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Evidence for SrHo2O4 and SrDy2O4 as model J1-J2 zig-zag chain materials

Neutron diffraction and inelastic spectroscopy is used to characterize the magnetic Hamiltonian of SrHo2O4 and SrDy2O4. Through a detailed computation of the crystal-field levels we find site- dependent anisotropic single-ion magnetism in both materials and diffraction measurements show the presence of strong one-dimensional spin correlations. Our measurements indicate that competing interactions of the zig-zag chain, combined with frustrated interchain interactions, play a crucial role in stabilizing spin-liquid type correlations in this series.

preprint2014arXivOpen access
Amy PooleVladimir PomjakushinAnne-Christine UldryBernhard DelleyBobby PrevostAlexandre Desilets-BenoitAndrea D BianchiRobert I BewleyBritt R HansenThomasz KlimczukRobert J CavaMichel Kenzelmann
cond-mat.str-elcond-mat.mtrl-sci
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Open access12 authors2 topics
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Amy PooleVladimir PomjakushinAnne-Christine UldryBernhard DelleyBobby PrevostAlexandre Desilets-BenoitAndrea D BianchiRobert I BewleyBritt R HansenThomasz KlimczukRobert J CavaMichel Kenzelmann

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