Abstract

The neutron-rich nucleus 144^{144}Ba (t1/2t_{1/2}=11.5 s) is expected to exhibit some of the strongest octupole correlations among nuclei with mass numbers AA less than 200. Until now, indirect evidence for such strong correlations has been inferred from observations such as enhanced E1E1 transitions and interleaving positive- and negative-parity levels in the ground-state band. In this experiment, the octupole strength was measured directly by sub-barrier, multi-step Coulomb excitation of a post-accelerated 650-MeV 144^{144}Ba beam on a 1.0-mg/cm2^2 208^{208}Pb target. The measured value of the matrix element, ⟨31−∥M(E3)∥01+⟩=0.65(−23+17)\langle 3_1^- \| \mathcal{M}(E3) \| 0_1^+ \rangle=0.65(^{+17}_{-23}) eeb3/2^{3/2}, corresponds to a reduced B(E3)B(E3) transition probability of 48(−34+25^{+25}_{-34}) W.u. This result represents an unambiguous determination of the octupole collectivity, is larger than any available theoretical prediction, and is consistent with octupole deformation.

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