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Two-Spinon and Orbital Excitations of the Spin-Peierls System TiOCl

We combine high-resolution resonant inelastic x-ray scattering with cluster calculations utilizing a recently derived effective magnetic scattering operator to analyze the polarization, excitation energy, and momentum dependent excitation spectrum of the low-dimensional quantum magnet TiOCl in the range expected for orbital and magnetic excitations (0 - 2.5 eV). Ti 3d orbital excitations yield complete information on the temperature-dependent crystal-field splitting. In the spin-Peierls phase we observe a dispersive two-spinon excitation and estimate the inter- and intra-dimer magnetic exchange coupling from a comparison to cluster calculations.

preprint2011arXivOpen access
Sebastian GlawionJakoba HeidlerMaurits W. HaverkortLaurent C. DudaThorsten SchmittVladimir N. StrocovClaude MonneyKejin ZhouAndreas RuffMichael SingRalph Claessen
cond-mat.str-el
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Open access11 authors1 topic
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Sebastian GlawionJakoba HeidlerMaurits W. HaverkortLaurent C. DudaThorsten SchmittVladimir N. StrocovClaude MonneyKejin ZhouAndreas RuffMichael SingRalph Claessen

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