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Momentum dependence of orbital excitations in Mott-insulating titanates

High-resolution resonant inelastic x-ray scattering has been used to determine the momentum dependence of orbital excitations in Mott-insulating LaTiO$_3$ and YTiO$_3$ over a wide range of the Brillouin zone. The data are compared to calculations in the framework of lattice-driven and superexchange-driven orbital ordering models. A superexchange model in which the experimentally observed modes are attributed to two-orbiton excitations yields the best description of the data.

preprint2009arXivOpen access
C. UlrichL. J. P. AmentG. GhiringhelliL. BraicovichM. Moretti SalaN. PezzottaT. SchmittG. KhaliullinJ. van den BrinkH. RothT. LorenzB. Keimer
cond-mat.str-el
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Open access12 authors1 topic
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C. UlrichL. J. P. AmentG. GhiringhelliL. BraicovichM. Moretti SalaN. PezzottaT. SchmittG. KhaliullinJ. van den BrinkH. RothT. LorenzB. Keimer

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