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Denys I. Bondar

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Published work

27 published item(s)

preprint2026arXiv

Geometric Kolmogorov--Arnold Network (GeoKAN)

We introduce Geometric Kolmogorov--Arnold Networks (GeoKANs), a family of geometry-aware KAN-type models in which approximation is carried out in learned, geometry-adapted coordinates rather than in fixed Euclidean input coordinates. GeoKAN achieves this by learning a diagonal Riemannian metric that warps the input before basis expansion and feature mixing. The learned metric provides a geometric inductive bias through local length scaling and volume distortion, and in physics-informed settings it also affects the differential structure seen by the model. Within this framework, we develop three main variants, namely GeoKAN-NNMetric, GeoKAN-$γ$, and LM-KAN. For LM-KAN, we further consider three basis-specific versions, LM-KAN-RBF, LM-KAN-Wav, and LM-KAN-Fourier. These variants allow us to study geometry-aware KAN models both as general function approximators and as surrogates in physics-informed learning. By stretching regions with rapid variation and compressing smoother regions, GeoKAN reallocates representational resolution in a task-dependent manner, allowing the model to place capacity where it is most needed. As a result, GeoKAN is well suited to sharp, stiff, localized, and strongly non-uniform regimes arising in scientific machine learning and differential-equation problems.

preprint2026arXiv

Hybrid non-degenerate parametric amplifier for a microwave cavity mode and an NV ensemble

We introduce an implementation of a non-degenerate parametric amplifier in which the signal and idler modes, respectively, a microwave mode and an ensemble of spins (e.g., nitrogen-vacancy centers in diamond), are operated in their linear regime. This paramp, which amplifies signals in both parts at room and cryogenic temperatures, can be used to generate both the two-mode and single-mode squeezing of either system. It requires merely modulating the frequency of the spin ensemble at the sum of the cavity and spin frequencies (providing the classical pump) with the two systems sufficiently detuned. This effect is remarkable given that modulating a spin ensemble by itself produces neither amplification nor squeezing, unlike modulating an oscillator, and that an off-resonant perturbative analysis would suggest that modulating the spin ensemble merely parametrically drives the cavity mode. With typical cavity parameters including a cavity quality factor~$Q=10^4$, and a 1 GHz modulation amplitude, the microwave signal can be amplified by approximately $18~\mbox{dB}$ in $1.7~\mbox{$μ$s}$, with a resonant bandwidth of about $0.5~\mbox{MHz}$. At $10~\mbox{mK}$ with the same modulation amplitude and a cavity and spin $Q=5\times 10^4$ it generates approximately $5~\mbox{dB}$ of squeezing. We also examine the experimental requirements for implementation.

preprint2023arXiv

Coherent Control of Evanescent Waves via Beam Shaping

Evanescent waves are central to many technologies such as near-field imaging that beats the diffraction limit and plasmonic devices. Frustrated total internal reflection (FTIR) is an experimental method commonly used to study evanescent waves. In this paper, we shape the incident beam of the FTIR process with a Mach-Zehnder interferometer and measure light transmittance while varying the path length difference and interferometric visibility. Our results show that the transmittance varies with the path length difference and, thus, the intensity distribution of the shaped beam. Experiment and finite element method simulation produce results that agree. We also show, through simulations, that the transmittance can be controlled via other methods of beam shaping. Our work provides a proof-of-concept demonstration of the coherent control of the FTIR process, which could lead to advancements in numerous applications of evanescent waves and FTIR.

preprint2022arXiv

All-optical input-agnostic polarization transformer via experimental Kraus-map control

The polarization of light is utilized in many technologies throughout science and engineering. The ability to transform one state of polarization to another is a key enabling technology. Common polarization transformers are simple polarizers and polarization rotators. Simple polarizers change the intensity depending on the input state and can only output a fixed polarized state, while polarization rotators rotates the input Stokes vector in the 3D Stokes space. We experimentally demonstrate an all-optical input-agnostic polarization transformer (AI-APT), which transforms all input states of polarization to a particular state that can be polarized or partially polarized. The output state of polarization and intensity depends solely on setup parameters, and not on the input state, thereby the AI-APT functions differently from simple polarizers and polarization rotators. The AI-APT is completely passive, and thus can be used as a polarization controller or stabilizer for single photons and ultrafast pulses. To achieve this, we, for the first time, experimentally realize complete kinematic state controllability of an open single-qubit by Kraus maps put forth in [Wu et al. J. Phys. A 40, 5681 (2007)]. The AI-APT may open a new frontier of partially polarized ultrafast optics.

