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Paper detail

Universal whirling magnetic orders in non-Heisenberg Tsai-type quasicrystal approximants

Magnetic orders of non-Heisenberg Tsai-type 1/1 approximant crystals (ACs) in the Au-Ga-Dy system were studied through bulk magnetization, neutron diffraction, and inelastic neutron scattering techniques. The results uncovered noncoplanar, ferromagnetic (FM) and antiferromagnetic (AFM) spin configurations whirling along [111] crystallographic axis, which is analogous to those observed in the Tb- and Ho-contained counterparts. The crystal electric field excitations similar to those in the Tb-based counterpart are also observed indicating the strong Ising-like magnetic anisotropy. These comprehensive experiments and analyses have revealed the existence of a universal mechanism that stabilizes noncoplanar FM and AFM structures in non-Heisenberg Tsai-type ACs, independent of the rare-earth species (Tb, Dy, Ho); FM intra-cluster interactions and strong Ising-like anisotropy.

preprint2026arXivOpen access
Farid LabibKazuhiro NawaYusuke NambuHiroyuki TakakuraYoichi IkedaKazuhiko DeguchiMasato MatsuuraAsuka IshikawaRyoichi KajimotoKazuhiko IkeuchiTaku J. SatoRyuji Tamura
cond-mat.str-elcond-mat.mtrl-sciquant-ph
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Farid LabibKazuhiro NawaYusuke NambuHiroyuki TakakuraYoichi IkedaKazuhiko DeguchiMasato MatsuuraAsuka IshikawaRyoichi KajimotoKazuhiko IkeuchiTaku J. SatoRyuji Tamura

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