The nuclear spin-lattice relaxation rate in the PuMGa5_5 materials

preprint2006arXivOpen access

Abstract

We examine the nuclear spin-lattice relaxation rates 1/T11/T_1 of PuRhGa5_5 and PuCoGa5_5, both in the superconducting and normal states, as well as their Knight shifts. Results for both compounds are consistent with a superconducting gap of d-wave symmetry in the presence of strong impurity scattering, though with quite different gap-over-TcT_c ratios 2Δ0/kBTc2 Δ_{0}/ k_B T_c (8 for PuCoGa5_5 and 5 for PuRhGa5_5). In the normal state, PuRhGa5_5 exhibits a gradual suppression of (T1T)−1(T_1 T)^{-1} below 25 K, while measurements for PuCoGa5_5 reveal a monotonic increase down to TcT_c. We propose that this behavior is consistently understood by the crossover from the two-dimensional quantum antiferromagnetic regime of the local 5f5f-electron spins of Pu to the concomitant formation of the fermion pseudogap based on the two-component spin-fermion model.

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