Simultaneous collapse of antiferroquadrupolar order and superconductivity in PrIr2_{2}Zn20_{20} by nonhydrostatic pressure

preprint2020arXivOpen access

Abstract

Superconductivity in PrIr2_{2}Zn20_{20} appears at Tc=0.05T_{\rm c} = 0.05 K in the presence of an antiferroquadrupolar order below TQ=0.11T_{\rm Q} = 0.11 K. We have studied pressure dependences of TcT_{\rm c}, TQT_{\rm Q}, and non-Fermi liquid behaviors in the resistivity ρ(T)ρ(T) by using two pressure transmitting media: argon maintaining highly hydrostatic pressure, and glycerol, which solidifies above 5 GPa producing nonhydrostatic pressure. Upon applying PP with argon up to 10.6 GPa, TcT_{\rm c} hardly changes, while TQT_{\rm Q} monotonically increases from 0.11 to 0.23 K. With glycerol, however, TQT_{\rm Q} and TcT_{\rm c} simultaneously fall below 0.04 K at 6.3 GPa. The contrasting results indicate that onsite quadrupolar fluctuations induce superconductivity in this compound.

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