and have developed a solution based on a novel unsupervised multi-task adversarial learning model. Inspired by the success of generative adversarial network (GAN) and CycleGAN, we employ cycle consistency loss, adversarial loss and perceptual loss together to learn a translation model. An important innovation of our work is the incorporation of super-resolution model and color transfer model that can solve unsupervised multi-task problem. To our knowledge, this is the first work that dedicated to the study of the relation between VHS and HDTV and the first computational solution to translate VHS to HDTV. We present experimental results to demonstrate the effectiveness of our solution qualitatively and quantitatively.

preprint2020arXiv

Gene-Environment Interaction: A Variable Selection Perspective

Gene-environment interactions have important implications to elucidate the genetic basis of complex diseases beyond the joint function of multiple genetic factors and their interactions (or epistasis). In the past, G$\times$E interactions have been mainly conducted within the framework of genetic association studies. The high dimensionality of G$\times$E interactions, due to the complicated form of environmental effects and presence of a large number of genetic factors including gene expressions and SNPs, has motivated the recent development of penalized variable selection methods for dissecting G$\times$E interactions, which has been ignored in majority of published reviews on genetic interaction studies. In this article, we first survey existing overviews on both gene-environment and gene-gene interactions. Then, after a brief introduction on the variable selection methods, we review penalization and relevant variable selection methods in marginal and joint paradigms respectively under a variety of conceptual models. Discussions on strengths and limitations, as well as computational aspects of the variable selection methods tailored for G$\times$E studies have also been provided.

preprint2020arXiv

Robust Bayesian variable selection for gene-environment interactions

Gene-environment (G$\times$E) interactions have important implications to elucidate the etiology of complex diseases beyond the main genetic and environmental effects. Outliers and data contamination in disease phenotypes of G$\times$E studies have been commonly encountered, leading to the development of a broad spectrum of robust regularization methods. Nevertheless, within the Bayesian framework, the issue has not been taken care of in existing studies. We develop a fully Bayesian robust variable selection method for G$\times$E interaction studies. The proposed Bayesian method can effectively accommodate heavy-tailed errors and outliers in the response variable while conducting variable selection by accounting for structural sparsity. In particular, for the robust sparse group selection, the spike-and-slab priors have been imposed on both individual and group levels to identify important main and interaction effects robustly. An efficient Gibbs sampler has been developed to facilitate fast computation. Extensive simulation studies and analysis of both the diabetes data with SNP measurements from the Nurses' Health Study and TCGA melanoma data with gene expression measurements demonstrate the superior performance of the proposed method over multiple competing alternatives.

preprint2020arXiv

Selection of strain and fitting schemes for calculating higher-order elastic constants

Criteria of selecting strain and fitting schemes are proposed for the calculation of higher-order elastic constants more efficiently, robustly and accurately. As demonstrated by the third-order elastic constants (TOECs) of diamond, the proposed method is 3-5 times faster than existing methods, and the range of strain for getting correct TOECs is expanded. In addition, our result provides an evidence for the inaccuracy of some previous experiments caused by higher-order effect, and the difference among experiments and several different theoretical methods is resolved. Finally, we give the recommend TOECs values for diamond.

preprint2020arXiv

Self-Supervised Learning and Prediction of Microstructure Evolution with Recurrent Neural Networks

Microstructural evolution is a key aspect of understanding and exploiting the structure-property-performance relation of materials. Modeling microstructure evolution usually relies on coarse-grained simulations with evolution principles described by partial differential equations (PDEs). Here we demonstrate that convolutional recurrent neural networks can learn the underlying physical rules and replace PDE-based simulations in the prediction of microstructure phenomena. Neural nets are trained by self-supervised learning with image sequences from simulations of several common processes, including plane wave propagation, grain growth, spinodal decomposition and dendritic crystal growth. The trained networks can accurately predict both short-term local dynamics and long-term statistical properties of microstructures and is capable of extrapolating beyond the training datasets in spatiotemporal domains and configurational and parametric spaces. Such a data-driven approach offers significant advantages over PDE-based simulations in time stepping efficiency and offers a useful alternative especially when the material parameters or governing PDEs are not well determined.

preprint2020arXiv

Tricritical physics in two-dimensional $p$-wave superfluids

We study effects of quantum fluctuations on two-dimensional $p+ip$ superfluids near resonance. In the standard paradigm, phase transitions between superfluids and zero density vacuum are continuous. When strong quantum fluctuations near resonance are taken into account, the line of continuous phase transitions terminates at two multicritical points near resonance, between which the transitions are expected to be first-order ones. The size of the window where first-order phase transitions occur is shown to be substantial when the coupling is strong. Near first-order transitions, superfluids self-contract due to phase separations between superfluids and vacuum.

