Magnetic phase diagrams, domain switching and a quantum phase transition of the quasi-1D Ising-like antiferromagnet BaCo2V2O8

In the effective Ising spin-1/2 antiferromagnetic chain system BaCo$_2$V$_2$O$_8, the magnetic-field influence is highly anisotropic. For magnetic fields along the easy axis$c$, the Néel order is strongly suppressed already for low fields and an incommensurate order is entered above 4 T. We present a detailed study of the magnetic phase diagrams for different magnetic field directions, which are derived from magnetization data, high-resolution thermal expansion and magnetostriction measurements as well as from the thermal conductivity. Zero-field thermal expansion data reveal that the magnetic transition is accompanied by an orthorhombic distortion within the$ab$plane. Under ambient conditions the crystals are heavily twinned, but the domain orientation can be influenced either by applying uniaxial pressure or a magnetic field along the [100] direction. In addition, our data reveal a pronounced in-plane magnetic anisotropy for fields applied within the$ab$plane. For$H || [110]$, the magnetic field influence on T$_N$is weak, whereas for magnetic fields applied along [100], T$_N$vanishes at about 10 T and the zero-field Néel order is completely suppressed as is confirmed by neutron diffraction data. The second-order phase transition strongly suggests a quantum critical point being present at$H\simeq 10$ T parallel [100], where the Néel order probably changes to a spin-liquid state.

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