preprint2022arXiv

Optical Distinguishability of Mott Insulators in Time vs Frequency Domain

High Harmonic Generation (HHG) promises to provide insight into ultrafast dynamics and has been at the forefront of attosecond physics since its discovery. One class of materials that demonstrate HHG are Mott insulators whose electronic properties are of great interest given their strongly-correlated nature. Here, we use the paradigmatic representation of Mott insulators, the half-filled Fermi-Hubbard model, to investigate the potential of using HHG response to distinguish these materials. We develop an analytical argument based on the Magnus expansion approximation to evolution by the Schrodinger equation that indicates decreased distinguishability of Mott insulators as lattice spacing, $a$, and the strength of the driving field, $F_0$, increase relative to the frequency, $ω_0$. This argument is then bolstered through numerical simulations of different systems and subsequent comparison of their responses in both the time and frequency domain. Ultimately, we demonstrate reduced resolution of Mott insulators in both domains when the dimensionless parameter $g \equiv aF_0 / ω_0$ is large, though the time domain provides higher distinguishability. Conductors are exempted from these trends, becoming much more distinguishable in the frequency domain at high $g$.

preprint2022arXiv

Sequential optical response suppression for chemical mixture characterization

The characterization of mixtures of non-interacting, spectroscopically similar quantum components has important applications in chemistry, biology, and materials science. We introduce an approach based on quantum tracking control that allows for determining the relative concentrations of constituents in a quantum mixture, using a single pulse which enhances the distinguishability of components of the mixture and has a length that scales linearly with the number of mixture constituents. To illustrate the method, we consider two very distinct model systems: mixtures of diatomic molecules in the gas phase, as well as solid-state materials composed of a mixture of components. A set of numerical analyses are presented, showing strong performance in both settings.

preprint2021arXiv

Joint quantum-classical Hamilton variation principle in the phase space

We show that the dynamics of a closed quantum system obeys the Hamilton variation principle. Even though quantum particles lack well-defined trajectories, their evolution in the Husimi representation can be treated as a flow of multidimensional probability fluid in the phase space. By introducing the classical counterpart of the Husimi representation in a close analogy to the Koopman-von Neumann theory, one can largely unify the formulations of classical and quantum dynamics. We prove that the motions of elementary parcels of both classical and quantum Husimi fluid obey the Hamilton variational principle, and the differences between associated action functionals stem from the differences between classical and quantum pure states. The Husimi action functionals are not unique and defined up to the Skodje flux gauge fixing [R. T. Skodje et al. Phys. Rev. A 40, 2894 (1989)]. We demonstrate that the gauge choice can dramatically alter flux trajectories. Applications of the presented theory for constructing semiclassical approximations and hybrid classical-quantum theories are discussed.

preprint2020arXiv

Accurate Lindblad-Form Master Equation for Weakly Damped Quantum Systems Across All Regimes

Realistic models of quantum systems must include dissipative interactions with an environment. For weakly-damped systems the Lindblad-form Markovian master equation is invaluable for this task due to its tractability and efficiency. This equation only applies, however, when the frequencies of any subset of the system's transitions are either equal (degenerate), or their differences are much greater than the transitions' linewidths (far-detuned). Outside of these two regimes the only available efficient description has been the Bloch-Redfield (B-R) master equation, the efficacy of which has long been controversial due to its failure to guarantee the positivity of the density matrix. The ability to efficiently simulate weakly-damped systems across all regimes is becoming increasingly important, especially in the area of quantum technologies. Here we solve this long-standing problem. We discover that a condition on the slope of the spectral density is sufficient to derive a Lindblad form master equation that is accurate for all regimes. We further show that this condition is necessary for weakly-damped systems to be described by the B-R equation or indeed any Markovian master equation. We thus obtain a replacement for the B-R equation over its entire domain of applicability that is no less accurate, simpler in structure, completely positive, allows simulation by efficient quantum trajectory methods, and unifies the previous Lindblad master equations. We also show via exact simulations that the new master equation can describe systems in which slowly-varying transition frequencies cross each other during the evolution. System identification tools, developed in systems engineering, play an important role in our analysis. We expect these tools to prove useful in other areas of physics involving complex systems.