preprint2016arXiv

Crystal field calculations for transition metal ions by application of an opposing potential

We propose a fully ab initio method, the opposing crystal potential (OCP), to calculate the crystal field parameters of transition metal impurities in insulator hosts. Through constrained density functional calculations, OCP obtains the constraining Lagrange multipliers, which act as cancellation potential against the crystal field and lead to spherical $d$-electron distribution. The method is applied to several insulators doped with Mn$^{4+}$ and Mn$^{2+}$ ions and shown to be in good agreement with experiment.

preprint2016arXiv

Integrated four-channel all-fiber up-conversion single-photon-detector with adjustable efficiency and dark count

Up-conversion single photon detector (UCSPD) has been widely used in many research fields including quantum key distribution (QKD), lidar, optical time domain reflectrometry (OTDR) and deep space communication. For the first time in laboratory, we have developed an integrated four-channel all-fiber UCSPD which can work in both free-running and gate modes. This compact module can satisfy different experimental demands with adjustable detection efficiency and dark count. We have characterized the key parameters of the UCSPD system.

preprint2016arXiv

Measurement device independent quantum key distribution over 404 km optical fibre

Quantum key distribution (QKD) can provide unconditional secure communication between two distant parties. Although the significance of QKD is undisputed, its feasibility has been questioned because of certain limitations in the practical application of real-life QKD systems. It is a common belief the lack of perfect single-photon source and the existence of detection loss will handicap the feasibility of QKD by creating security loopholes and distance limitations. The measurement device independent QKD (MDIQKD) with decoy-state method removes the security threats from both the imperfect single-photon source and the detection loss. Lengthening the distance and improving the key rate of QKD with such a superior method is thus the central issue in the practical application of QKD. Here, we report the results of MDIQKD over 404 km of ultralow-loss optical fibre and 311 km of standard optical fibre by employing an optimized four-intensity decoy-state method. This record-breaking implementation of MDIQKD method not only provides a new distance record for both MDIQKD and all types of QKD systems, more significantly, it achieves a distance that the traditional BB84 QKD would not be able to achieve with the same detection devices even with ideal single-phone sources. For the first time, our work demonstrates that with the MDIQKD method, imperfect devices can achieve better results than what ideal sources could have achieved. This work represents a significant step towards proving and developing a feasible long-distance QKD.

preprint2016arXiv

Universal scaling of the electronic and the elastic energies of small polarons revealed by high-throughput first-principles calculations

Formation of self-trapped holes (STH) in a comprehensive list of scintillator materials, including halides and chalcogenides, are studied using an accurate and computationally efficient first-principles method, the polaron self-interaction correction (pSIC). The key characteristics of small hole polarons, including their geometries, energies and degree of localization, are found vastly different from halides to oxides to systems with open-shell cations. Nevertheless, we find a universal linear relation between the energy gap separating the bound hole level from the valence band maximum and the elastic energy associated with the lattice displacement field that accompanies the polaron.

preprint2015arXiv

Stability and Anomalous Compressibility of Bose Gases Near Resonance: The scale-dependent interactions and thermal effects

The stability of Bose gases near resonance has been a puzzling problem in recent years. In this Letter, we demonstrate that in addition to generating thermal pressure, thermal atoms enhance the repulsiveness of the scale-dependent interactions between condensed atoms due to renormalization effect and further stabilize the Bose gases. Consequently, we find that, as a precursor of instability, the compressibility develops an anomalous structure as a function of scattering length and is drastically reduced compared with the mean-field value. Furthermore, the density profile of a Bose gas in a harmonic trap is found to develop a flat top near the center. This is due to the anomalous behavior of compressibility and can be a potential smoking gun for probing such an effect.

preprint2015arXiv

Universal Scaling Properties of Cold Atom Scattering Dynamics in Confined Low Dimensional Geometries

Intermediate energy scale physics plays a very important role in non-equilibrium dynamics of quasi-low dimensional cold atom systems. In this article we obtain the universal scaling relations for the generalized reflection coefficient, i.e., the fraction of atoms scattered out of the initial state, at intermediate energies scales. These intermediate energies are larger than the trap frequency, but necessarily smaller than the effective range of the inter-atomic potential. For harmonically confined one and two dimensional geometries, whenever the energy of the system is commensurate with a transverse energy level, it is shown that the system becomes non-interacting. For energies close to a transverse energy level, the reflection coefficient and scattering dynamics take on universal scaling forms, only depending on the difference between the energy of the particles and the transverse energy level. In this article, the universal power law behaviors of these scattering observables are obtained.

