Theory of field-induced quantum phase transition in spin dimer system Ba3_3Cr2_2O8_8

preprint2014arXivOpen access

Abstract

Motivated by recent experiments on Ba3_3Cr2_2O8_8, we propose a theory describing low-temperature properties in magnetic field hh of dimer spin-12\frac12 systems on a stacked triangular lattice with spatially anisotropic exchange interactions. Considering the interdimer interaction as a perturbation we derive in the second order the elementary excitations (triplon) spectrum and the effective interaction between triplons at the quantum critical point h=hch=h_c separating the paramagnetic phase (h<hch<h_c) and a magnetically ordered one (hc<h<hsh_c<h<h_s, where hsh_s is the saturation field). Expressions are derived for hc(T)h_c(T) and the staggered magnetization M⊥(h)M_\perp(h) at hh close to hch_c. We apply the theory to Ba3_3Cr2_2O8_8 and determine exchange constants of the model by fitting the triplon spectrum obtained experimentally. It is demonstrated that in accordance with experimental data the system follows the 3D BEC scenario at T<1T<1 K only due to a pronounced anisotropy of the spectrum near its minimum. Our expressions for hsh_s, hc(T)h_c(T) and M⊥(h)M_\perp(h) fit well available experimental data.

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