Abstract

Isomers with three- and five-nucleon-hole configurations have been established in 203^{203}Tl. These include newly identified levels with a three-nucleon structure: {\it I}π^{π} = (15/2−^{-}) with {\it T}1/2_{1/2} = 7.9(5) ns, and {\it I}π^{π} = (35/2−^{-}) with {\it T}1/2_{1/2} = 4.0(5) ns. In addition, five-quasiparticle states: {\it I}π^{π} = (39/2−^{-}) with {\it T}1/2_{1/2} = 1.9(2) ns, and {\it I}π^{π} = (49/2+^{+}) with {\it T}1/2_{1/2} = 3.4(4) ns have also been established. The previously determined long-lived decay [{\it T}1/2_{1/2} = 6.6(3) μμs from this work] is associated with isomerism of the {\it I}π^{π} = (29/2+^{+}) state. Levels above this long-lived isomer have been identified through a delayed-prompt coincidence measurement. Five-nucleon-hole states with excitation energies {\it E}x_{x} ≈\approx 7 MeV have been established as well as possible octupole excitations of the 208^{208}Pb core built on these levels. The level scheme of 203^{203}Tl is extended up to {\it E}x_{x} ≈\approx 11 MeV with the inclusion of 25 new transitions. Empirical and shell-model calculations have been performed to aid in the description of the observed states which are found to be predominantly of intrinsic character.

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