preprint2014arXiv

Correlated spontaneous symmetry breaking induced by zero-point fluctuations in a quantum mixture

We propose a form of spontaneous symmetry breaking driven by zero-point quantum fluctuations. To be specific, we consider the low-energy dynamics of a mixture of two species of spin-$1$ Bose gases. It is demonstrated that the quantum fluctuations lift a degeneracy regarding the relative orientations of the spin directors of the two species, and result in correlation or locking between these macroscopic variables. This locking persists in the presence of the trapping potential and weak magnetic fields, allowing, in principle, an experimental probe of this correlated spontaneous symmetry breaking, as a macroscopic manifestation of zero-point quantum fluctuations.

preprint2014arXiv

Experimental Passive Decoy-State Quantum Key Distribution

The decoy-state method is widely used in practical quantum key distribution systems to replace ideal single photon sources with realistic light sources by varying intensities. Instead of active modulation, the passive decoy-state method employs built-in decoy states in a parametric down-conversion photon source, which can decrease the side channel information leakage in decoy state preparation and hence increase the security. By employing low dark count up-conversion single photon detectors, we have experimentally demonstrated the passive decoy-state method over a 50-km-long optical fiber and have obtained a key rate of about 100 bit/s. Our result suggests that the passive decoy-state source is a practical candidate for future quantum communication implementation.

preprint2014arXiv

Lattice anharmonicity and thermal conductivity from compressive sensing of first-principles calculations

First-principles prediction of lattice thermal conductivity $κ_L$ of strongly anharmonic crystals is a long-standing challenge in solid state physics. Making use of recent advances in information science, we propose a systematic and rigorous approach to this problem, compressive sensing lattice dynamics (CSLD). Compressive sensing is used to select the physically important terms in the lattice dynamics model and determine their values in one shot. Non-intuitively, high accuracy is achieved when the model is trained on first-principles forces in {\it quasi-random\/} atomic configurations. The method is demonstrated for Si, NaCl, and Cu$_{12}$Sb$_4$S$_{13}$, an earth-abundant thermoelectric with strong phonon-phonon interactions that limit the room-temperature $κ_L$ to values near the amorphous limit.

preprint2014arXiv

Non-Grotthuss Proton Diffusion Mechanism in Tungsten Oxide Dihydrate from First-Principles Calculations

Fast proton conduction mechanism is of key importance for achieving high performance in fuel cell membranes, batteries, supercapacitors, and electrochromic materials. Enhanced proton diffusion is often observed in hydrated materials where it is thought to occur via the famous Grotthuss mechanism through pathways formed by structural water. Using first-principles density-functional theory calculations, we demonstrate that proton diffusion in tungsten oxide dihydrate (WO$_{3}$.2H$_{2}$O), a known good proton conductor, takes place within the layers of corner-sharing WO$_{6}$ octahedra without direct involvement of structural water. The calculated proton migration barrier in WO$_{3}$.2H$_{2}$O (0.42 eV) is in good agreement with the experimental value inferred from the temperature dependence of conductivity (0.36 eV). The preferred proton diffusion path in WO$_{3}$.2H$_{2}$O is essentially the same as in $γ$-WO$_{3}$, and we find an activation energy of 0.35 eV for the latter, which agrees well with the experimental values. In contrast to the small intercalation voltages calculated for WO$_{3}$ and WO$_{3}$.2H$_{2}$O, we find that proton absorption in the monohydrate WO$_{3}$.H$_{2}$O is energetically highly favorable, corresponding to voltages in excess of 1 eV in the dilute limit. However, strong proton-proton repulsion limits the equilibrium H content at zero voltage. We find a fast one-dimensional diffusion channel in WO$_{3}$.H$_{2}$O with an activation energy of only 0.07 eV at dilute proton concentrations, but much higher barriers are expected at near-equilibrium concentrations due to strong repulsive interactions with other protons. Our results illustrate that low proton diffusion barriers and low insertion voltages both contribute to fast proton transport in bulk WO$_{3}$.2H$_{2}$O and $γ$-WO$_{3}$.

preprint2014arXiv

Quantum N-Boson States and Quantized Motion of Solitonic Droplets: Universal Scaling Properties in Low Dimensions

