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Shaojun Xu

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Published work

4 published item(s)

preprint2026arXiv

Mind Dreamer: Untethering Imagination via Active Latent Intervention on Latent Manifolds

Model-Based Reinforcement Learning (MBRL) leverages latent imagination for sample efficiency, yet remains constrained by Historical Tethering: imagination is typically initialized from observed states. This creates a learning asymmetry, where the world model's manifold discovery outpaces the policy's sparse-reward optimization. We propose Mind Dreamer (MD), a framework that operationalizes Active Latent Intervention (ALI) to transcend Markovian continuity. MD reformulates discovery as the minimization of a global Relay Manifold Expected Free Energy (R-EFE); by sampling initial states from a learned generator $s_0 \sim p_{gen}(\cdot)$ rather than the historical buffer, MD utilizes an adversarial generator to synthesize non-continuous latent jumps to epistemic blind spots that are physically plausible yet cognitively challenging. To resolve the credit assignment paradox across these spatial ruptures, we derive the Relay Value Function (RVF) and Relay Uncertainty Function (RUF). These potentials treat synthesized anchors as counterfactual intermediary states, propagating pragmatic and epistemic value through a principled Bellman-style formulation. Notably, we prove that uncertainty propagation across discontinuities necessitates a quadratic discount $γ^2$, establishing a formal epistemic horizon. Theoretically, MD approximates a variance-minimizing importance sampler that expands the manifold's spectral gap, reducing the hitting time to critical bottleneck states. Empirically, MD achieves a 1.67$\times$ average speedup over DreamerV3 on DeepMind Control Suite, reaching 8.8$\times$ in sparse-reward tasks.

preprint2022arXiv

Metalated Porous-Organic-Polymer Renders Mustard-Gas Simulant Harmless: Core Planarity Matters

The presence of open active metal sites in Metal-Organic Frameworks (MOFs) exhibit higher catalytic activity. However, rational accomplishment of MOFs in heterogeneous catalysis is limited due to coordination bonds. Recently balanced characteristic feature with combination of both the covalent bonds (structural stability) and open metal sites (single site catalysis) introduced an entirely organic alternative architecture named as Metalated Porous-Organic-Polymers (M-POPs). In this contribution, we demonstrate successful construction of two Fe-POPs (Fe-Tt-POP & Fe-Rb-POP) by ternary copolymerization approach for catalytic oxidative decontamination of different sulfur-based mustard gas simulants. Fe-Tt-POP exhibited superior catalytic performance for oxidation of the thioanisole (TA) studied in terms of conversion (99% after 13 h) in comparison with Fe-Rb-POP (43% after 13h). The remarkable difference in the mechanistic pathways towards catalytic performance for oxidation of TA was investigated by in situ operando Diffuse Reflectance Infrared Fourier Transform Spectroscopy (DRIFTS) analysis, complemented by Density Functional Theory (DFT) computational study.

preprint2014arXiv

Numerical operator method for the real time dynamics of strongly-correlated quantum impurity systems far from equilibrium

We develop a method for studying the real time dynamics of Heisenberg operators in strongly-interacting nonequilibrium quantum impurity models. Our method is applicable to a wide range of interaction strengths and to bias voltages beyond the linear response regime, works at zero temperature, and overcomes the finite-size limitations faced by other numerical methods. We compare our method with quantum Monte Carlo simulations at a strong interaction strength, at which no analytical method is applicable up to now. We find a very good coincidence of the results at high bias voltage, and in the short time period at low bias voltage. We discuss the possible reason of the deviation in the long time period at low bias voltage. We also find a good coincidence of our results with the perturbation results at weak interactions.

preprint2013arXiv

Randomly Fluctuating Potential Controlled Multistable Resonant Tunneling Current through a Quantum Dot

We study the transport through a quantum dot subject to a randomly fluctuating potential, generated by a sequence of pulses in the gate voltage with the help of the autoregressive model. We find that the tunneling current is multistable when the fluctuating potential with a finite correlation time is applied before the non-equilibrium steady state is built up. The non-equilibrium stationary current is heavily dependent on the history of the fluctuating potential during the transient period if the potential has a finite correlation time. Furthermore, the averaged current over the path of the fluctuating potential is a function of its strength and correlation time. Our work therefore provides a robust theoretical proposal for the controlling of the non-equilibrium stationary current through a quantum dot in a randomly fluctuating potential.