Abstract

We use nuclear magnetic resonance (NMR), high-resolution x-ray and neutron scattering to study structural and magnetic phase transitions in phosphorus-doped BaFe2_2(As1−x_{1-x}Px_x)2_2. Previous transport, NMR, specific heat, and magnetic penetration depth measurements have provided compelling evidence for the presence of a quantum critical point (QCP) near optimal superconductivity at x=0.3x=0.3. However, we show that the tetragonal-to-orthorhombic structural (TsT_s) and paramagnetic to antiferromagnetic (AF, TNT_N) transitions in BaFe2_2(As1−x_{1-x}Px_x)2_2 are always coupled and approach to TN≈Ts≥TcT_N\approx T_s \ge T_c (≈29\approx 29 K) for x=0.29x=0.29 before vanishing abruptly for x≥0.3x\ge 0.3. These results suggest that AF order in BaFe2_2(As1−x_{1-x}Px_x)2_2 disappears in a weakly first order fashion near optimal superconductivity, much like the electron-doped iron pnictides with an avoided QCP.

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