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Intrinsic Structural Disorder and the Magnetic Ground State in Bulk EuTiO3

The magnetic properties of single-crystal EuTiO3 are suggestive of nanoscale disorder below its cubic-tetragonal phase transition. We demonstrate that electric field cooling acts to restore monocrystallinity, thus confirming that emergent structural disorder is an intrinsic low-temperature property of this material. Using torque magnetometry, we deduce that tetragonal EuTiO3 enters an easy-axis antiferromagnetic phase at 5.6 K, with a first-order transition to an easy-plane ground state below 3 K. Our data is reproduced by a 3D anisotropic Heisenberg spin model.

preprint2012arXivOpen access
A. P. PetrovicY. KatoS. S. SunkuT. ItoP. SenguptaL. SpalekM. ShimutaT. KatsufujiC. D. BatistaS. SaxenaC. Panagopoulos
cond-mat.str-el
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Open access11 authors1 topic
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A. P. PetrovicY. KatoS. S. SunkuT. ItoP. SenguptaL. SpalekM. ShimutaT. KatsufujiC. D. BatistaS. SaxenaC. Panagopoulos

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