Fractional spin textures in the frustrated magnet SrCr9p_{9p}Ga12−9p_{12-9p}O19_{19}

preprint2010arXivOpen access

Abstract

We consider the archetypal frustrated antiferromagnet SrCr9p_{9p}Ga12−9p_{12-9p}O19_{19} in its well-known spin-liquid state, and demonstrate that a Cr3+^{3+} spin S=3/2S=3/2 ion in direct proximity to a pair of vacancies (in disordered p<1p<1 samples) is cloaked by a spatially extended spin texture that encodes the correlations of the parent spin-liquid. In this spin-liquid regime, the combined object has a magnetic response identical to a classical spin of length S/2=3/4S/2 = 3/4, which dominates over the small intrinsic susceptibility of the pure system. This fractional-spin texture leaves an unmistakable imprint on the measured 71^{71}Ga nuclear magnetic resonance (NMR) lineshapes, which we compute using Monte-Carlo simulations and compare with experimental data.

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