Low temperature ferromagnetism in perovskite SrIrO3_3 films

preprint2021arXivOpen access

Abstract

The 5dd based SrIrO3_3 represents prototype example of nonmagnetic correlated metal which mainly originates from a combined effect of spin-orbit coupling, lattice dimensionality and crystal structure. Therefore, tuning of these parameters results in diverse physical properties in this material. Here, we study the structural, magnetic and electrical transport behavior in epitaxial SrIrO3_3 film (∼\sim 40 nm) grown on SrTiO3_3 substrate. Opposed to bulk material, the SrIrO3_3 film exhibits a ferromagnetic ordering at low temperature below ∼\sim 20 K. The electrical transport data indicate an insulating behavior where the nature of charge transport follows Mott's variable-range-hopping model. A positive magnetoresistance is recorded at 2 K which has correlation with magnetic moment. We further observe a nonlinear Hall effect at low temperature (<< 20 K) which arises due to an anomalous component of Hall effect. An anisotropic behavior of both magnetoresistance and Hall effect has been evidenced at low temperature which coupled with anomalous Hall effect indicate the development of ferromagnetic ordering. We believe that an enhanced (local) structural distortion caused by lattice strain at low temperatures induces ferromagnetic ordering, thus showing structural instability plays vital role to tune the physical properties in SrIrO3_3.

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