Ultrafast photoinduced phase separation dynamics in Pr(0.6)Ca(0.4)MnO(3) thin films

The time resolved Magnetooptical Kerr effect in the substrate-strain-induced insulating ferromagnetic phase in (Pr$_{0.6}$Ca$_{0.4}$)MnO$_3$ thin films on two different substrates was measured in a magnetic field up to 1.1T. The photoinduced Kerr rotation and ellipticity show remarkably different magnetic-field dependence. From the comparison of the magnetic field dependencies of the photoinduced and static Kerr rotation and ellipticity we conclude that a transient ferromagnetic metallic phase, embedded within the insulating ferromagnetic phase, is created upon the photoexcitation at low temperatures. A comparison of temporal dependence of the photoinduced Kerr signals with the photoinduced reflectivity indicates the change of the fractions of the phases takes place on a timescale of ten picoseconds independent of the substrate.

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