In this article, we illustrate the scaling properties of a family of solutions for N attractive bosonic atoms in the limit of large $N$. These solutions represent the quantized dynamics of solitonic degrees of freedom in atomic droplets. In dimensions lower than two, or $d=2-ε$, we demonstrate that the number of isotropic droplet states scales as $N^{3/2}/ε^{1/2}$, and for $ε=0$, or $d=2$, scales as ${N^2}$. The ground state energies scale as $N^{2 / ε+ 1}$ in $d=2-ε$, and when $d=2$, scale as an exponential function of N. We obtain the universal energy spectra and the generalized Tjon relation; their scaling properties are uniquely determined by the asymptotic freedom of quantum bosonic fields at short distances, a distinct feature in low dimensions. We also investigate the effect of quantum loop corrections that arise from various virtual processes and show that the resultant lifetime for a wide range of excited states scales as $N^{ε/2}E^{1-ε/2}$.

preprint2014arXiv

Universal Bose Gases Near Resonance: A Rigorous Solution

We obtain a rigorous solution of universal Bose gases near resonance and offer an answer to one of the long-standing challenges of quantum gases at large scattering lengths, where the standard dilute theory breaks down. The solution was obtained by using an $ε$ expansion near four spatial dimension. In dimension $d = 4 - ε$, the chemical potential of Bose gases near resonances is shown to approach the universal value $ε^{(2/(4-ε))} ε_F \sqrt{2/3} (1 + 0.474 ε- i 1.217 ε+ ...)$, where $ε_F$ is the Fermi energy defined for a Fermi gas of density $n$, and the condensation fraction is equal to $2/3 (1 + 0.0877 ε+ ...)$. We also discuss the implications on ultra-cold gases in physical dimensions.

preprint2013arXiv

A complicated Duffing oscillator in the surface-electrode ion trap

The oscillation coupling and different nonlinear effects are observed in a single trapped $^{40}Ca^{+}$ ion confined in our home-built surface-electrode trap (SET). The coupling and the nonlinearity are originated from the high-order multipole potentials due to different layouts and the fabrication asymmetry of the SET. We solve a complicated Duffing equation with coupled oscillation terms by the multiple scale method, which fits the experimental values very well. Our investigation in the SET helps for exploring nonlinearity using currently available techniques and for suppressing instability of qubits in quantum information processing with trapped ions.

preprint2013arXiv

Cluster expansion made easy with Bayesian compressive sensing

Long-standing challenges in cluster expansion (CE) construction include choosing how to truncate the expansion and which crystal structures to use for training. Compressive sensing (CS), which is emerging as a powerful tool for model construction in physics, provides a mathematically rigorous framework for addressing these challenges. A recently-developed Bayesian implementation of CS (BCS) provides a parameterless framework, a vast speed up over current CE construction techniques, and error estimates on model coefficients. Here, we demonstrate the use of BCS to build cluster expansion models for several binary alloy systems. The speed of the method and the accuracy of the resulting fits are shown to be far superior than state-of-the-art evolutionary methods for all alloy systems shown. When combined with high throughput first-principles frameworks, the implications of BCS are that hundreds of lattice models can be automatically constructed, paving the way to high throughput thermodynamic modeling of alloys.

preprint2013arXiv

Entanglement-based quantum key distribution with biased basis choice via free space

We report a free-space entanglement-based quantum key distribution experiment, implementing the biased basis protocol between two sites which are 15.3 km apart. Photon pairs from a polarization-entangled source are distributed through two 7.8-km free-space optical links. An optimal bias 20:80 between the X and Z basis is used. A post-processing scheme with finite-key analysis is applied to extract the final secure key. After three-hour continuous operation at night, a 4293-bit secure key is obtained, with a final key rate of 0.124 bit per raw key bit which increases the final key rate by 14.8% comparing to the standard BB84 case. Our results experimentally demonstrate that the efficient BB84 protocol, which increases key generation efficiency by biasing Alice and Bob's basis choices, is potentially useful for the ground-satellite quantum communication.

preprint2013arXiv

Quantum teleportation and entanglement distribution over 100-kilometre free-space channels

A long standing goal for quantum communication is to transfer a quantum state over arbitrary distances. Free-space quantum communication provides a promising solution towards this challenging goal. Here, through a 97-km free space channel, we demonstrate long distance quantum teleportation over a 35-53 dB loss one-link channel, and entanglement distribution over a 66-85 dB high-loss two-link channel. We achieve an average fidelity of {80.4(9)}% for teleporting six distinct initial states and observe the violation of the Clauser-Horne-Shimony-Holt inequality after distributing entanglement. Besides being of fundamental interest, our result represents a significant step towards a global quantum network. Moreover, the high-frequency and high-accuracy acquiring, pointing and tracking technique developed in our experiment provides an essential tool for future satellite-based quantum communication.

