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On the Origin of Zigzag Magnetic Order in Iridium Oxide Na2IrO3

We explore the phase diagram of spin-orbit Mott insulators on a honeycomb lattice, within the Kitaev-Heisenberg model extended to its full parameter space. Zigzag-type magnetic order is found to occupy a large part of the phase diagram of the model, and its physical origin is explained as due to interorbital t2g-eg hopping. Magnetic susceptibility and spin wave spectra are calculated and compared to the experimental data, obtaining thereby the spin coupling constants in Na2IrO3 and Li2IrO3.

preprint2012arXivOpen access
Jiří ChaloupkaGeorge JackeliGiniyat Khaliullin
cond-mat.str-el
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Jiří ChaloupkaGeorge JackeliGiniyat Khaliullin

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