Abstract

The atomic masses of 55^{55}Sc, 56,58^{56,58}Ti, and 56−59^{56-59}V have been determined using the high-precision multi-reflection time-of-flight technique. The radioisotopes have been produced at RIKEN's RIBF facility and delivered to the novel designed gas cell and multi-reflection system (ZD MRTOF), which has been recently commissioned downstream of the ZeroDegree spectrometer following the BigRIPS separator. For 56,58^{56,58}Ti and 56−59^{56-59}V the mass uncertainties have been reduced down to the order of 10 keV10\,\mathrm{keV}, shedding new light on the N=34N=34 shell effect in Ti and V isotopes by the first high-precision mass measurements of the critical species 58^{58}Ti and 59^{59}V. With the new precision achieved, we reveal the non-existence of the N=34N=34 empirical two-neutron shell gaps for Ti and V, and the enhanced energy gap above the occupied νp3/2νp_{3/2} orbit is identified as a feature unique to Ca. We perform new Monte Carlo shell model calculations including the νd5/2νd_{5/2} and νg9/2νg_{9/2} orbits and compare the results with conventional shell model calculations, which exclude the νg9/2νg_{9/2} and the νd5/2νd_{5/2} orbits. The comparison indicates that the shell gap reduction in Ti is related to a partial occupation of the higher orbitals for the outer two valence neutrons at N=34N=34.

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