Theoretical study on the variation of ordering vector in Ce(Pd1−x_{1-x}Mx_x)2_2Al3_3 (M=={Ag, Cu})

preprint2010arXivOpen access

Abstract

In heavy-fermion compounds, the crossover from the localized to itinerant heavy-fermion state is observed with lowering temperature, frequently accompanied by magnetism. Ordering vectors of magnetism often vary with applying pressure or with substituting atoms. In Ce(Pd1−x_{1-x}Mx_x)2_2Al3_3 with M=Ag,Cu\mathrm{M}=\mathrm{Ag,Cu}, the (0,0,1/2)(0,0,1/2)-antiferromagnetic (AF), ferromagnetic (F), and another AF orders are observed for x<0.05x<0.05, 0.1<x<0.40.1<x<0.4, and 0.5<x0.5<x, respectively. This change in the ordering vector is considered to be caused by the change in the conduction-band structures. Using the anisotropic RKKY interaction model reflecting the spacial anisotropic distribution of the ff states and also the conduction-band structures, % obtained by the band calculation, we study the change in the ordering vector of Ce(Pd1−x_{1-x}Mx_x)2_2Al3_3 with xx theoretically. As a result, the variation of the ordering vector is explained by treating the substitution of atoms as the conduction-electron doping, and the ordering vector of the AF state for x>0.5x>0.5 is considered to be (1/2,0,1/2)(1/2,0,1/2).

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