Abstract

Monolayer transition metal dichalcogenides (TMDCs), like MoS2_2, MoSe2_2, WS2_2, and WSe2_2, feature direct bandgaps, strong spin-orbit coupling, and exciton-polariton interactions at the atomic scale, which could be harnessed for efficient light emission, valleytronics, and polaritonic lasing, respectively. Nevertheless, to build next-generation photonic devices that make use of these features, it is first essential to model the all-optical control mechanisms in TMDCs. Herein, a simple model is proposed to quantify the performance of a 35 \,\textmu m long Si3_3N4_4 waveguide-integrated all-optical MoSe2_2 modulator. Using this model, a switching energy of 14.6 \,pJ is obtained for a transverse-magnetic (TM) and transverse-electric (TE) polarised pump signals at λ= λ=\,480 \,nm. Moreover, maximal extinction ratios of 20.6 \,dB and 20.1 \,dB are achieved for a TM and TE polarised probe signal at λ= λ=\,500 \,nm, respectively, with an ultra-low insertion loss of <0.3 <0.3\,dB. Moreover, the device operates with an ultrafast recovery time of 50 \,ps, while maintaining a high extinction ratio for practical applications. These findings facilitate modeling and designing novel TMDC-based photonic devices.

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