Abstract
Isomers with three- and five-nucleon-hole configurations have been established in Tl. These include newly identified levels with a three-nucleon structure: {\it I} = (15/2) with {\it T} = 7.9(5) ns, and {\it I} = (35/2) with {\it T} = 4.0(5) ns. In addition, five-quasiparticle states: {\it I} = (39/2) with {\it T} = 1.9(2) ns, and {\it I} = (49/2) with {\it T} = 3.4(4) ns have also been established. The previously determined long-lived decay [{\it T} = 6.6(3) s from this work] is associated with isomerism of the {\it I} = (29/2) state. Levels above this long-lived isomer have been identified through a delayed-prompt coincidence measurement. Five-nucleon-hole states with excitation energies {\it E} 7 MeV have been established as well as possible octupole excitations of the Pb core built on these levels. The level scheme of Tl is extended up to {\it E} 11 MeV with the inclusion of 25 new transitions. Empirical and shell-model calculations have been performed to aid in the description of the observed states which are found to be predominantly of intrinsic character.
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