Abstract

Three-dimensional (3D) antiferromagnets with random magnetic anisotropy (RMA) experimentally studied to date do not have random single-ion anisotropies, but rather have competing two-dimensional and three-dimensional exchange interactions which can obscure the authentic effects of RMA. The magnetic phase diagram Fex_{x}Ni1−x_{1-x}F2_{2} epitaxial thin films with true random single-ion anisotropy was deduced from magnetometry and neutron scattering measurements and analyzed using mean field theory. Regions with uniaxial, oblique and easy plane anisotropies were identified. A RMA-induced glass region was discovered where a Griffiths-like breakdown of long-range spin order occurs.

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