Superconductivity-induced transverse plasma mode and phonon anomaly in the cc-axis response of the bilayer compound RbCa2_2Fe4_4As4_4F2_2

preprint2020arXivOpen access

Abstract

With infrared spectroscopy we studied the out-of-plane (cc-axis) response of the iron arsenide superconductor ACa2_2Fe4_4As4_4F2_2 (A = Rb,Cs) which has a bilayer structure similar to the high TcT_c cuprates YBa2_2Cu3_3O7_7 (YBCO) and Bi2_2Sr2_2CaCu2_2O8_8 (Bi2212). In analogy to the cuprates, we observe a superconductivity-induced transverse plasma mode (tPM) and a phonon anomaly that are both signatures of local electric field effects that arise from a large difference between the local conductivities in the intra- and inter-bilayer regions. Using a multilayer model developed for the cuprates, we obtain a good description of the cc-axis response and derive the local conductivities at T≃TcT \simeq T_c of σ1bl(ω→0)≃σ_1^{\mathrm{bl}}(ω\rightarrow 0) \simeq 1\,000 Ω−1cm−1Ω^{-1}\mathrm{cm}^{-1} and σ1int(ω→0)≃σ_1^{\mathrm{int}}(ω\rightarrow 0) \simeq 15 Ω−1cm−1Ω^{-1}\mathrm{cm}^{-1}, respectively, that are similar to the ones previously found in underdoped YBCO. Different from the cuprates, we find no evidence of a normal state pseudogap in terms of a partial suppression of the low-energy electronic states that sets in already well above TcT_c. There is also no clear sign of an onset of precursor superconducting pairing correlations well above Tc≃T_c \simeq 30~K. This highlights that the pseudogap and the precursor superconducting pairing well above TcT_c are unique features of the cuprates with their strong electronic correlations and, for example, not just the result of a strongly anisotropic electronic response due to the layered crystal structure.

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