preprint2012arXiv

Bose Gases Near Resonance: renormalized interactions in a condensate

We study the interplay between few- and many-body physics in Bose gases near resonance. The effect of condensates on the two-body running coupling constant is investigated via imposing a boundary condition on a self-consistent renormalization flow equation. Bose gases are found to become nearly fermionized when the chemical potential as a function of scattering lengths reaches a maximum and the atomic condensates lose meta-stability. The maximum and accompanied insta- bility are illustrated as a precursor of the sign change of g_2, the renormalized two-body interaction between condensed atoms from effectively repulsive to effectively attractive when approaching res- onance even though the scattering length is still positive. This occurs when dimers, under the influence of condensates, emerge at zero energy in the atomic gases at a finite positive scattering length.

preprint2012arXiv

Compressive sensing as a new paradigm for model building

The widely-accepted intuition that the important properties of solids are determined by a few key variables underpins many methods in physics. Though this reductionist paradigm is applicable in many physical problems, its utility can be limited because the intuition for identifying the key variables often does not exist or is difficult to develop. Machine learning algorithms (genetic programming, neural networks, Bayesian methods, etc.) attempt to eliminate the a priori need for such intuition but often do so with increased computational burden and human time. A recently-developed technique in the field of signal processing, compressive sensing (CS), provides a simple, general, and efficient way of finding the key descriptive variables. CS is a new paradigm for model building-we show that its models are just as robust as those built by current state-of-the-art approaches, but can be constructed at a fraction of the computational cost and user effort.

preprint2012arXiv

Nature of 3D Bose Gases near Resonance

In this paper, we explore the nature of three-dimensional Bose gases at large positive scattering lengths via resummation of dominating processes involving a minimum number of virtual atoms. We focus on the energetics of the nearly fermionized Bose gases beyond the usual dilute limit. We also find that an onset instability sets in at a critical scattering length, beyond which the near-resonance Bose gases become strongly coupled to molecules and lose the metastability. Near the point of instability, the chemical potential reaches a maximum, and the effect of the three-body forces can be estimated to be around a few percent.

preprint2012arXiv

Self-consistent density functional calculations of the crystal field levels in lanthanide and actinide dioxides

Using a recently developed method combining a nonspherical self-interaction corrected LDA+$U$ scheme and an on-site multi-body Hamiltonian [Phys.\ Rev.\ B 83, 085106 (2011)], we calculate the crystal field parameters and crystal field (CF) excitation levels of $f$-element dioxides in the fluorite structure with $f^{n}$ electronic configurations, including $n=1$ (PaO$_{2}$, PrO$_{2}$), $n=2$ (UO$_{2}$), $n=3$ (NpO$_{2}$), and $n=4$ (PuO$_{2}$). It is shown that good agreement with experimental data (within approximately 10 to 20 meV) can be obtained in all cases. The properties of the multi-electron CF ground states are analyzed.

preprint2012arXiv

Two-dimensional Bose gases near resonance: universal three-body effects

We report in this Letter the results of our investigation of 2D Bose gases beyond the dilute limit emphasizing the role played by three-body scattering events. We demonstrate that a competition between three-body attractive interactions and two-body repulsive forces results in the chemical potential of 2D Bose gases to exhibit a maximum at a critical scattering length beyond which these quantum gases possess a negative compressibility. For larger scattering lengths, the increasingly prominent role played by three-body attractive interactions leads to an onset instability at a second critical value. The three-body effects studied here are universal, fully characterized by the effective 2D scattering length $a_{2D}$ (or the size of the 2D bound states) and are, in comparison to the 3D case, independent of three-body ultraviolet physics. We find, within our approach, the ratios of the contribution to the chemical potential due to three-body interactions to the one due to two-body to be 0.27 near the maximum of the chemical potential and 0.73 in the vicinity of the onset instability.

preprint2011arXiv

Anomalous Dimers in Quantum Mixtures near Broad Resonances: Pauli Blocking, Fermi Surface Dynamics and Implications

