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ZhiMing Li

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Published work

21 published item(s)

preprint2026arXiv

Higher-Order Equilibrium Tracking for EM-Compressible Online Estimation

We study online estimation in latent-variable models by recasting the problem as tracking a moving empirical equilibrium. Standard online EM and stochastic approximation analyses primarily study convergence toward the population parameter and typically do not isolate the empirical batch optimum from the online tracking error at finite horizon. Our framework decomposes the online estimate into the frozen batch equilibrium at the current running statistic and a tracking lag that captures the algorithm's delay behind this moving target. We prove a batch-to-online transfer theorem: provided $\lVert e_T \rVert_{L^{2}} = o(T^{-1/2})$, the online estimator inherits the batch central limit theorem and the sharp first-order risk constant. Our key observation is that the empirical optimum evolves on a smooth equilibrium manifold indexed by the running statistic. An $m$-th order equilibrium-jet predictor combined with an order-$ν$ frozen corrector yields localized tracking rates $O(T^{-ν(m+1)})$. We formalize EM-compressibility and EM-jet$^R$-compressibility as the structural conditions that make the equilibrium response and the Newton corrector evaluable from a retained streaming statistic. The theory is instantiated in latent linear Gaussian covariance estimation, where the first-order scheme operates on a compressed $d \times d$ statistic with explicit finite-sample risk envelopes and a certified restart rule.

preprint2022arXiv

A mechanically strong and ductile soft magnet with extremely low coercivity

Soft magnetic materials (SMMs) serve in electrical applications and sustainable energy supply, allowing magnetic flux variation in response to changes in applied magnetic field, at low energy loss1. The electrification of transport, households and manufacturing leads to an increase in energy consumption due to hysteresis losses2. Therefore, minimizing coercivity, which scales these losses, is crucial3. Yet, meeting this target alone is not enough: SMMs in electrical engines must withstand severe mechanical loads, i.e., the alloys need high strength and ductility4. This is a fundamental design challenge, as most methods that enhance strength introduce stress fields that can pin magnetic domains, thus increasing coercivity and hysteretic losses5. Here, we introduce an approach to overcome this dilemma. We have designed a Fe-Co-Ni-Ta-Al multicomponent alloy with ferromagnetic matrix and paramagnetic coherent nanoparticles (~91 nm size, ~55% volume fraction). They impede dislocation motion, enhancing strength and ductility. Their small size, low coherency and small magnetostatic energy create an interaction volume below the magnetic domain wall width, leading to minimal domain wall pinning, thus maintaining the soft magnetic properties. The alloy has a tensile strength of 1336 MPa at 54% tensile elongation, extremely low coercivity of 78 A/m (<1 Oe), moderate saturation magnetization of 100 Am2/kg, and high electrical resistivity of 103 μΩ u Ohm cm.

preprint2022arXiv

GALOIS: Boosting Deep Reinforcement Learning via Generalizable Logic Synthesis

Despite achieving superior performance in human-level control problems, unlike humans, deep reinforcement learning (DRL) lacks high-order intelligence (e.g., logic deduction and reuse), thus it behaves ineffectively than humans regarding learning and generalization in complex problems. Previous works attempt to directly synthesize a white-box logic program as the DRL policy, manifesting logic-driven behaviors. However, most synthesis methods are built on imperative or declarative programming, and each has a distinct limitation, respectively. The former ignores the cause-effect logic during synthesis, resulting in low generalizability across tasks. The latter is strictly proof-based, thus failing to synthesize programs with complex hierarchical logic. In this paper, we combine the above two paradigms together and propose a novel Generalizable Logic Synthesis (GALOIS) framework to synthesize hierarchical and strict cause-effect logic programs. GALOIS leverages the program sketch and defines a new sketch-based hybrid program language for guiding the synthesis. Based on that, GALOIS proposes a sketch-based program synthesis method to automatically generate white-box programs with generalizable and interpretable cause-effect logic. Extensive evaluations on various decision-making tasks with complex logic demonstrate the superiority of GALOIS over mainstream baselines regarding the asymptotic performance, generalizability, and great knowledge reusability across different environments.

preprint2022arXiv

Investigations into the characteristics and influences of nonequilibrium evolution

