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Spectral origin of the colossal magnetodielectric effect in multiferroic DyMn2O5

The origin of the colossal magnetodielectric effect in DyMn2O5 [1] has been an outstanding question in multiferroics. Here, we report the activation of the electric dipole mode at 4-5 cm-1 in an applied magnetic field which fully accounts for the CMD effect. We examine two alternative explanations of this mode: an electromagnon and transitions between f-electron levels of Dy3+ ions. The experimental and theoretical evidence supports the electromagnon origin of the CMD effect.

preprint2014arXivOpen access
A. B. SushkovCh. KantM. SchieblA. M. ShuvaevAnna PimenovAndrei PimenovB. LorenzS. ParkS-W. CheongMaxim MostovoyH. D. Drew
cond-mat.str-el
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Open access11 authors1 topic
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A. B. SushkovCh. KantM. SchieblA. M. ShuvaevAnna PimenovAndrei PimenovB. LorenzS. ParkS-W. CheongMaxim MostovoyH. D. Drew

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