preprint2020arXiv

Amplification of quadratic Hamiltonians

Speeding up the dynamics of a quantum system is of paramount importance for quantum technologies. However, in finite dimensions and without full knowledge of the details of the system, it is easily shown to be impossible. In contrast we show that continuous variable systems described by a certain class of quadratic Hamiltonians can be sped up without such detailed knowledge. We call the resultant procedure Hamiltonian amplification (HA). The HA method relies on the application of local squeezing operations allowing for amplifying even unknown or noisy couplings and frequencies by acting on individual modes. Furthermore, we show how to combine HA with dynamical decoupling to achieve amplified Hamiltonians that are free from environmental noise. Finally, we illustrate a significant reduction in gate times of cavity resonator qubits as one potential use of HA.

preprint2020arXiv

Beating the House: Fast Simulation of Dissipative Quantum Systems with Ensemble Rank Truncation

We introduce a new technique for the simulation of dissipative quantum systems. This method is composed of an approximate decomposition of the Lindblad equation into a Kraus map, from which one can define an ensemble of wavefunctions. Using principal component analysis, this ensemble can be truncated to a manageable size without sacrificing numerical accuracy. We term this method \emph{Ensemble Rank Truncation} (ERT), and find that in the regime of weak coupling, this method is able to outperform existing wavefunction Monte-Carlo methods by an order of magnitude in both accuracy and speed. We also explore the possibility of combining ERT with approximate techniques for simulating large systems (such as Matrix Product States (MPS)), and show that in many cases this approach will be more efficient than directly expressing the density matrix in its MPS form. We expect the ERT technique to be of practical interest when simulating dissipative systems for quantum information, metrology and thermodynamics.

preprint2020arXiv

Driven Imposters: Controlling Expectations in Many-Body Systems

We present a framework to control and track the observables of a general solid state system driven by an incident laser field. The main result is a non-linear equation of motion for tracking an observable, together with a constraint on the size of expectations which may be reproduced via tracking. Among other applications, this model provides a potential route to the design of laser fields which cause photo-induced superconductivity in materials above their critical temperature. As a first test, the strategy is used to make the expectation value of the current conform to an arbitrary function under a range of model parameters. Additionally, using two reference spectra for materials in the conducting and insulating regimes respectively, the tracking algorithm is used to make each material mimic the optical spectrum of the other.

preprint2020arXiv

Quantum and semiclassical dynamics as fluid theories where gauge matters

The family of trajectories-based approximations employed in computational quantum physics and chemistry is very diverse. For instance, Bohmian and Heller's frozen Gaussian semiclassical trajectories seem to have nothing in common. Based on a hydrodynamic analogy to quantum mechanics, we furnish the unified gauge theory of all such models. In the light of this theory, currently known methods are just a tip of the iceberg, and there exists an infinite family of yet unexplored trajectory-based approaches. Specifically, we show that each definition for a semiclassical trajectory corresponds to a specific hydrodynamic analogy, where a quantum system is mapped to an effective probability fluid in the phase space. We derive the continuity equation for the effective fluid representing dynamics of an arbitrary open bosonic many-body system. We show that unlike in conventional fluid, the flux of the effective fluid is defined up to Skodje's gauge [R. T. Skodje et. al. Phys. Rev. A 40, 2894 (1989)]. We prove that the Wigner, Husimi and Bohmian representations of quantum mechanics are particular cases of our generic hydrodynamic analogy, and all the differences among them reduce to the gauge choice. Infinitely many gauges are possible, each leading to a distinct quantum hydrodynamic analogy and a definition for semiclassical trajectories. We propose a scheme for identifying practically useful gauges and apply it to improve a semiclassical initial value representation employed in quantum many-body simulations.

preprint2019arXiv

Controlling Arbitrary Observables in Correlated Many-body Systems

Here we present an expanded analysis of a model for the manipulation and control of observables in a strongly correlated, many-body system, which was first presented in [McCaul et al., eprint: arXiv:1911.05006]. A field-free, non-linear equation of motion for controlling the expectation value of an essentially arbitrary observable is derived, together with rigorous constraints that determine the limits of controllability. We show that these constraints arise from the physically reasonable assumptions that the system will undergo unitary time evolution, and has enough degrees of freedom for the electrons to be mobile. Furthermore, we give examples of multiple solutions to generating target observable trajectories when the constraints are violated. Ehrenfest theorems are used to further refine the model, and provide a check on the validity of numerical simulations. Finally, the experimental feasibility of implementing the control fields generated by this model is discussed.

