Neutron-diffraction and linear {Grüneisen} parameter studies of magnetism in NdFe2_2Ga8_8

preprint2022arXivOpen access

Abstract

We study the magnetism in NdFe2_2Ga8_8 by the neutron-diffraction and temperature-modulated linear {Grüneisen} parameter measurements. Previous thermodynamical measurements have demonstrated that there are two magnetic transitions at 10 and 14.5 K, respectively. Neutron-diffraction measurements confirm that the lower one is an antiferromagnetic (AFM) transition with a commensurate magnetic structure. Both the commensurate and the incommensurate (IC) magnetic peaks are found below the higher transition but their intensities only gradually increase with decreasing temperature. Below 10 K, the commensurate peak intensity increases quickly with decreasing temperature, signaling the AFM transition, while the IC peak intensity disappears below 5 K. The linear {Grüneisen} parameter along the cc axis, ΓcΓ_c, shows a hysteresis behavior that is different from the hysteresis behavior for the magnetization MM. We give a discussion of the origin of the magnetism in NdFe2_2Ga8_8.

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