In order to estimate qualitatively the influence of nonequilibrium evolution in relativistic heavy ion collisions, we use the three dimensional Ising model with Metropolis algorithm to study the evolution from nonequilibrium to equilibrium on the phase boundary. The evolution of order parameter approaches its equilibrium value exponentially, the same as that given by Langevin equation. The average relaxation time is defined which is demonstrated to well represent the relaxation time in dynamical equations. It is shown that the average relaxation time at critical temperature diverges as the zth power of system size. The third and the fourth cumulants of order parameter during the nonequilibrium evolution could be either positive or negative, depending on the observation time, consistent with dynamical models at T > Tc. It is found that the nonequilibrium evolution at T > Tc lasts very short, and the influence is weaker than that at T < Tc. Those qualitative features are instructive to determine experimentally the critical point and the phase boundary of QCD.

preprint2022arXiv

Machine learning-enabled high-entropy alloy discovery

High-entropy alloys are solid solutions of multiple principal elements, capable of reaching composition and feature regimes inaccessible for dilute materials. Discovering those with valuable properties, however, relies on serendipity, as thermodynamic alloy design rules alone often fail in high-dimensional composition spaces. Here, we propose an active-learning strategy to accelerate the design of novel high-entropy Invar alloys in a practically infinite compositional space, based on very sparse data. Our approach works as a closed-loop, integrating machine learning with density-functional theory, thermodynamic calculations, and experiments. After processing and characterizing 17 new alloys (out of millions of possible compositions), we identified 2 high-entropy Invar alloys with extremely low thermal expansion coefficients around 2*10-6 K-1 at 300 K. Our study thus opens a new pathway for the fast and automated discovery of high-entropy alloys with optimal thermal, magnetic and electrical properties.

preprint2022arXiv

Overview of intermittency analysis in heavy-ion collisions

In this paper, a search for power-law fluctuations with fractality and intermittency analysis to explore the QCD phase diagram and the critical point is summarized. Experimental data on self-similar correlations and fluctuations with respect to the size of phase space volume in various high energy heavy-ion collisions are presented, with special emphasis on background subtraction and efficiency correction of the measurement. Phenomenological modelling and theoretical work on the subject are discussed. Finally, we highlight possible directions for future research.

preprint2021arXiv

Intermittency analysis in relativistic heavy-ion collisions

Local density fluctuations near the QCD critical point can be probed by an intermittency analysis of power-law behavior on scaled factorial moments in relativistic heavy-ion collisions. We study the second-order scaled factorial moment in Au + Au collisions at $\sqrt{s_\mathrm{NN}}$ = 7.7-200 GeV from the UrQMD model. Since the background subtraction and efficiency correction are two important aspects in this measurement, we propose a cumulative variable method to remove background contribution and a cell-by-cell method for efficiency correction in the intermittency analysis.

preprint2021arXiv

Radiation-tolerant high-entropy alloys via interstitial-solute-induced chemical heterogeneities

High-entropy alloys (HEAs) composed of multiple principal elements have been shown to offer improved radiation resistance over their elemental or dilute-solution counterparts. Using NiCoFeCrMn HEA as a model, here we introduce carbon and nitrogen interstitial alloying elements to impart chemical heterogeneities in the form of the local chemical order (LCO) and associated compositional variations. Density functional theory simulations predict chemical short-range order (CSRO) (nearest neighbors and the next couple of atomic shells) surrounding C and N, due to the chemical affinity of C with (Co, Fe) and N with (Cr, Mn). Atomic-resolution chemical mapping of the elemental distribution confirms marked compositional variations well beyond statistical fluctuations. Ni+ irradiation experiments at elevated temperatures demonstrate a remarkable reduction in void swelling by at least one order of magnitude compared to the base HEA without C and N alloying. The underlying mechanism is that the interstitial-solute-induced chemical heterogeneities roughen the lattice as well as the energy landscape, impeding the movements of, and constraining the path lanes for, the normally fast-moving self-interstitials and their clusters. The irradiation-produced interstitials and vacancies therefore recombine more readily, delaying void formation. Our findings thus open a promising avenue towards highly radiation-tolerant alloys.

preprint2020arXiv

Entropies of commuting transformations on Hilbert spaces

By establishing Multiplicative Ergodic Theorem for commutative transformations on a separable infinite dimensional Hilbert space, in this paper, we investigate Pesin's entropy formula and SRB measures of a finitely generated random transformations on such space via its commuting generators. Moreover, as an application, we give a formula of Friedland's entropy for certain $C^{2}$ $\mathbb{N}^2$-actions.

