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Spatially Resolved Mapping of Local Polarization Dynamics in an Ergodic Phase of Ferroelectric Relaxor

Spatial variability of polarization relaxation kinetics in relaxor ferroelectric 0.9Pb(Mg1/3Nb2/3)O3-0.1PbTiO3 is studied using time-resolved Piezoresponse Force Microscopy. Local relaxation attributed to the reorientation of polar nanoregions is shown to follow stretched exponential dependence, exp(-(t/tau)^beta), with beta~~0.4, much larger than the macroscopic value determined from dielectric spectra (beta~~0.09). The spatial inhomogeneity of relaxation time distributions with the presence of 100-200 nm "fast" and "slow" regions is observed. The results are analyzed to map the Vogel-Fulcher temperatures on the nanoscale.

preprint2008arXivOpen access
S. V. KalininB. J. RodriguezJ. D. BudaiS. JesseA. N. MorozovskaA. A. BokovZ. -G. Ye
cond-mat.mtrl-sci
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S. V. KalininB. J. RodriguezJ. D. BudaiS. JesseA. N. MorozovskaA. A. BokovZ. -G. Ye

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