We study the energetics and dispersion of anomalous dimers that are induced by the Pauli blocking effect in a quantum Fermi gas of majority atoms near interspecies resonances. Unlike in vacuum, we find that both the sign and magnitude of the dimer masses are tunable via Feshbach resonances. We also investigate the effects of particle-hole fluctuations on the dispersion of dimers and demonstrate that the particle-hole fluctuations near a Fermi surface (with Fermi momentum $\hbar k_F$) generally reduce the effective two-body interactions and the binding energy of dimers. Furthermore, in the limit of light minority atoms the particle-hole fluctuations disfavor the formation of dimers with a total momentum $\hbar k_F$, because near $\hbar k_F$ the modes where the dominating particle-hole fluctuations appear are the softest. Our calculation suggests that near broad interspecies resonances when the minority-majority mass ratio $m_B/m_F$ is smaller than a critical value (estimated to be 0.136), dimers in a finite-momentum channel are energetically favored over dimers in the zero-momentum channel. We apply our theory to quantum gases of $^{6}$Li$^{40}$K, $^{6}$Li$^{87}$Rb, $^{40}$K$^{87}$Rb and $^{6}$Li$^{23}$Na near broad interspecies resonances, and discuss the limitations of our calculations and implications.

preprint2011arXiv

Crystal field and magnetic structure of UO$_{2}$

The properties of UO$_{2}$ result from rich $f$-electron physics, including electronic Coulomb interactions, spin-orbit and crystal field effects, as well as inter-ionic multipolar coupling. We present a comprehensive theoretical study of the electronic structure of UO$_{2}$ using a combined application of self-consistent DFT+$U$ calculations and a model Hamiltonian. The $Γ_{5}$ ground state of U$^{4+}$ and the energies of crystal field excitations $Γ_{5} \rightarrow Γ_{3,4,1}$ are reproduced in very good agreement with experiment. We also investigate competing non-collinear magnetic structures and confirm 3-k as the T=0 K ground state magnetic structure of UO$_2$.

preprint2011arXiv

Magnetic Catalysis and Quantum Hall Ferromagnetism in Weakly Coupled Graphene

We study the realization in a model of graphene of the phenomenon whereby the tendency of gauge-field mediated interactions to break chiral symmetry spontaneously is greatly enhanced in an external magnetic field. We prove that, in the weak coupling limit, and where the electron-electron interaction satisfies certain mild conditions, the ground state of charge neutral graphene in an external magnetic field is a quantum Hall ferromagnet which spontaneously breaks the emergent U(4) symmetry to U(2)XU(2). We argue that, due to a residual CP symmetry, the quantum Hall ferromagnet order parameter is given exactly by the leading order in perturbation theory. On the other hand, the chiral condensate which is the order parameter for chiral symmetry breaking generically obtains contributions at all orders. We compute the leading correction to the chiral condensate. We argue that the ensuing fermion spectrum resembles that of massive fermions with a vanishing U(4)-valued chemical potential. We discuss the realization of parity and charge conjugation symmetries and argue that, in the context of our model, the charge neutral quantum Hall state in graphene is a bulk insulator, with vanishing longitudinal conductivity due to a charge gap and Hall conductivity vanishing due to a residual discrete particle-hole symmetry.

preprint2011arXiv

Pauli Blocking Effect on Efimov States Near Feshbach Resonance

In this Letter we study the effect of Pauli blocking on the Efimov states in a quantum Fermi gas and illustrate that the universal Efimov potential is altered at large distances. We obtain the universal spectrum flow of Efimov trimers when the Fermi density is varied and further consider the effect of scattering of trimers by the Fermi sea. We argue that the universal flow is robust against fluctuating particle-hole pairs that result in an infrared catastrophe in impurity problems.

preprint2010arXiv

Experimental Quantum Error-Free Transmission

Error-free transmission (EFT) of quantum information is a crucial ingredient in quantum communication network. To overcome the unavoidable decoherence in noisy channel, to date, many efforts have focused on faithfully transmitting one state by consuming large numbers of synchronized ancillary states. However, huge demands of quantum resources are hard to meet with current technology, thus restrict practical applications. Here we propose and demonstrate an economical method of reliably transmitting quantum information. An arbitrary unknown quantum state is converted into time bins deterministically in terms of its own polarization using a modified Franson interferometer. Any arisen noise in channel will induce an associated error to the reference frame of the time bins, which can be utilized to reject errors and recover the initial state. By virtue of state-independent feature, our method can be applied to entanglement distribution. After passing through 0.8 km randomly twisted optical fiber, the entanglement still survives and is verified. Our approach significantly simplifies the implementation of quantum EFT and enables a general quantum state even entanglement to be protected by feedback, thus can be used as a basic building block in practical long-distance quantum communication network.

preprint2010arXiv

Fermi-Bose Mixtures Near Broad Interspecies Feshbach Resonances

In this Letter we have studied dressed bound states in Fermi-Bose mixtures near broad interspecies resonance, and implications on many-body correlations. We present the evidence for a first order phase transition between a mixture of Fermi gas and condensate, and a fully paired mixture where extended fermionic molecules occupy a single pairing channel instead of forming a molecular Fermi surface. We have further investigated the effect of Fermi surface dynamics, pair fluctuations and discussed the validity of our results.

