Remarkably robust and correlated coherence and antiferromagnetism in (Ce1−x_{1-x}Lax_x)Cu2_2Ge2_2

preprint2015arXivOpen access

Abstract

We present magnetic susceptibility, resistivity, specific heat, and thermoelectric power measurements on (Ce1−x_{1-x}Lax_x)Cu2_2Ge2_2 single crystals (0 ≤x≤\leq x\leq 1). With La substitution, the antiferromagnetic temperature TNT_N is suppressed in an almost linear fashion and moves below 0.36 K, the base temperature of our measurements for x>x> 0.8. Surprisingly, in addition to robust antiferromagnetism, the system also shows low temperature coherent scattering below TcohT_{coh} up to ∼\sim 0.9 of La, indicating a small percolation limit ∼\sim 9%\% of Ce that separates a coherent regime from a single-ion Kondo impurity regime. TcohT_{coh} as a function of magnetic field was found to have different behavior for xx< 0.9 and xx> 0.9. Remarkably, (Tcoh)2(T_{coh})^2 at HH = 0 was found to be linearly proportional to TNT_N. The jump in the magnetic specific heat δCmδC_{m} at TNT_N as a function of TK/TNT_K/T_N for (Ce1−x_{1-x}Lax_x)Cu2_2Ge2_2 follows the theoretical prediction based on the molecular field calculation for the SS = 1/2 resonant level model.

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