preprint2016arXiv

Dirac open quantum system dynamics: formulations and simulations

We present an open system interaction formalism for the Dirac equation. Overcoming a complexity bottleneck of alternative formulations, our framework enables efficient numerical simulations (utilizing a typical desktop) of relativistic dynamics within the von Neumann density matrix and Wigner phase space descriptions. Employing these instruments, we gain important insights into the effect of quantum dephasing for relativistic systems in many branches of physics. In particular, the conditions for robustness of Majorana spinors against dephasing are established. Using the Klein paradox and tunneling as examples, we show that quantum dephasing does not suppress negative energy particle generation. Hence, the Klein dynamics is also robust to dephasing.

preprint2016arXiv

Efficient computations of quantum canonical Gibbs state in phase space

The Gibbs canonical state, as a maximum entropy density matrix, represents a quantum system in equilibrium with a thermostat. This state plays an essential role in thermodynamics and serves as the initial condition for nonequilibrium dynamical simulations. We solve a long standing problem for computing the Gibbs state Wigner function with nearly machine accuracy by solving the Bloch equation directly in the phase space. Furthermore, the algorithms are provided yielding high quality Wigner distributions for pure stationary states as well as for Thomas-Fermi and Bose-Einstein distributions. The developed numerical methods furnish a long-sought efficient computation framework for nonequilibrium quantum simulations directly in the Wigner representation.

preprint2016arXiv

Wigner-Lindblad equations for quantum friction

Dissipative forces are ubiquitous and thus constitute an essential part of realistic physical theories. However, quantization of dissipation has remained an open challenge for nearly a century. We construct a quantum counterpart of classical friction, a velocity-dependent force acting against the direction of motion. In particular, a translationary invariant Lindblad equation is derived satisfying the appropriate dynamical relations for the coordinate and momentum (i.e., the Ehrenfest equations). Numerical simulations establish that the model approximately equilibrates. These findings significantly advance a long search for a universally valid Lindblad model of quantum friction and open opportunities for exploring novel dissipation phenomena.

preprint2015arXiv

Efficient method to generate time evolution of the Wigner function for open quantum systems

The Wigner function is a useful tool for exploring the transition between quantum and classical dynamics, as well as the behavior of quantum chaotic systems. Evolving the Wigner function for open systems has proved challenging however; a variety of methods have been devised but suffer from being cumbersome and resource intensive. Here we present an efficient fast-Fourier method for evolving the Wigner function, that has a complexity of $O(N\log N)$ where $N$ is the size of the array storing the Wigner function. The efficiency, stability, and simplicity of this method allows us to simulate open system dynamics previously thought to be prohibitively expensive. As a demonstration we simulate the dynamics of both one-particle and two-particle systems under various environmental interactions. For a single particle we also compare the resulting evolution with that of the classical Fokker-Planck and Koopman-von Neumann equations, and show that the environmental interactions induce the quantum-to-classical transition as expected. In the case of two interacting particles we show that an environment interacting with one of the particles leads to the loss of coherence of the other.

preprint2015arXiv

Excess of positrons in cosmic rays: A Lindbladian model of quantum electrodynamics

The fraction of positrons and electrons in cosmic rays recently observed on the International Space Station unveiled an unexpected excess of the positrons, undermining the current foundations of cosmic rays sources. We provide a quantum electrodynamics phenomenological model explaining the observed data. This model incorporates electroproduction, in which cosmic ray electrons decelerating in the interstellar medium emit photons that turn into electron-positron pairs. These findings not only advance our knowledge of cosmic ray physics, but also pave the way for computationally efficient formulations of quantum electrodynamics, critically needed in physics and chemistry.

preprint2014arXiv

Non-classicality of positive relativistic Wigner function

In nonrelativistic quantum mechanics, Hudsons theorem states that a Gaussian wavefunction is the only pure state corresponding to a positive Wigner function (WF). We explicitly construct non Gaussian Dirac spinors with positive relativistic WF. These pure states are coherent superpositions of particles and antiparticles, while the existence of positive WF exclusive composed of particles is conjectured. These observations challenge a common belief that states with positive WF are classical or have classical analogues, and may open new venues in relativistic quantum information.

