Abstract
We provide a complete toolkit for coherent control experiments on the nano-scale. By exploiting the second harmonic emission from single (150 nm) nonlinear nano-particles, we show that ultrafast femtosecond laser pulses can be compressed and controlled in time with unprecedented spatial accuracy. The method is tested on various nano-particles of different sizes, shapes and materials, both dielectric BaTiO3, Fe(IO3)3) and metallic (Au) thus demonstrating its robustness and versatility.
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