Low-Temperature Low-Field Phases of the Pyrochlore Quantum Magnet Tb2_2Ti2_2O7_7

preprint2013arXivOpen access

Abstract

By means of ac magnetic-susceptibility measurements, we find evidence for a new magnetic phase of Tb2_2Ti2_2O7_7 below about 140 mK in zero magnetic field. In magnetic fields parallel to [111], this phase---exhibiting frequency- and amplitude-dependent susceptibility and an extremely slow spin dynamics---extends to about 70 mT, at which it gives way to another phase. The field dependence of the susceptibility of this second phase, which extends to about 0.6 T, indicates the presence of a weak magnetization plateau below 50 mK, as has been predicted by a single-tetrahedron four-spin model, giving support to the underlying proposal that the disordered low-field ground state of Tb2_2Ti2_2O7_7 is a quantum spin ice.

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