preprint2013arXiv

Conceptual inconsistencies in finite-dimensional quantum and classical mechanics

Utilizing operational dynamic modeling [Phys. Rev. Lett. 109, 190403 (2012); arXiv:1105.4014], we demonstrate that any finite-dimensional representation of quantum and classical dynamics violates the Ehrenfest theorems. Other peculiarities are also revealed, including the nonexistence of the free particle and ambiguity in defining potential forces. Non-Hermitian mechanics is shown to have the same problems. This work compromises a popular belief that finite-dimensional mechanics is a straightforward discretization of the corresponding infinite-dimensional formulation.

preprint2013arXiv

Operational Dynamic Modeling Transcending Quantum and Classical Mechanics

We introduce a general and systematic theoretical framework for Operational Dynamic Modeling (ODM) by combining a kinematic description of a model with the evolution of the dynamical average values. The kinematics includes the algebra of the observables and their defined averages. The evolution of the average values is drawn in the form of Ehrenfest-like theorems. We show that ODM is capable of encompassing wide ranging dynamics from classical non-relativistic mechanics to quantum field theory. The generality of ODM should provide a basis for formulating novel theories.

preprint2013arXiv

Wigner phase space distribution as a wave function

We demonstrate that the Wigner function of a pure quantum state is a wave function in a specially tuned Dirac bra-ket formalism and argue that the Wigner function is in fact a probability amplitude for the quantum particle to be at a certain point of the classical phase space. Additionally, we establish that in the classical limit, the Wigner function transforms into a classical Koopman-von Neumann wave function rather than into a classical probability distribution. Since probability amplitude need not be positive, our findings provide an alternative outlook on the Wigner function's negativity.

preprint2012arXiv

Relativistic Wigner function and consistent classical limit for spin 1/2 particles

The relativistic Wigner function for spin 1/2 particles is the subject of active research due to diverse applications. However, further progress is hindered by the fabulous complexity of the integro-differential equations of motion. We simplify these equations to partial differential equations of the Dirac type that are not only well suited for numerical computation, but also posses a well defined classical limit in a manifestly covariant form.

preprint2011arXiv

Quantum mechanics of a free particle from properties of the Dirac delta function

Based on the assumption that the probability density of finding a free particle is independent of position, we infer the form of the eigenfunction for the free particle, $\bra{x} p > = \exp(ipx/\hbar)/\sqrt{2π\hbar}$. The canonical commutation relation between the momentum and position operators and the Ehrenfest theorem in the free particle case are derived solely from differentiation of the delta function and the form of $\bra{x} p >$.

preprint2011arXiv

Shapes of leading tunnelling trajectories for single-electron molecular ionization

Based on the geometrical approach to tunnelling by P.D. Hislop and I.M. Sigal [Memoir. AMS 78, No. 399 (1989)], we introduce the concept of a leading tunnelling trajectory. It is then proven that leading tunnelling trajectories for single-active-electron models of molecular tunnelling ionization (i.e., theories where a molecular potential is modelled by a single-electron multi-centre potential) are linear in the case of short range interactions and "almost" linear in the case of long range interactions. The results are presented on both the formal and physically intuitive levels. Physical implications of the obtained results are discussed.

preprint2010arXiv

The reproduction of the dynamics of a quantum system by an ensemble of classical particles beyond de Broglie--Bohmian mechanics

It is shown that for any given quantum system evolving unitarily with the Hamiltonian, $\hat{H} = \hat{\bf p}^2/(2m) + U({\bf q})$, [bold letters denote $D$-dimensional ($D \geqslant 3$) vectors] and with a sufficiently smooth potential $U({\bf q})$, there exits a classical ensemble with the Hamilton function, $\mathrsfs{H} ({\bf p}, {\bf q}) = {\bf p}^2/(2m) + U^{(\infty)} ({\bf q})$, where the potential $U^{(\infty)}({\bf q})$ coincides with $U({\bf q})$ for almost all ${\bf q}$ (i.e., $U^{(\infty)}$ can be different from $U$ only on a measure zero set), such that the square modulus of the wave function in the coordinate (momentum) representation approximately equals the coordinate (momentum) distribution of the classical ensemble within an arbitrary given accuracy. Furthermore, the trajectories of this classical ensemble, generally speaking, need not coincide with the trajectories obtained from de Broglie--Bohmian mechanics. Consequences of this result are discussed.