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Magnetic Structure and Ordering of Multiferroic Hexagonal LuFeO3

We report on the magnetic structure and ordering of hexagonal LuFeO3 films grown by molecular-beam epitaxy (MBE) on YSZ (111) and Al2O3 (0001) substrates. Using a set of complementary probes including neutron diffraction, we find that the system magnetically orders into a ferromagnetically-canted antiferromagnetic state via a single transition between 138-155 K, while a paraelectric to ferroelectric transition occurs above 1000 K. The symmetry of the magnetic structure in the ferroelectric state implies that this material is a strong candidate for linear magnetoelectric coupling and control of the ferromagnetic moment directly by an electric field.

preprint2014arXivOpen access
Steven M. DisselerJulie A. BorchersCharles M. BrooksJulia A. MundyJarrett A. MoyerD. A. HillsberryE. L. ThiesD. A. TenneJohn HeronJames D. ClarksonGregory M. StiehlPeter SchifferDavid A. MullerDarrell G. SchlomWilliam D. Ratcliff
cond-mat.str-elcond-mat.mtrl-sci
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Steven M. DisselerJulie A. BorchersCharles M. BrooksJulia A. MundyJarrett A. MoyerD. A. HillsberryE. L. ThiesD. A. TenneJohn HeronJames D. ClarksonGregory M. StiehlPeter SchifferDavid A. MullerDarrell G. SchlomWilliam D. Ratcliff

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