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Singlet-Triplet Excitations in the Unconventional Spin-Peierls System TiOBr

We have performed time-of-flight neutron scattering measurements on powder samples of the unconventional spin-Peierls compound TiOBr using the fine-resolution Fermi chopper spectrometer (SEQUOIA) at the SNS. These measurements reveal two branches of magnetic excitations within the commensurate and incommensurate spin-Peierls phases, which we associate with n = 1 and n = 2 triplet excitations out of the singlet ground state. These measurements represent the first direct measure of the singlet-triplet energy gap in TiOBr, which is determined to be Eg = 21.2 +/- 1.0 meV.

preprint2010arXivOpen access
J. P. ClancyB. D. GaulinC. P. AdamsG. E. GranrothA. I. KolesnikovT. E. SherlineF. C. Chou
cond-mat.str-el
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J. P. ClancyB. D. GaulinC. P. AdamsG. E. GranrothA. I. KolesnikovT. E. SherlineF. C. Chou

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