preprint2010arXiv

First-principles determined charge and orbital interactions in Fe$_3$O$_4$

The interactions between charge and orbitally ordered $d$-electrons are important in many transition metal oxides. We propose an effective energy model for such interactions, parameterized with DFT+U calculations, so that energy contributions of both electronic and lattice origin can be simultaneously accounted for. The model is applied to the low-temperature phase of magnetite, for which we propose a new ground state structure. The effective interactions on the B-lattice of Fe$_3$O$_4$ can be interpreted in terms of electrostatics and short-range Kugel-Khomskii exchange coupling. The frustration between optimal charge and orbital orderings leads to a complex energy landscape whereby the supercell for the charge ordering, orbital ordering and ionic displacements can all be different.

preprint2010arXiv

Resonance Scattering in Optical Lattices and Molecules: Interband versus Intraband Effects

We study the low-energy two-body scattering in optical lattices with all higher-band effects included in an effective potential, using a renormalization group approach. As the potential depth reaches a certain value, a resonance of low energy scattering occurs even when the negative s-wave scattering length $(a_s)$ is much shorter than the lattice constant. These resonances can be mainly driven either by interband or intraband effects or by both, depending on the magnitude of $a_s$. Furthermore the low-energy scattering matrix in optical lattices has a much stronger energy-dependence than that in free space. We also investigate the momentum distribution for molecules when released from optical lattices.

preprint2009arXiv

Obtaining correct orbital ground states in $f$ electron systems using a nonspherical self-interaction corrected LDA+$U$ method

The electronic structure of lanthanide and actinide compounds is often characterized by orbital ordering of localized $f$-electrons. Density-functional theory (DFT) studies of such systems using the currently available LDA+$U$ method are plagued by significant orbital-dependent self-interaction, leading to erroneous orbital ground states. An alternative scheme that modifies the exchange, not Hartree, energy is proposed as a remedy. We show that our LDA+$U$ approach reproduces the expected degeneracy of $f^1$ and $f^2$ states in free ions and the correct ground states in solid PrO$_2$. We expect our method to be useful in studying compounds of $f$- and heavy-$d$ elements.

preprint2008arXiv

Domain walls in gapped graphene

The electronic properties of a particular class of domain walls in gapped graphene are investigated. We show that they can support mid-gap states which are localized in the vicinity of the domain wall and propagate along its length. With a finite density of domain walls, these states can alter the electronic properties of gapped graphene significantly. If the mid-gap band is partially filled,the domain wall can behave like a one-dimensional metal embedded in a semi-conductor, and could potentially be used as a single-channel quantum wire.

preprint2007arXiv

Quantum fluctuation-induced uniaxial and biaxial spin nematics

It is shown that zero point quantum fluctuations (ZPQFs) completely lift the accidental continuous degeneracy that is found in mean field analysis of quantum spin nematic phases of hyperfine spin 2 cold atoms. The result is two distinct ground states which have higher symmetries: a uniaxial spin nematic and a biaxial spin nematic with dihedral symmetry ${Dih}_4$. There is a novel first order quantum phase transition between the two phases as atomic scattering lengths are varied. We find that the ground state of $^{87}Rb$ atoms should be a uniaxial spin nematic. We note that the energy barrier between the phases could be observable in dynamical experiments.

preprint2006arXiv

Configurational electronic entropy and the phase diagram of mixed-valence oxides: the case of Li$_x$FePO$_4$

We demonstrate that configurational electronic entropy, previously neglected, in {\it ab initio} thermodynamics of materials can qualitatively modify the finite-temperature phase stability of mixed-valence oxides. While transformations from low-T ordered or immiscible states are almost always driven by configurational disorder (i.e. random occupation of lattice sites by multiple species), in FePO$_4$--LiFePO$_4$ the formation of a solid solution is almost entirely driven by electronic, rather than ionic configurational entropy. We argue that such an electronic entropic mechanism may be relevant to most other mixed-valence systems.

preprint2005arXiv

Coarse-graining protein energetics in sequence variables

We show that cluster expansions (CE), previously used to model solid-state materials with binary or ternary configurational disorder, can be extended to the protein design problem. We present a generalized CE framework, in which properties such as energy can be unambiguously expanded in the amino-acid sequence space. The CE coarse grains over nonsequence degrees of freedom (e.g., side-chain conformations) and thereby simplifies the problem of designing proteins, or predicting the compatibility of a sequence with a given structure, by many orders of magnitude. The CE is physically transparent, and can be evaluated through linear regression on the energies of training sequences. We show, as example, that good prediction accuracy is obtained with up to pairwise interactions for a coiled-coil backbone, and that triplet interactions are important in the energetics of a more globular zinc-finger backbone.

