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Pressure-induced metallization and structural phase transition of the Mott-Hubbard insulator TiOBr

We investigated the pressure-dependent optical response of the low-dimensional Mott-Hubbard insulator TiOBr by transmittance and reflectance measurements in the infrared and visible frequency range. A suppression of the transmittance above a critical pressure and a concomitant increase of the reflectance are observed, suggesting a pressure-induced metallization of TiOBr. The metallic phase of TiOBr at high pressure is confirmed by the presence of additional excitations extending down to the far-infrared range. The pressure-induced metallization coincides with a structural phase transition, according to the results of x-ray powder diffraction experiments under pressure.

preprint2007arXivOpen access
C. A. KuntscherS. FrankA. PashkinH. HoffmannA. SchönleberS. van SmaalenM. HanflandS. GlawionM. KlemmM. SingS. HornR. Claessen
cond-mat.str-el
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C. A. KuntscherS. FrankA. PashkinH. HoffmannA. SchönleberS. van SmaalenM. HanflandS. GlawionM. KlemmM. SingS. HornR. Claessen

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