preprint2020arXiv

Probing QCD critical fluctuations from intermittency analysis in relativistic heavy-ion collisions

It is shown that intermittency, a self-similar correlation with respect to the size of the phase space volume, is sensitive to critical density fluctuations of baryon numbers in a system belonging to the three-dimensional (3D) Ising universality class. The relation between intermittency index and relative baryon density fluctuation is obtained. We thus suggest that measuring the intermittency in relativistic heavy-ion collisions could be used as a good probe of density fluctuations associated with the QCD critical phenomena. From recent preliminary results on neutron density fluctuations in central Au + Au collisions at $\sqrt{s_{NN}}$ = 7.7, 11.5, 19.6, 27, 39, 62.4 and 200 GeV at RHIC/STAR, the collision energy dependence of intermittency index is extracted and shows a non-monotonic behavior with a peak at around 20 - 27 GeV, indicating that the strength of intermittency becomes the largest in this energy region. The transport UrQMD model without implementing critical physics cannot describe the observed behavior.

preprint2020arXiv

Subtracting non-critical fluctuations in higher cumulants of conserved charges

Using the sample produced by the AMPT default model, we construct a corresponding mixed sample by the method of mixed events. The mixed sample provides an effective estimation for non-critical fluctuations which are caused by global and systematic effects. The dynamical cumulants of conserved charges are defined as the cumulants of the original sample minus the cumulants of the mixed sample. It is demonstrated that dynamical cumulants are subtracted statistical fluctuations, and centrality bin width or detection efficiency independent, in consistent with formulae corrected cumulants. Therefore, dynamical cumulants are helpful in obtaining critical fluctuations at the RHIC BES.

preprint2016arXiv

Measurement of the ratio of the sixth order to the second order cumulant of net-proton multiplicity distributions in relativistic heavy-ion collisions

We investigate the measurement of the sixth order cumulant and its ratio to the second order cumulant ($C_6/C_2$) in relativistic heavy-ion collisions. The influence of statistics and different methods of centrality bin width correction on $C_6/C_2$ of net-proton multiplicity distributions is demonstrated. There is no satisfactory method to extract $C_6/C_2$ with the current statistics recorded at lower energies by STAR at RHIC. With statistics comparable to the expected statistics at the planned future RHIC Beam Energy Scan II (BES II), no energy dependence of $C_6/C_2$ is observed in central collisions using the UrQMD model. We find if the transition signal is as strong as predicted by the PQM model, then it is hopefully observed at the upcoming RHIC BES II.

preprint2016arXiv

Multiscale persistent functions for biomolecular structure characterization

In this paper, we introduce multiscale persistent functions for biomolecular structure characterization. The essential idea is to combine our multiscale rigidity functions with persistent homology analysis, so as to construct a series of multiscale persistent functions, particularly multiscale persistent entropies, for structure characterization. To clarify the fundamental idea of our method, the multiscale persistent entropy model is discussed in great detail. Mathematically, unlike the previous persistent entropy or topological entropy, a special resolution parameter is incorporated into our model. Various scales can be achieved by tuning its value. Physically, our multiscale persistent entropy can be used in conformation entropy evaluation. More specifically, it is found that our method incorporates in it a natural classification scheme. This is achieved through a density filtration of a multiscale rigidity function built from bond and/or dihedral angle distributions. To further validate our model, a systematical comparison with the traditional entropy evaluation model is done. It is found that our model is able to preserve the intrinsic topological features of biomolecular data much better than traditional approaches, particularly for resolutions in the mediate range. Moreover, our method can be successfully used in protein classification. For a test database with around nine hundred proteins, a clear separation between all-alpha and all-beta proteins can be achieved, using only the dihedral and pseudo-bond angle information. Finally, a special protein structure index (PSI) is proposed, for the first time, to describe the "regularity" of protein structures. Essentially, PSI can be used to describe the "regularity" information in any systems.