preprint2005arXiv

Emergent Geometric Hamiltonian and Insulator-Superfluid Phase Transitions

I argue that certain bosonic insulator-superfluid phase transitions as an interaction constant varies are driven by emergent geometric properties of insulating states. The {\em renormalized} chemical potential and distribution of disordered bosons define the geometric aspect of an effective low energy Hamiltonian which I employ to study various resonating states and quantum phase transitions. In a mean field approximation, I also demonstrate that the quantum phase transitions are in the universality class of a percolation problem.

preprint2005arXiv

The electronic structure and band gap of LiFePO4 and LiMnPO4

Materials with the olivine LixMPO4 structure form an important new class of materials for rechargeable Li batteries. There is significant interest in their electronic properties because of the importance of electronic conductivity in batteries for high rate applications. The density of states of LixMPO4 (x = 0, 1 and M = Fe, Mn) has been determined with the ab initio GGA+U method, appropriate for these correlated electron systems. Computed results are compared with the optical gap of LiFePO4, as measured using UV-Vis-NIR diffuse reflectance spectroscopy. The results obtained from experiment (3.8-4.0 eV) and GGA+U computations (3.7 eV) are in very good agreement. However, standard GGA, without the same level of treatment of electron correlation, is shown to make large errors in predicting the electronic structure. It is argued that olivines are likely to be polaronic conductors with extrinsically determined carrier levels and that their electronic conductivity is therefore not simply related to the band gap.

preprint2005arXiv

The Li intercalation potential of LiMPO4 and LiMSiO4 olivines with M = Fe, Mn, Co, Ni

The Li intercalation potential of LiMPO4 and LiMSiO4 compounds with M = Fe, Mn, Co, and Ni is computed with the GGA+U method. It is found that this approach is considerably more accurate than standard LDA or GGA methods. The calculated potentials for LiFePO4, LiMnPO4 and LiCoOPO4 agree to within 0.1 V with experimental results. The LiNiPO4 potential is predicted to be above 5 V. The potentials of the silicate materials are all found to be rather high, but LiFeSiO4 and LiCoSiO4 have negligible volume change upon Li extraction.

preprint2004arXiv

Topological spin pumps I

We have established a semiclassical kinetic approach for various spin correlated pumping phenomena incorporating spin rotation in wave functions into transport equations. We employ this technique to study topological pumps and illustrate spin pumping in a few models where various spin configurations or topological motors drive adiabatic pumps. In the Rashba model we find that a topological spin pump is driven by a meron with positive one half skyrmion charge, the size of which can be controlled by external gates or Zeeman fields. In the Dresselhaus model on the other hand, electron spins are pumped out by a negative meron. We examine effects of Zeeman fields on topological spin pumping and responses of fermi seas in various pumps. The phenomena of topological pumping are attributed to topological Stern-Gerlach splitting and occur in a transverse direction along which charge pumping currents either vanish or are negligible. The transport equations established here might also be applied for the studies of anomalous Hall effect and spin Hall effect as demonstrated in one of appendices.

preprint2003arXiv

Spin Singlet Mott States and Evidence For Spin Singlet Quantum Condensates of Spin-One Bosons in Lattices

We have investigated spin singlet Mott states of spin-one bosons with antiferromagnetic interactions. These spin singlet states do not break rotational symmetry and exhibit remarkably different macroscopic properties compared with nematic Mott states of spin-one bosons. We demonstrate that the dynamics of spin singlet Mott states is fully characterized by even- and odd-class quantum dimer models. The difference between spin singlet Mott states for even and odd numbers of atoms per site can be attributed to a selection rule in the low energy sectors of on-site Hilbert spaces; alternatively, it can also be attributed to an effect of Berry's phases on bosonic Mott states. We also discuss evidence for spin singlet quantum condensate of spin-one atoms. Our main finding is that in a projected spin singlet Hilbert space, the low energy physics of spin-one bosons is fully characterized by a Bose-Hubbard model of interacting spinless bosons carrying charges of Ising gauge fields; the other major finding is spin-charge separation in some one-dimensional Mott states. We propose charge-e spin singlet superfluid for an odd number of atoms per lattice site and charge-2e spin singlet superfluid for an even number of atoms per lattice site in one-dimensional lattices. All discussions in this article are limited to integer numbers of bosons per site.