Two successive field-induced spin-flop transitions in single-crystalline CaCo2_{2}As2_{2}

preprint2012arXivOpen access

Abstract

CaCo2_{2}As2_{2}, a ThCr2_{2}Si2_{2}-structure compound, undergoes an antiferromagnetic transition at \emph{TN_{N}}=76K with the magnetic moments being aligned parallel to the \emph{c} axis. Electronic transport measurement reveals that the coupling between conducting carriers and magnetic order in CaCo2_{2}As2_{2} is much weaker comparing to the parent compounds of iron pnictide. Applying magnetic field along \emph{c} axis induces two successive spin-flop transitions in its magnetic state. The magnetization saturation behaviors with \emph{\textbf{H}∥\parallelc} and \emph{\textbf{H}∥\parallelab} at 10K indicate that the antiferromagnetic coupling along \emph{c} direction is very weak. The interlayer antiferromagntic coupling constant \emph{Jc_{c}} is estimated to be about 2 meV.

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