Abstract

We describe why Ising spin chains with competing interactions in SrHo2O4\rm SrHo_2O_4 segregate into ordered and disordered ensembles at low temperatures (TT). Using elastic neutron scattering, magnetization, and specific heat measurements, the two distinct spin chains are inferred to have Néel (↑↓↑↓\uparrow\downarrow\uparrow\downarrow) and double-Néel (↑↑↓↓\uparrow\uparrow\downarrow\downarrow) ground states respectively. Below TN=0.68(2)T_\mathrm{N}=0.68(2)~K, the Néel chains develop three dimensional (3D) long range order (LRO), which arrests further thermal equilibration of the double-Néel chains so they remain in a disordered incommensurate state for TT below TS=0.52(2)T_\mathrm{S}= 0.52(2)~K. SrHo2O4\rm SrHo_2O_4 distills an important feature of incommensurate low dimensional magnetism: kinetically trapped topological defects in a quasi−d−-d-dimensional spin system can preclude order in d+1d+1 dimensions.

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