preprint2016arXiv

On the sensitivities dependence in non-autonomous dynamical systems

For discrete autonomous dynamical systems (ADS) $(X, d, f)$, it was found that in the three conditions defining Devaney chaos, topological transitivity and dense periodic points together imply sensitive dependence on initial condition(Banks, Brooks, Cairns, Davis and Stacey, 1992). In this paper, the result of Banks et al. is generalized to a class of the non-autonomous dynamical systems (NADS) $(X,f_{1,\infty})$. Also, by the studying of NADS over their iterated systems $(X,f_{1,\infty}^{[k]})$, we know that for two sensitive NADS, the one which preserve sensitive in its any times iterated systems is more sensitive than the one not. In this case, several sufficient conditions ensuring two kinds of sensitivities are preserved under the arbitrary number of iterations of certain NADS are given.

preprint2015arXiv

Influence of statistics on the measured moments of conserved quantities in relativistic heavy ion collisions

We study statistics dependence of the probability distributions and the means of measured moments of conserved quantities, respectively. The required statistics of all interested moments and their products are estimated based on a simple simulation. We also explain why the measured moments are underestimated when the statistics are insufficient.With the statistics at RHIC/BES, the second and third order moments can be reliably obtained based on the method of Centrality bin width correction (CBWC), which can not be applied for the fourth order moments at low energy. With planning statistics at RHIC/BES II, and improved CBWC method, $κσ^2$ in a finer centrality bin scale should be measurable. This will help us to understand the current observation of energy and centrality dependence of high-order moments.

preprint2014arXiv

Influences of statistics and initial size fluctuation on high-order cumulants of conserved quantities in relativistic heavy ion collisions

By the generator of the UrQMD model, event statistics for the products of kurtosis ($κ$) and variance ($σ^2$) of net-proton and net-charge multiplicity distributions are carefully studied. It is shown that the statistics at RHIC/BES below $\sqrt {s_{NN}} < 19.6$ GeV are not sufficient for using the method of Centrality Bin Width Correction (CBWC). Corresponding results are systematically underestimated. A way to improve the CBWC method is proposed. It can remove the statistics dependence of the data and reduce the initial size fluctuation as well.

preprint2013arXiv

Co-compact entropy and its variational principle for non-compact spaces

The purpose of this paper is to generalize the variational principle, which states that the topological entropy is equal to the supremum of the measure theoretical entropies and also the minimum of the metric theoretical entropies, to non-compact dynamical systems by utilizing the co-compact entropy. The equivalence between positive co-compact entropy and the existence of p-horseshoes over the real line is also proved. This implies a system over real line with positive co-compact entropy contains a compact invariant subset.

preprint2013arXiv

Influence of initial size on higher cumulant ratios of net-proton number fluctuations

With the help of AMPT default model, we study the influence of initial size (centrality of collisions) on higher cumulant ratios of net-proton distributions. If the centrality is presented by impact parameter, there is a strong centrality dependent, in particular, in those peripheral collisions. This dependence is slightly reduced if the centrality is presented by number of participant, or charged multiplicity. However, the dynamical ratios are almost centrality independent. So the centrality dependence of dynamical ratios at RHIC beam energy scan are presented.

preprint2013arXiv

Statistical and dynamical fluctuations of Binder ratios in heavy ion collisions

Higher moments of net-proton Binder ratio, which is suggested to be a good experimental measurement to locate the QCD critical point, is measured in relativistic heavy ion collisions. We firstly estimate the effect of statistical fluctuations of the third and forth order Binder ratios. Then the dynamical Binder ratio is proposed and investigated in both transport and statistical models. The energy dependence of dynamical Binder ratios with different system sizes at RHIC beam scan energies are presented and discussed.

preprint2013arXiv

Statistical and dynamical parts of the cumulants of conserved charges in relativistic heavy ion collisions

The Poisson-liked statistical fluctuations, which are caused by the finite number of produced particles, are firstly estimated for the cumulants of conserved charges, i.e., the cumulants of net-baryon, net-electric charge, and net-strangeness. They turn out to be the same as those baselines derived from Hadron Resonance Gas (HRG) model. The energy and centrality dependence of net-proton cumulants at the Relativistic Heavy-Ion Collider (RHIC) are demonstrated to be mainly caused by statistical fluctuations. Subtracting the statistical fluctuations, the dynamical kurtosis of net- and total-proton from two versions of the AMPT model and the UrQMD model at current RHIC beam energies are presented. It is found that the observed sign change in the kurtosis of net-proton can not be reproduced by these three transport models. There is no significant difference between net- and total-proton kurtosis in model calculations, in contrary to the data at RHIC.