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Staggered Spin Order of Localized pi-electrons in the Insulating State of the Organic Conductor kappa-BETS)2Mn[N(CN)2]3

Magnetic properties of the conduction pi-electron system of kappa-BETS)2Mn[N(CN)2]3 have been probed using 13C NMR. At ambient pressure, the metal-insulator transition observed in the resistivity measurements below T~23K is shown to be accompanied by ordering of the pi-spins in a long-range staggered structure. As the metal-insulator transition is suppressed by applying a small pressure of ~0.5 kbar, the pi-spin system maintains the properties of the metallic state down to 5K.

preprint2012arXivOpen access
O. M. VyaselevM. V. KartsovnikN. D. KushchE. B. Yagubskii
cond-mat.str-el
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O. M. VyaselevM. V. KartsovnikN. D. KushchE. B. Yagubskii

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