Abstract

CeRuPO is a rare example of a ferromagnetic (FM) Kondo-lattice system. External pressure suppresses the ordering temperature to zero at about pc≈3p_c\approx3 GPa. Our ac-susceptibility and electrical-resistivity investigations evidence that the type of magnetic ordering changes from FM to antiferromagnetic (AFM) at about p∗≈0.87p^*\approx0.87 GPa. Studies in applied magnetic fields suggest that ferromagnetic and antiferromagnetic correlations compete for the ground state at p>p∗p>p^*, but finally the AFM correlations win. The change in the magnetic ground-state properties is closely related to the pressure evolution of the crystalline-electric-field level (CEF) scheme and the magnetic Ruderman-Kittel-Kasuya-Yosida (RKKY) exchange interaction. The Néel temperature disappears abruptly in a first-order-like fashion at pcp_c, hinting at the absence of a quantum critical point. This is consistent with the low-temperature transport properties exhibiting Landau-Fermi-liquid (LFL) behavior in the whole investigated pressure range up to 7.5 GPa.

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