Ferromagnetic quantum phase transition in Sr1−x_{1-x}Cax_xRuO3_3 thin films

preprint2009arXivOpen access

Abstract

The ferromagnetic quantum phase transition in the perovskite ruthenate Sr1−x_{1-x}Cax_xRuO3_3 is studied by low-temperature magnetization and electrical resistivity measurements on thin films. The films were grown epitaxially on SrTiO3_3 substrates using metalorganic aerosol deposition and characterized by X-ray diffraction and room temperature scanning tunneling microscopy. High residual resistivity ratios of 29 and 16 for x=0x=0 and x=1x=1, respectively, prove the high quality of the investigated samples. We observe a continuous suppression of the ferromagnetic Curie temperature from TC=160T_C=160 K at x=0x=0 towards TC→0T_C\to 0 at xc≈0.8x_c\approx 0.8. The analysis of the electrical resistivity between 2 and 10 K reveals T2T^2 and T3/2T^{3/2} behavior at x≤0.6x\leq 0.6 and x≥0.7x\geq 0.7, respectively. For undoped CaRuO3_3, the measurement has been extended down to 60 mK, revealing a crossover to T2T^2 behavior around 2 K, which suggests a Fermi-liquid ground state in this system.

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