Abstract

Atomically precise epitaxial structures are unique systems for tunneling spectroscopy that minimize extrinsic effects of disorder. We present a systematic tunneling spectroscopy study, over a broad doping, temperature, and bias range, in epitaxial c-axis La2−x_{2-x}Srx_{x}CuO4_{4}/La2_{2}CuO4_{4}/La2−x_{2-x}Srx_{x}CuO4_{4} heterostructures. The behavior of these superconductor/insulator/superconductor (SIS) devices is unusual. Down to 20 mK there is complete suppression of c-axis Josephson critical current with a barrier of only 2 nm of La2_{2}CuO4_{4}, and the zero-bias conductance remains at 20-30% of the normal-state conductance, implying a substantial population of in-gap states. Tunneling spectra show greatly suppressed coherence peaks. As the temperature is raised, the superconducting gap fills in rather than closing at TcT_{c}. For all doping levels, the spectra show an inelastic tunneling feature at ∼\sim 80 meV, suppressed as TT exceeds TcT_{c}. These nominally simple epitaxial cuprate junctions deviate markedly from expectations based on the standard Bardeen-Cooper-Schrieffer (BCS) theory.

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