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Paper detail

Observation of Rayleigh optical activity for chiral molecules: a new chiroptical tool

By measuring a small circularly polarized component in the scattered light, we report the first observation of Rayleigh optical activity (RayOA) for isotropic samples of chiral molecules, namely the two enantiomers of $α$-pinene in neat liquid form. Our work validates fundamental theoretical predictions made over fifty years ago and expands the chiroptical toolkit.

preprint2025arXivOpen access
Duncan McArthurEmmanouil I. AlexakisAndrew R. PuenteRebecca McGonigleAndrew J. LovePrasad L. PolavarapuLaurence D. BarronLewis E. MacKenzieAidan S. ArnoldRobert P. Cameron
physics.atom-phphysics.ins-detBiological Physicsphysics.chem-phphysics.optics
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Open access10 authors5 topics
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Duncan McArthurEmmanouil I. AlexakisAndrew R. PuenteRebecca McGonigleAndrew J. LovePrasad L. PolavarapuLaurence D. BarronLewis E. MacKenzieAidan S. ArnoldRobert P. Cameron

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